IDEAS home Printed from https://ideas.repec.org/a/eee/energy/v87y2015icp586-593.html
   My bibliography  Save this article

Air gasification of PVC (polyvinyl chloride)-containing plastic waste in a two-stage gasifier using Ca-based additives and Ni-loaded activated carbon for the production of clean and hydrogen-rich producer gas

Author

Listed:
  • Cho, Min-Hwan
  • Choi, Young-Kon
  • Kim, Joo-Sik

Abstract

A plastic waste containing polyvinyl chloride was gasified in a two-stage gasifier consisting of a fluidized bed reactor and tar-cracking zone to produce a hydrogen-rich producer gas with low tar and HCl contents. In particular, this study investigated the effects of calcined Ca-based additives, especially oyster shells, and a Ni-loaded activated carbon on the chlorine and tar removal. Additionally, a ∼3 h gasification of the plastic waste was performed using a distributor with a large hole size to confirm the gasification stability. In the experiments, where 900 g activated carbon was applied, all the producer gases were free of tar. The maximum H2 content (30 vol.%) in the producer gas was obtained with 900 g of Ni-loaded activated carbon. Chlorine in the feed material was mainly distributed in char and condensate liquid. The HCl contents in the producer gases obtained with the calcined Ca-based additives including oyster shells were under 1 ppm. The ∼3 h gasification revealed that the gasification was stable in terms of tar content in producer gas and producer gas composition.

Suggested Citation

  • Cho, Min-Hwan & Choi, Young-Kon & Kim, Joo-Sik, 2015. "Air gasification of PVC (polyvinyl chloride)-containing plastic waste in a two-stage gasifier using Ca-based additives and Ni-loaded activated carbon for the production of clean and hydrogen-rich prod," Energy, Elsevier, vol. 87(C), pages 586-593.
  • Handle: RePEc:eee:energy:v:87:y:2015:i:c:p:586-593
    DOI: 10.1016/j.energy.2015.05.026
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0360544215006076
    Download Restriction: Full text for ScienceDirect subscribers only

