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A method based on impedance spectroscopy for predicting the behavior of novel ionic liquid-polymer inclusion membranes in microbial fuel cells

Author

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  • Salar-García, M.J.
  • Ortiz-Martínez, V.M.
  • de los Ríos, A.P.
  • Hernández-Fernández, F.J.

Abstract

MFCs (microbial fuel cells) are an emerging technology for simultaneous treatment of wastewater and energy recovery. These devices exploit microbial metabolism to generate electricity from organic matter. The separator is a critical factor in the design of MFCs as it plays a crucial role in the transport of protons from the anode to the cathode, affecting the performance of the cell. It is thus of interest to develop a method to predict the behavior of a separator before being used in MFCs. The present work proposes a new method based on spectroscopy to calculate the internal resistance of several PIMs (polymer inclusion membranes) based on ILs (ionic liquids) and predict their behavior as novel proton exchange membranes in MFCs. Four types of PIMs based on three different groups of ionic liquids were prepared and electrochemically characterized: Methyltrioctyl ammonium chloride, [MTOA+][Cl−], 1-methyl-3-octylimidazolium hexafluorophosphate, [OMIM+][PF6−], Tri-butylmethylphosphonium methylsulphate, [P4,4,4,1+][MeSO4−], and Triisobutyl-(methyl)-phosphonium tosylate, [PI4,I4,I4,1+][TOS−], some of which were patented by our research group to be used as separator in MFCs (P201330453). Finally, the PIMs were evaluated in MFCs for energy production and wastewater treatment and compared with Nafion®117. The results show that the [PI4,I4,I4,1+][TOS−]-based membrane outperformed the rest of separators in terms of power output.

Suggested Citation

  • Salar-García, M.J. & Ortiz-Martínez, V.M. & de los Ríos, A.P. & Hernández-Fernández, F.J., 2015. "A method based on impedance spectroscopy for predicting the behavior of novel ionic liquid-polymer inclusion membranes in microbial fuel cells," Energy, Elsevier, vol. 89(C), pages 648-654.
    • Handle: RePEc:eee:energy:v:89:y:2015:i:c:p:648-654
    DOI: 10.1016/j.energy.2015.05.149
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    References listed on IDEAS

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    1. Malik, Monu & Dincer, Ibrahim & Rosen, Marc A., 2015. "Development and analysis of a new renewable energy-based multi-generation system," Energy, Elsevier, vol. 79(C), pages 90-99.
    2. Suleman, F. & Dincer, I. & Agelin-Chaab, M., 2014. "Development of an integrated renewable energy system for multigeneration," Energy, Elsevier, vol. 78(C), pages 196-204.
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    Cited by:

    1. de Ramón-Fernández, A. & Salar-García, M.J. & Ruiz Fernández, D. & Greenman, J. & Ieropoulos, I.A., 2020. "Evaluation of artificial neural network algorithms for predicting the effect of the urine flow rate on the power performance of microbial fuel cells," Energy, Elsevier, vol. 213(C).
    2. Ortiz-Martínez, V.M. & Salar-García, M.J. & Touati, K. & Hernández-Fernández, F.J. & de los Ríos, A.P. & Belhoucine, F. & Berrabbah, A. Alioua, 2016. "Assessment of spinel-type mixed valence Cu/Co and Ni/Co-based oxides for power production in single-chamber microbial fuel cells," Energy, Elsevier, vol. 113(C), pages 1241-1249.
    3. Salar-García, M.J. & Ortiz-Martínez, V.M. & Baicha, Z. & de los Ríos, A.P. & Hernández-Fernández, F.J., 2016. "Scaled-up continuous up-flow microbial fuel cell based on novel embedded ionic liquid-type membrane-cathode assembly," Energy, Elsevier, vol. 101(C), pages 113-120.
    4. Liu, Jiaran & Tan, Jinzhu & Yang, Weizhan & Li, Yang & Wang, Chao, 2021. "Better electrochemical performance of PEMFC under a novel pneumatic clamping mechanism," Energy, Elsevier, vol. 229(C).
    5. Ortiz-Martínez, V.M. & Salar-García, M.J. & Hernández-Fernández, F.J. & de los Ríos, A.P., 2015. "Development and characterization of a new embedded ionic liquid based membrane-cathode assembly for its application in single chamber microbial fuel cells," Energy, Elsevier, vol. 93(P2), pages 1748-1757.

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