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Thermochemical analysis of premixed ammonia/biogas flames in a model gas turbine swirl combustion system

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Listed:
  • Zhao, Xu
  • Ng, Jo-Han
  • Mong, Guo Ren
  • Mashruk, Syed
  • Lee, Chew Tin
  • Fang, Xueliang
  • Wong, Keng Yinn
  • Ooi, Jong Boon
  • Valera-Medina, Agustin
  • Chiong, Meng-Choung

Abstract

This study examined the premixed NH3/biogas combustion at near stoichiometric using an experimentally validated numerical method. Raising the NH3 wt.% in NH3/CH4 combustion at φ = 0.8 brought up the average reaction temperature (Tavg) due to heat retention. Intensified by CO2 addition, Tavg in NH3/biogas increased by a factor of 1.2 compared to NH3/CH4. At φ = 1.1, higher NH3 and CO2 wt.% reduced Tavg. The local Damköhler number (Da) was reduced marginally in the absence of CO2 as φ increased from 0.8 to 1.1. Conversely, local Da grew considerably in the presence of CO2 and was particularly sensitive to variations in the excess air ratio. Increased NH3 wt.% promoted NO emission, primarily via N + OH → NO + H and H + HCNO → CH2 + NO pathways. NH3/biogas produced more NO than NH3/CH4 from φ = 0.9 to 1.1, but as φ approached 1.1, NO is generally lowered. N2O is produced mainly by NH + NO → N2O + H. Fuel-lean operation generally results in a higher N2O than fuel-rich operation. The NH3/biogas combustion at φ = 0.8 is a potential clean fuel solution in lowering NO emissions, as compared to NH3/CH4 combustion.

Suggested Citation

  • Zhao, Xu & Ng, Jo-Han & Mong, Guo Ren & Mashruk, Syed & Lee, Chew Tin & Fang, Xueliang & Wong, Keng Yinn & Ooi, Jong Boon & Valera-Medina, Agustin & Chiong, Meng-Choung, 2024. "Thermochemical analysis of premixed ammonia/biogas flames in a model gas turbine swirl combustion system," Renewable Energy, Elsevier, vol. 236(C).
    • Handle: RePEc:eee:renene:v:236:y:2024:i:c:s0960148124015465
    DOI: 10.1016/j.renene.2024.121478
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    References listed on IDEAS

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