    File URL: https://libkey.io/10.1016/j.energy.2015.05.026?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Arena, Umberto & Di Gregorio, Fabrizio, 2014. "Energy generation by air gasification of two industrial plastic wastes in a pilot scale fluidized bed reactor," Energy, Elsevier, vol. 68(C), pages 735-743.
    2. Cho, Min-Hwan & Mun, Tae-Young & Choi, Young-Kon & Kim, Joo-Sik, 2014. "Two-stage air gasification of mixed plastic waste: Olivine as the bed material and effects of various additives and a nickel-plated distributor on the tar removal," Energy, Elsevier, vol. 70(C), pages 128-134.
    3. Cho, Min-Hwan & Mun, Tae-Young & Kim, Joo-Sik, 2013. "Air gasification of mixed plastic wastes using calcined dolomite and activated carbon in a two-stage gasifier to reduce tar," Energy, Elsevier, vol. 53(C), pages 299-305.
    4. Cho, Min-Hwan & Mun, Tae-Young & Kim, Joo-Sik, 2013. "Production of low-tar producer gas from air gasification of mixed plastic waste in a two-stage gasifier using olivine combined with activated carbon," Energy, Elsevier, vol. 58(C), pages 688-694.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Jeong, Yong-Seong & Kim, Jong-Woo & Seo, Myung-Won & Mun, Tae-Young & Kim, Joo-Sik, 2021. "Characteristics of two-stage air gasification of polystyrene with active carbon as a tar removal agent," Energy, Elsevier, vol. 219(C).
    2. Lin, Chiou-Liang & Chou, Jing-Dong & Iu, Chi-Hou, 2020. "Effects of second-stage bed materials on hydrogen production in the syngas of a two-stage gasification process," Renewable Energy, Elsevier, vol. 154(C), pages 903-912.
    3. Li, Jinhu & Burra, Kiran Raj G. & Wang, Zhiwei & Liu, Xuan & Gupta, Ashwani K., 2021. "Co-gasification of high-density polyethylene and pretreated pine wood," Applied Energy, Elsevier, vol. 285(C).
    4. Jeong, Yong-Seong & Choi, Young-Kon & Kim, Joo-Sik, 2019. "Three-stage air gasification of waste polyethylene: In-situ regeneration of active carbon used as a tar removal additive," Energy, Elsevier, vol. 166(C), pages 335-342.
    5. Choi, Young-Kon & Mun, Tae-Young & Cho, Min-Hwan & Kim, Joo-Sik, 2016. "Gasification of dried sewage sludge in a newly developed three-stage gasifier: Effect of each reactor temperature on the producer gas composition and impurity removal," Energy, Elsevier, vol. 114(C), pages 121-128.
    6. Ichiro Tsuchimoto & Yuya Kajikawa, 2022. "Recycling of Plastic Waste: A Systematic Review Using Bibliometric Analysis," Sustainability, MDPI, vol. 14(24), pages 1-39, December.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Chen, Zhijie & Wei, Wei & Chen, Xueming & Liu, Yiwen & Shen, Yansong & Ni, Bing-Jie, 2024. "Upcycling of plastic wastes for hydrogen production: Advances and perspectives," Renewable and Sustainable Energy Reviews, Elsevier, vol. 195(C).
    2. Huang, Jijiang & Veksha, Andrei & Chan, Wei Ping & Giannis, Apostolos & Lisak, Grzegorz, 2022. "Chemical recycling of plastic waste for sustainable material management: A prospective review on catalysts and processes," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).
    3. Bassey, Uduak & Sarquah, Khadija & Hartmann, Michael & Tom, Abasi-ofon & Beck, Gesa & Antwi, Edward & Narra, Satyanarayana & Nelles, Michael, 2023. "Thermal treatment options for single-use, multilayered and composite waste plastics in Africa," Energy, Elsevier, vol. 270(C).
    4. Ichiro Tsuchimoto & Yuya Kajikawa, 2022. "Recycling of Plastic Waste: A Systematic Review Using Bibliometric Analysis," Sustainability, MDPI, vol. 14(24), pages 1-39, December.
    5. Choi, Young-Kon & Cho, Min-Hwan & Kim, Joo-Sik, 2015. "Steam/oxygen gasification of dried sewage sludge in a two-stage gasifier: Effects of the steam to fuel ratio and ash of the activated carbon on the production of hydrogen and tar removal," Energy, Elsevier, vol. 91(C), pages 160-167.
    6. Arena, Umberto & Di Gregorio, Fabrizio, 2014. "Energy generation by air gasification of two industrial plastic wastes in a pilot scale fluidized bed reactor," Energy, Elsevier, vol. 68(C), pages 735-743.
    7. Shahbaz, Muhammad & Al-Ansari, Tareq & Inayat, Muddasser & Sulaiman, Shaharin A. & Parthasarathy, Prakash & McKay, Gordon, 2020. "A critical review on the influence of process parameters in catalytic co-gasification: Current performance and challenges for a future prospectus," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).
    8. Choi, Min-Jun & Jeong, Yong-Seong & Kim, Joo-Sik, 2021. "Air gasification of polyethylene terephthalate using a two-stage gasifier with active carbon for the production of H2 and CO," Energy, Elsevier, vol. 223(C).
    9. Han, Si Woo & Lee, Jeong Jae & Tokmurzin, Diyar & Lee, Seok Hyeong & Nam, Ji Young & Park, Sung Jin & Ra, Ho Won & Mun, Tae-Young & Yoon, Sang Jun & Yoon, Sung Min & Moon, Ji Hong & Lee, Jae Goo & Kim, 2022. "Gasification characteristics of waste plastics (SRF) in a bubbling fluidized bed: Effects of temperature and equivalence ratio," Energy, Elsevier, vol. 238(PC).
    10. Jeong, Yong-Seong & Choi, Young-Kon & Kim, Joo-Sik, 2019. "Three-stage air gasification of waste polyethylene: In-situ regeneration of active carbon used as a tar removal additive," Energy, Elsevier, vol. 166(C), pages 335-342.
    11. Cho, Min-Hwan & Mun, Tae-Young & Choi, Young-Kon & Kim, Joo-Sik, 2014. "Two-stage air gasification of mixed plastic waste: Olivine as the bed material and effects of various additives and a nickel-plated distributor on the tar removal," Energy, Elsevier, vol. 70(C), pages 128-134.
    12. Inayat, Muddasser & Sulaiman, Shaharin A. & Kurnia, Jundika Candra & Shahbaz, Muhammad, 2019. "Effect of various blended fuels on syngas quality and performance in catalytic co-gasification: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 105(C), pages 252-267.
    13. Buentello-Montoya, D.A. & Duarte-Ruiz, C.A. & Maldonado-Escalante, J.F., 2023. "Co-gasification of waste PET, PP and biomass for energy recovery: A thermodynamic model to assess the produced syngas quality," Energy, Elsevier, vol. 266(C).
    14. David Antonio Buentello-Montoya & Miguel Ángel Armenta-Gutiérrez & Victor Manuel Maytorena-Soria, 2023. "Parametric Modelling Study to Determine the Feasibility of the Co-Gasification of Macroalgae and Plastics for the Production of Hydrogen-Rich Syngas," Energies, MDPI, vol. 16(19), pages 1-18, September.
    15. M. Shahabuddin & Tanvir Alam, 2022. "Gasification of Solid Fuels (Coal, Biomass and MSW): Overview, Challenges and Mitigation Strategies," Energies, MDPI, vol. 15(12), pages 1-20, June.
    16. Cho, Min-Hwan & Mun, Tae-Young & Kim, Joo-Sik, 2013. "Production of low-tar producer gas from air gasification of mixed plastic waste in a two-stage gasifier using olivine combined with activated carbon," Energy, Elsevier, vol. 58(C), pages 688-694.
    17. Ardolino, Filomena & Lodato, Concetta & Astrup, Thomas F. & Arena, Umberto, 2018. "Energy recovery from plastic and biomass waste by means of fluidized bed gasification: A life cycle inventory model," Energy, Elsevier, vol. 165(PB), pages 299-314.
    18. Sreejith, C.C. & Haridasan, Navaneeth & Muraleedharan, C. & Arun, P., 2014. "Allothermal air–steam gasification of biomass with CO2 (carbon dioxide) sorption: Performance prediction based on a chemical kinetic model," Energy, Elsevier, vol. 69(C), pages 399-408.
    19. Parrillo, Francesco & Ardolino, Filomena & Boccia, Carmine & Calì, Gabriele & Marotto, Davide & Pettinau, Alberto & Arena, Umberto, 2023. "Co-gasification of plastics waste and biomass in a pilot scale fluidized bed reactor," Energy, Elsevier, vol. 273(C).
    20. Rizkiana, Jenny & Guan, Guoqing & Widayatno, Wahyu Bambang & Hao, Xiaogang & Li, Xiumin & Huang, Wei & Abudula, Abuliti, 2014. "Promoting effect of various biomass ashes on the steam gasification of low-rank coal," Applied Energy, Elsevier, vol. 133(C), pages 282-288.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:energy:v:87:y:2015:i:c:p:586-593. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.journals.elsevier.com/energy .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.