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Catalytic combustion of the retentate gas from a CO2/H2 separation membrane reactor for further CO2 enrichment and energy recovery

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Listed:
  • Hwang, Kyung-Ran
  • Park, Jin-Woo
  • Lee, Sung-Wook
  • Hong, Sungkook
  • Lee, Chun-Boo
  • Oh, Duck-Kyu
  • Jin, Min-Ho
  • Lee, Dong-Wook
  • Park, Jong-Soo

Abstract

The CCR (catalytic combustion reaction) of the retentate gas, consisting of 90% CO2 and 10% H2 obtained from a CO2/H2 separation membrane reactor, was investigated using a porous Ni metal catalyst in order to recover energy and further enrich CO2. A disc-shaped porous Ni metal catalyst, namely Al[0.1]/Ni, was prepared by a simple method and a compact MCR (micro-channel reactor) equipped with a catalyst plate was designed for the CCR. CO2 and H2 concentrations of 98.68% and 0.46%, respectively, were achieved at an operating temperature of 400 °C, GHSV (gas-hourly space velocity) of 50,000 h−1 and a H2/O2 ratio (R/O) of 2 in the unit module. In the case of the MCR, a sheet of the Ni metal catalyst was easily installed along with the other metal plates and the concentration of CO2 in the retentate gas increased up to 96.7%. The differences in temperatures measured before and after the CCR were 31 °C at the product outlet and 19 °C at the N2 outlet in the MCR. The disc-shaped porous metal catalyst and MCR configuration used in this study exhibit potential advantages, such as high thermal transfer resulting in improved energy recovery rate, simple catalyst preparation, and easy installation of the catalyst in the MCR.

Suggested Citation

  • Hwang, Kyung-Ran & Park, Jin-Woo & Lee, Sung-Wook & Hong, Sungkook & Lee, Chun-Boo & Oh, Duck-Kyu & Jin, Min-Ho & Lee, Dong-Wook & Park, Jong-Soo, 2015. "Catalytic combustion of the retentate gas from a CO2/H2 separation membrane reactor for further CO2 enrichment and energy recovery," Energy, Elsevier, vol. 90(P1), pages 1192-1198.
    • Handle: RePEc:eee:energy:v:90:y:2015:i:p1:p:1192-1198
    DOI: 10.1016/j.energy.2015.06.067
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    References listed on IDEAS

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    1. Olajire, Abass A., 2010. "CO2 capture and separation technologies for end-of-pipe applications – A review," Energy, Elsevier, vol. 35(6), pages 2610-2628.
    2. Lee, Sung-Wook & Park, Jong-Soo & Lee, Chun-Boo & Lee, Dong-Wook & Kim, Hakjoo & Ra, Ho Won & Kim, Sung-Hyun & Ryi, Shin-Kun, 2014. "H2 recovery and CO2 capture after water–gas shift reactor using synthesis gas from coal gasification," Energy, Elsevier, vol. 66(C), pages 635-642.
    3. Lee, Chun-Boo & Cho, Sung-Ho & Lee, Dong-Wook & Hwang, Kyung-Ran & Park, Jong-Soo & Kim, Sung-Hyun, 2014. "Combination of preferential CO oxidation and methanation in hybrid MCR (micro-channel reactor) for CO clean-up," Energy, Elsevier, vol. 78(C), pages 421-425.
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    1. Peydayesh, Mohammad & Mohammadi, Toraj & Bakhtiari, Omid, 2017. "Effective hydrogen purification from methane via polyimide Matrimid® 5218- Deca-dodecasil 3R type zeolite mixed matrix membrane," Energy, Elsevier, vol. 141(C), pages 2100-2107.
    2. Turi, Davide Maria & Chiesa, Paolo & Macchi, Ennio & Ghoniem, Ahmed F., 2016. "High fidelity model of the oxygen flux across ion transport membrane reactor: Mechanism characterization using experimental data," Energy, Elsevier, vol. 96(C), pages 127-141.
    3. Spallina, V. & Matturro, G. & Ruocco, C. & Meloni, E. & Palma, V. & Fernandez, E. & Melendez, J. & Pacheco Tanaka, A.D. & Viviente Sole, J.L. & van Sint Annaland, M. & Gallucci, F., 2018. "Direct route from ethanol to pure hydrogen through autothermal reforming in a membrane reactor: Experimental demonstration, reactor modelling and design," Energy, Elsevier, vol. 143(C), pages 666-681.

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