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H2 recovery and CO2 capture after water–gas shift reactor using synthesis gas from coal gasification

Author

Listed:
  • Lee, Sung-Wook
  • Park, Jong-Soo
  • Lee, Chun-Boo
  • Lee, Dong-Wook
  • Kim, Hakjoo
  • Ra, Ho Won
  • Kim, Sung-Hyun
  • Ryi, Shin-Kun

Abstract

In this study, a combined test of the WGS (water–gas shift) reactor and a Pd-based composite membrane was carried out for pre-combustion CO2 capture in a coal gasifier. The two series of WGS reactions, i.e., a high-temperature shift and a low-temperature shift, were performed under a gas composition of 60% CO and 40% H2 at 2100 kPa to imitate coal gasification. The CO2 enrichment and H2 recovery tests at 673 K and 2100 kPa with the high-pressure membrane module after the WGS reaction presented the enriched CO2 concentration and H2 recovery ratios of ∼92% and ∼96%, respectively. The long-term stability test showed that the CO2 concentration decreased to 78.2%, and CO was generated and reached to 8.8% in the retentate stream after 47 h because of reverse WGS and CO2 hydrogenation reaction on 316L stainless steel module. The stability test for ∼3137 h showed that these catalytic activities could be successfully prevented using steel with higher Cr and Ni contents, such as 310S. The WGS-membrane combination test using the outlet gas from a real coal gasifier was continued for ∼100 h and showed that the WGS catalysts and membrane module made of 310S would be stable under real conditions.

Suggested Citation

  • Lee, Sung-Wook & Park, Jong-Soo & Lee, Chun-Boo & Lee, Dong-Wook & Kim, Hakjoo & Ra, Ho Won & Kim, Sung-Hyun & Ryi, Shin-Kun, 2014. "H2 recovery and CO2 capture after water–gas shift reactor using synthesis gas from coal gasification," Energy, Elsevier, vol. 66(C), pages 635-642.
    • Handle: RePEc:eee:energy:v:66:y:2014:i:c:p:635-642
    DOI: 10.1016/j.energy.2014.01.043
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    References listed on IDEAS

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    1. Ryi, Shin-Kun & Lee, Chun-Boo & Lee, Sung-Wook & Hwang, Kyung-Ran & Park, Jong-Soo, 2012. "Hydrogen recovery from ethylene mixture with PD-AU composite membrane," Energy, Elsevier, vol. 47(1), pages 3-10.
    2. Irfan, Muhammad F. & Usman, Muhammad R. & Kusakabe, K., 2011. "Coal gasification in CO2 atmosphere and its kinetics since 1948: A brief review," Energy, Elsevier, vol. 36(1), pages 12-40.
    3. Ryi, Shin-Kun & Lee, Chun-Boo & Lee, Sung-Wook & Park, Jong-Soo, 2013. "Pd-based composite membrane and its high-pressure module for pre-combustion CO2 capture," Energy, Elsevier, vol. 51(C), pages 237-242.
    4. Kunze, Christian & Spliethoff, Hartmut, 2012. "Assessment of oxy-fuel, pre- and post-combustion-based carbon capture for future IGCC plants," Applied Energy, Elsevier, vol. 94(C), pages 109-116.
    5. Li, Bingyun & Duan, Yuhua & Luebke, David & Morreale, Bryan, 2013. "Advances in CO2 capture technology: A patent review," Applied Energy, Elsevier, vol. 102(C), pages 1439-1447.
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    Cited by:

    1. Gao, Wanlin & Zhou, Tuantuan & Gao, Yanshan & Wang, Qiang, 2019. "Enhanced water gas shift processes for carbon dioxide capture and hydrogen production," Applied Energy, Elsevier, vol. 254(C).
    2. Mohammad Fakhrulrezza & Joon Ahn & Hyun-Jin Lee, 2022. "Thermal Design of a Biohydrogen Production System Driven by Integrated Gasification Combined Cycle Waste Heat Using Dynamic Simulation," Energies, MDPI, vol. 15(9), pages 1-25, April.
    3. Hwang, Kyung-Ran & Park, Jin-Woo & Lee, Sung-Wook & Hong, Sungkook & Lee, Chun-Boo & Oh, Duck-Kyu & Jin, Min-Ho & Lee, Dong-Wook & Park, Jong-Soo, 2015. "Catalytic combustion of the retentate gas from a CO2/H2 separation membrane reactor for further CO2 enrichment and energy recovery," Energy, Elsevier, vol. 90(P1), pages 1192-1198.
    4. Theo, Wai Lip & Lim, Jeng Shiun & Hashim, Haslenda & Mustaffa, Azizul Azri & Ho, Wai Shin, 2016. "Review of pre-combustion capture and ionic liquid in carbon capture and storage," Applied Energy, Elsevier, vol. 183(C), pages 1633-1663.
    5. Obara, Shin'ya & Morel, Jorge & Okada, Masaki & Kobayashi, Kazuma, 2016. "Performance evaluation of an independent microgrid comprising an integrated coal gasification fuel cell combined cycle, large-scale photovoltaics, and a pumped-storage power station," Energy, Elsevier, vol. 116(P1), pages 78-93.
    6. Chen, Wei-Hsin & Kuo, Pei-Chi & Lin, Yu-Li, 2019. "Evolutionary computation for maximizing CO2 and H2 separation in multiple-tube palladium-membrane systems," Applied Energy, Elsevier, vol. 235(C), pages 299-310.

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