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Solar fuel processing efficiency for ceria redox cycling using alternative oxygen partial pressure reduction methods

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  • Lin, Meng
  • Haussener, Sophia

Abstract

Solar-driven non-stoichiometric thermochemical redox cycling of ceria for the conversion of solar energy into fuels shows promise in achieving high solar-to-fuel efficiency. This efficiency is significantly affected by the operating conditions, e.g. redox temperatures, reduction and oxidation pressures, solar irradiation concentration, or heat recovery effectiveness. We present a thermodynamic analysis of five redox cycle designs to investigate the effects of working conditions on the fuel production. We focused on the influence of approaches to reduce the partial pressure of oxygen in the reduction step, namely by mechanical approaches (sweep gassing or vacuum pumping), chemical approaches (chemical scavenger), and combinations thereof. The results indicated that the sweep gas schemes work more efficient at non-isothermal than isothermal conditions, and efficient gas phase heat recovery and sweep gas recycling was important to ensure efficient fuel processing. The vacuum pump scheme achieved best efficiencies at isothermal conditions, and at non-isothermal conditions heat recovery was less essential. The use of oxygen scavengers combined with sweep gas and vacuum pump schemes further increased the system efficiency. The present work can be used to predict the performance of solar-driven non-stoichiometric redox cycles and further offers quantifiable guidelines for system design and operation.

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  • Lin, Meng & Haussener, Sophia, 2015. "Solar fuel processing efficiency for ceria redox cycling using alternative oxygen partial pressure reduction methods," Energy, Elsevier, vol. 88(C), pages 667-679.
    • Handle: RePEc:eee:energy:v:88:y:2015:i:c:p:667-679
    DOI: 10.1016/j.energy.2015.06.006
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    1. Abanades, Stéphane & Charvin, Patrice & Flamant, Gilles & Neveu, Pierre, 2006. "Screening of water-splitting thermochemical cycles potentially attractive for hydrogen production by concentrated solar energy," Energy, Elsevier, vol. 31(14), pages 2805-2822.
    2. Lapp, J. & Davidson, J.H. & Lipiński, W., 2012. "Efficiency of two-step solar thermochemical non-stoichiometric redox cycles with heat recovery," Energy, Elsevier, vol. 37(1), pages 591-600.
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    2. Chen, Jing & Kong, Hui & Wang, Hongsheng, 2023. "A novel high-efficiency solar thermochemical cycle for fuel production based on chemical-looping cycle oxygen removal," Applied Energy, Elsevier, vol. 343(C).
    3. Lin, Meng & Reinhold, Jan & Monnerie, Nathalie & Haussener, Sophia, 2018. "Modeling and design guidelines for direct steam generation solar receivers," Applied Energy, Elsevier, vol. 216(C), pages 761-776.
    4. Kong, Hui & Hao, Yong & Jin, Hongguang, 2018. "Isothermal versus two-temperature solar thermochemical fuel synthesis: A comparative study," Applied Energy, Elsevier, vol. 228(C), pages 301-308.
    5. Xiangjun Yu & Wenlei Lian & Ke Gao & Zhixing Jiang & Cheng Tian & Nan Sun & Hangbin Zheng & Xinrui Wang & Chao Song & Xianglei Liu, 2022. "Solar Thermochemical CO 2 Splitting Integrated with Supercritical CO 2 Cycle for Efficient Fuel and Power Generation," Energies, MDPI, vol. 15(19), pages 1-20, October.
    6. Milanese, Marco & Colangelo, Gianpiero & Laforgia, Domenico & de Risi, Arturo, 2017. "Multi-parameter optimization of double-loop fluidized bed solar reactor for thermochemical fuel production," Energy, Elsevier, vol. 134(C), pages 919-932.
    7. Guo, Yongpeng & Chen, Jing & Song, Hualong & Zheng, Ke & Wang, Jian & Wang, Hongsheng & Kong, Hui, 2024. "A review of solar thermochemical cycles for fuel production," Applied Energy, Elsevier, vol. 357(C).
    8. Kong, Hui & Kong, Xianghui & Wang, Jian & Zhang, Jun, 2019. "Thermodynamic analysis of a solar thermochemical cycle-based direct coal liquefaction system for oil production," Energy, Elsevier, vol. 179(C), pages 1279-1287.
    9. Koepf, E. & Alxneit, I. & Wieckert, C. & Meier, A., 2017. "A review of high temperature solar driven reactor technology: 25years of experience in research and development at the Paul Scherrer Institute," Applied Energy, Elsevier, vol. 188(C), pages 620-651.
    10. Imponenti, Luca & Albrecht, Kevin J. & Kharait, Rounak & Sanders, Michael D. & Jackson, Gregory S., 2018. "Redox cycles with doped calcium manganites for thermochemical energy storage to 1000 °C," Applied Energy, Elsevier, vol. 230(C), pages 1-18.
    11. Wang, Hongsheng & Wang, Bingzheng & Qi, Xingyu & Wang, Jian & Yang, Rufan & Li, Duanxing & Hu, Xuejiao, 2021. "Innovative non–oxidative methane dehydroaromatization via solar membrane reactor," Energy, Elsevier, vol. 216(C).

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