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Air gasification of PVC (polyvinyl chloride)-containing plastic waste in a two-stage gasifier using Ca-based additives and Ni-loaded activated carbon for the production of clean and hydrogen-rich producer gas

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  • Cho, Min-Hwan
  • Choi, Young-Kon
  • Kim, Joo-Sik

Abstract

A plastic waste containing polyvinyl chloride was gasified in a two-stage gasifier consisting of a fluidized bed reactor and tar-cracking zone to produce a hydrogen-rich producer gas with low tar and HCl contents. In particular, this study investigated the effects of calcined Ca-based additives, especially oyster shells, and a Ni-loaded activated carbon on the chlorine and tar removal. Additionally, a ∼3 h gasification of the plastic waste was performed using a distributor with a large hole size to confirm the gasification stability. In the experiments, where 900 g activated carbon was applied, all the producer gases were free of tar. The maximum H2 content (30 vol.%) in the producer gas was obtained with 900 g of Ni-loaded activated carbon. Chlorine in the feed material was mainly distributed in char and condensate liquid. The HCl contents in the producer gases obtained with the calcined Ca-based additives including oyster shells were under 1 ppm. The ∼3 h gasification revealed that the gasification was stable in terms of tar content in producer gas and producer gas composition.

Suggested Citation

  • Cho, Min-Hwan & Choi, Young-Kon & Kim, Joo-Sik, 2015. "Air gasification of PVC (polyvinyl chloride)-containing plastic waste in a two-stage gasifier using Ca-based additives and Ni-loaded activated carbon for the production of clean and hydrogen-rich prod," Energy, Elsevier, vol. 87(C), pages 586-593.
    • Handle: RePEc:eee:energy:v:87:y:2015:i:c:p:586-593
    DOI: 10.1016/j.energy.2015.05.026
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    References listed on IDEAS

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    1. Cho, Min-Hwan & Mun, Tae-Young & Choi, Young-Kon & Kim, Joo-Sik, 2014. "Two-stage air gasification of mixed plastic waste: Olivine as the bed material and effects of various additives and a nickel-plated distributor on the tar removal," Energy, Elsevier, vol. 70(C), pages 128-134.
    2. Arena, Umberto & Di Gregorio, Fabrizio, 2014. "Energy generation by air gasification of two industrial plastic wastes in a pilot scale fluidized bed reactor," Energy, Elsevier, vol. 68(C), pages 735-743.
    3. Cho, Min-Hwan & Mun, Tae-Young & Kim, Joo-Sik, 2013. "Air gasification of mixed plastic wastes using calcined dolomite and activated carbon in a two-stage gasifier to reduce tar," Energy, Elsevier, vol. 53(C), pages 299-305.
    4. Cho, Min-Hwan & Mun, Tae-Young & Kim, Joo-Sik, 2013. "Production of low-tar producer gas from air gasification of mixed plastic waste in a two-stage gasifier using olivine combined with activated carbon," Energy, Elsevier, vol. 58(C), pages 688-694.
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    1. Jeong, Yong-Seong & Kim, Jong-Woo & Seo, Myung-Won & Mun, Tae-Young & Kim, Joo-Sik, 2021. "Characteristics of two-stage air gasification of polystyrene with active carbon as a tar removal agent," Energy, Elsevier, vol. 219(C).
    2. Lin, Chiou-Liang & Chou, Jing-Dong & Iu, Chi-Hou, 2020. "Effects of second-stage bed materials on hydrogen production in the syngas of a two-stage gasification process," Renewable Energy, Elsevier, vol. 154(C), pages 903-912.
    3. Li, Jinhu & Burra, Kiran Raj G. & Wang, Zhiwei & Liu, Xuan & Gupta, Ashwani K., 2021. "Co-gasification of high-density polyethylene and pretreated pine wood," Applied Energy, Elsevier, vol. 285(C).
    4. Jeong, Yong-Seong & Choi, Young-Kon & Kim, Joo-Sik, 2019. "Three-stage air gasification of waste polyethylene: In-situ regeneration of active carbon used as a tar removal additive," Energy, Elsevier, vol. 166(C), pages 335-342.
    5. Choi, Young-Kon & Mun, Tae-Young & Cho, Min-Hwan & Kim, Joo-Sik, 2016. "Gasification of dried sewage sludge in a newly developed three-stage gasifier: Effect of each reactor temperature on the producer gas composition and impurity removal," Energy, Elsevier, vol. 114(C), pages 121-128.
    6. Ichiro Tsuchimoto & Yuya Kajikawa, 2022. "Recycling of Plastic Waste: A Systematic Review Using Bibliometric Analysis," Sustainability, MDPI, vol. 14(24), pages 1-39, December.

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