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Transition metals supported on bone-derived hydroxyapatite as potential catalysts for the Water-Gas Shift reaction

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  • Iriarte-Velasco, Unai
  • Ayastuy, Jose L.
  • Boukha, Zouhair
  • Bravo, Raquel
  • Gutierrez-Ortiz, Miguel Ángel

Abstract

Calcined pork bone which is mainly composed by hydroxyapatite (HAp) was used as catalytic support of transition metals (Ni, Cu, Co, Fe) for WGS reaction. The catalysts were characterised by TGA, ICP, XRD, FTIR, H2-TPR, H2 chemisorption, OSC, CO2-TPD and N2 adsorption. The activity and selectivity was investigated and correlated with the chemical, structural and textural properties of the catalysts. For comparison, the performance of Ni loaded onto synthetic HAp was also investigated. The catalytic activity followed this trend: Ni > Co > Cu > Fe. Interestingly, natural support decreased methanation activity of Ni and increased stability as compared to synthetic HAp.

Suggested Citation

  • Iriarte-Velasco, Unai & Ayastuy, Jose L. & Boukha, Zouhair & Bravo, Raquel & Gutierrez-Ortiz, Miguel Ángel, 2018. "Transition metals supported on bone-derived hydroxyapatite as potential catalysts for the Water-Gas Shift reaction," Renewable Energy, Elsevier, vol. 115(C), pages 641-648.
    • Handle: RePEc:eee:renene:v:115:y:2018:i:c:p:641-648
    DOI: 10.1016/j.renene.2017.08.086
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    1. Nisar, Jan & Razaq, Rameez & Farooq, Muhammad & Iqbal, Munawar & Khan, Rafaqat Ali & Sayed, Murtaza & Shah, Afzal & Rahman, Inayat ur, 2017. "Enhanced biodiesel production from Jatropha oil using calcined waste animal bones as catalyst," Renewable Energy, Elsevier, vol. 101(C), pages 111-119.
    2. Farooq, Muhammad & Ramli, Anita & Naeem, Abdul, 2015. "Biodiesel production from low FFA waste cooking oil using heterogeneous catalyst derived from chicken bones," Renewable Energy, Elsevier, vol. 76(C), pages 362-368.
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