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Numerical investigation of oxygen permeation and methane oxy-combustion in a stagnation flow ion transport membrane reactor

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  • Ben Mansour, R.
  • Nemitallah, M.A.
  • Habib, M.A.

Abstract

In this work, a two-step oxy-combustion reaction kinetics model for methane-oxygen combustion is used to predict the oxy-combustion characteristics in the permeate side of the membrane. More accurate permeation rate characteristics inside this simple symmetric design ITM reactor is also expected using this model. New oxygen permeation model is introduced in this work for an LSCF-1991 ion transport membrane. The simulation of the oxygen permeation process across the membrane has been performed through series of visual C++ user defined function compiled and incorporated to FLUENT. The analysis of the permeation process has been conducted for separation only process (no reactions) using an inert gas (argon) as a sweep gas and a comparison has been done with cases of using CH4 plus CO2 as sweep gases. The effect of reactivity using the same sweep gases (CH4 plus CO2) is investigated by comparing the same cases with and without reactions in the permeate side. It was found that there are important parameters affecting the operation of ITM reactors like the inlet gases temperature, percentage of CH4 in the sweep gases mixture and the reactor geometry. Also, there are less important parameters like, feed and sweep volume flow rates, oxygen partial pressure in the feed side.

Suggested Citation

  • Ben Mansour, R. & Nemitallah, M.A. & Habib, M.A., 2013. "Numerical investigation of oxygen permeation and methane oxy-combustion in a stagnation flow ion transport membrane reactor," Energy, Elsevier, vol. 54(C), pages 322-332.
    • Handle: RePEc:eee:energy:v:54:y:2013:i:c:p:322-332
    DOI: 10.1016/j.energy.2013.03.027
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    References listed on IDEAS

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    1. Mancini, N.D. & Mitsos, A., 2011. "Ion transport membrane reactors for oxy-combustion–Part II: Analysis and comparison of alternatives," Energy, Elsevier, vol. 36(8), pages 4721-4739.
    2. Mancini, N.D. & Mitsos, A., 2011. "Ion transport membrane reactors for oxy-combustion – Part I: intermediate-fidelity modeling," Energy, Elsevier, vol. 36(8), pages 4701-4720.
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    4. Sjardin, M. & Damen, K.J. & Faaij, A.P.C., 2006. "Techno-economic prospects of small-scale membrane reactors in a future hydrogen-fuelled transportation sector," Energy, Elsevier, vol. 31(14), pages 2523-2555.
    5. Rahimpour, M.R. & Mirvakili, A. & Paymooni, K., 2011. "A novel water perm-selective membrane dual-type reactor concept for Fischer–Tropsch synthesis of GTL (gas to liquid) technology," Energy, Elsevier, vol. 36(2), pages 1223-1235.
    6. Perry, Simon & Klemeš, Jiří & Bulatov, Igor, 2008. "Integrating waste and renewable energy to reduce the carbon footprint of locally integrated energy sectors," Energy, Elsevier, vol. 33(10), pages 1489-1497.
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    1. Nemitallah, Medhat A. & Habib, Mohamed A. & Mezghani, K., 2015. "Experimental and numerical study of oxygen separation and oxy-combustion characteristics inside a button-cell LNO-ITM reactor," Energy, Elsevier, vol. 84(C), pages 600-611.
    2. Habib, Mohamed A. & Nemitallah, Medhat A., 2015. "Design of an ion transport membrane reactor for application in fire tube boilers," Energy, Elsevier, vol. 81(C), pages 787-801.
    3. Rashwan, Sherif S. & Ibrahim, Abdelmaged H. & Abou-Arab, Tharwat W. & Nemitallah, Medhat A. & Habib, Mohamed A., 2017. "Experimental study of atmospheric partially premixed oxy-combustion flames anchored over a perforated plate burner," Energy, Elsevier, vol. 122(C), pages 159-167.
    4. Shin, Donghwan & Kang, Sanggyu, 2018. "Numerical analysis of an ion transport membrane system for oxy–fuel combustion," Applied Energy, Elsevier, vol. 230(C), pages 875-888.
    5. Habib, Mohamed A. & Salaudeen, Shakirudeen A. & Nemitallah, Medhat A. & Ben-Mansour, R. & Mokheimer, Esmail M.A., 2016. "Numerical investigation of syngas oxy-combustion inside a LSCF-6428 oxygen transport membrane reactor," Energy, Elsevier, vol. 96(C), pages 654-665.

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