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Alternative production of methanol from industrial CO2

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  • Meunier, Nicolas
  • Chauvy, Remi
  • Mouhoubi, Seloua
  • Thomas, Diane
  • De Weireld, Guy

Abstract

Carbon dioxide valorization into value added products have become subject to much study to reduce industrial CO2 emissions and fossil energy resource consumption. In this context, the purpose of this study is to evaluate and highlight the interest of CO2 conversion into methanol through a complete techno-economic and environmental assessment of the entire process chain. The integrated process, successfully implemented in Aspen Plus®, is designed to treat the CO2 coming from a conventional cement plant. A MEA-based CO2 capture process is considered, and the captured CO2 is then directly sent to the conversion unit for its catalytic conversion. Consequently, combining the two units leads to relevant integrations, especially regarding the reuse of the heat provided by the exothermal methanol reactions for the regeneration of the CO2 capture solvent. An economic assessment is proposed to estimate the operational and investment costs, as well as the net present value, which demonstrates that the economic feasibility strongly depends on electricity and H2 production costs. A Life Cycle Analysis method is finally performed to identify the main environmental hotspots. The underlying process design offers a significant reduction in greenhouse gases (besides other categories) when compared to the conventional fossil production from natural gas.

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  • Meunier, Nicolas & Chauvy, Remi & Mouhoubi, Seloua & Thomas, Diane & De Weireld, Guy, 2020. "Alternative production of methanol from industrial CO2," Renewable Energy, Elsevier, vol. 146(C), pages 1192-1203.
    • Handle: RePEc:eee:renene:v:146:y:2020:i:c:p:1192-1203
    DOI: 10.1016/j.renene.2019.07.010
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    10. Zhang, Zhien & Pan, Shu-Yuan & Li, Hao & Cai, Jianchao & Olabi, Abdul Ghani & Anthony, Edward John & Manovic, Vasilije, 2020. "Recent advances in carbon dioxide utilization," Renewable and Sustainable Energy Reviews, Elsevier, vol. 125(C).
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    12. Mancusi, E. & Bareschino, P. & Brachi, P. & Coppola, A. & Ruoppolo, G. & Urciuolo, M. & Pepe, F., 2021. "Feasibility of an integrated biomass-based CLC combustion and a renewable-energy-based methanol production systems," Renewable Energy, Elsevier, vol. 179(C), pages 29-36.
    13. Byun, Manhee & Kim, Heehyang & Lee, Hyunjun & Lim, Dongjun & Lim, Hankwon, 2022. "Conceptual design for methanol steam reforming in serial packed-bed reactors and membrane filters: Economic and environmental perspectives," Energy, Elsevier, vol. 241(C).
    14. Simon Pratschner & Pavel Skopec & Jan Hrdlicka & Franz Winter, 2021. "Power-to-Green Methanol via CO 2 Hydrogenation—A Concept Study including Oxyfuel Fluidized Bed Combustion of Biomass," Energies, MDPI, vol. 14(15), pages 1-33, July.
    15. Bakhtyari, Ali & Bardool, Roghayeh & Rahimpour, Mohammad Reza & Iulianelli, Adolfo, 2021. "Dehydration of bio-alcohols in an enhanced membrane-assisted reactor: A rigorous sensitivity analysis and multi-objective optimization," Renewable Energy, Elsevier, vol. 177(C), pages 519-543.
    16. Hosseinzadeh-Bandbafha, Homa & Tan, Yie Hua & Kansedo, Jibrail & Mubarak, N.M. & Liew, Rock Keey & Yek, Peter Nai Yuh & Aghbashlo, Mortaza & Ng, Hui Suan & Chong, William Woei Fong & Lam, Su Shiung & , 2023. "Assessing biodiesel production using palm kernel shell-derived sulfonated magnetic biochar from the life cycle assessment perspective," Energy, Elsevier, vol. 282(C).
    17. Latifah M. Alsarhan & Alhanouf S. Alayyar & Naif B. Alqahtani & Nezar H. Khdary, 2021. "Circular Carbon Economy (CCE): A Way to Invest CO 2 and Protect the Environment, a Review," Sustainability, MDPI, vol. 13(21), pages 1-25, October.
    18. Maqbool, Wahab & Kwon, Yuree & Im, Mintaek & An, Jinjoo, 2024. "Toward sustainable recycled methanol production from CO2 and steel by-product gases in South Korea; process design and assessment," Energy, Elsevier, vol. 301(C).
    19. Zhang, Zhiwei & Vo, Dat-Nguyen & Nguyen, Tuan B.H. & Sun, Jinsheng & Lee, Chang-Ha, 2024. "Advanced process integration and machine learning-based optimization to enhance techno-economic-environmental performance of CO2 capture and conversion to methanol," Energy, Elsevier, vol. 293(C).
    20. Gustafsson, Marcus & Cordova, Stephanie S. & Svensson, Niclas & Eklund, Mats, 2024. "Climate performance of liquefied biomethane with carbon dioxide utilization or storage," Renewable and Sustainable Energy Reviews, Elsevier, vol. 192(C).
    21. Adnan, Muflih A. & Kibria, Md Golam, 2020. "Comparative techno-economic and life-cycle assessment of power-to-methanol synthesis pathways," Applied Energy, Elsevier, vol. 278(C).
    22. Kotowicz, Janusz & Węcel, Daniel & Kwilinski, Aleksy & Brzęczek, Mateusz, 2022. "Efficiency of the power-to-gas-to-liquid-to-power system based on green methanol," Applied Energy, Elsevier, vol. 314(C).

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