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Activated carbon nanotubes/polyaniline composites as supercapacitor electrodes

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  • Lee, Seul-Yi
  • Kim, Ji-Il
  • Park, Soo-Jin

Abstract

Chemically A-MWCNT (activated multiwalled carbon nanotube)/PANI (polyaniline) composites produced via ultrasonic polymerization of an aniline monomer in the presence of A-MWCNTs were investigated as potential electrode materials for supercapacitors. These composites were compared to pristine MWCNTs and MWCNT/PANI composites. The influence of the pore structure, which developed because of the polymerization process, was investigated by measuring N2 adsorption/desorption isotherms at 77 K. The electrochemical properties of the materials were determined by cyclic voltammetry and galvanostatic charge–discharge cycling measurements in 1 M NaNO3 electrolyte solution, using a three-electrode system at room temperature. The results suggested that the pore structure of the A-MWCNTs could effectively promote the homogenous-dispersion of aniline and consequently result in excellent cycling performance. Furthermore, interaction between the π-conjugated structure of carbon and the quinoid ring of the PANI matrix can lead to enhancement in the charge transfer process.

Suggested Citation

  • Lee, Seul-Yi & Kim, Ji-Il & Park, Soo-Jin, 2014. "Activated carbon nanotubes/polyaniline composites as supercapacitor electrodes," Energy, Elsevier, vol. 78(C), pages 298-303.
    • Handle: RePEc:eee:energy:v:78:y:2014:i:c:p:298-303
    DOI: 10.1016/j.energy.2014.10.011
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    1. Christinelli, W.A. & da Trindade, L.G. & Trench, A.B. & Quintans, C.S. & Paranhos, C.M. & Pereira, E.C., 2017. "High-performance energy storage of poly (o-methoxyaniline) film using an ionic liquid as electrolyte," Energy, Elsevier, vol. 141(C), pages 1829-1835.
    2. Shao, Zhou & Li, Hongji & Li, Mingji & Li, Cuiping & Qu, Changqing & Yang, Baohe, 2015. "Fabrication of polyaniline nanowire/TiO2 nanotube array electrode for supercapacitors," Energy, Elsevier, vol. 87(C), pages 578-585.
    3. Miao, Fujun & Shao, Changlu & Li, Xinghua & Lu, Na & Wang, Kexin & Zhang, Xin & Liu, Yichun, 2016. "Polyaniline-coated electrospun carbon nanofibers with high mass loading and enhanced capacitive performance as freestanding electrodes for flexible solid-state supercapacitors," Energy, Elsevier, vol. 95(C), pages 233-241.
    4. Yuan, Chuanjun & Lin, Haibo & Lu, Haiyan & Xing, Endong & Zhang, Yusi & Xie, Bingyao, 2016. "Synthesis of hierarchically porous MnO2/rice husks derived carbon composite as high-performance electrode material for supercapacitors," Applied Energy, Elsevier, vol. 178(C), pages 260-268.
    5. Mirzaeian, Mojtaba & Abbas, Qaisar & Gibson, Des & Mazur, Michal, 2019. "Effect of nitrogen doping on the electrochemical performance of resorcinol-formaldehyde based carbon aerogels as electrode material for supercapacitor applications," Energy, Elsevier, vol. 173(C), pages 809-819.
    6. Chen, Yingwen & Xu, Yuan & Chen, Liuliu & Li, Peiwen & Zhu, Shemin & Shen, Shubao, 2015. "Microbial electrolysis cells with polyaniline/multi-walled carbon nanotube-modified biocathodes," Energy, Elsevier, vol. 88(C), pages 377-384.
    7. Bavio, M.A. & Acosta, G.G. & Kessler, T. & Visintin, A., 2017. "Flexible symmetric and asymmetric supercapacitors based in nanocomposites of carbon cloth/polyaniline - carbon nanotubes," Energy, Elsevier, vol. 130(C), pages 22-28.
    8. Raoof, Jahan-Bakhsh & Hosseini, Sayed Reza & Ojani, Reza & Mandegarzad, Sakineh, 2015. "MOF-derived Cu/nanoporous carbon composite and its application for electro-catalysis of hydrogen evolution reaction," Energy, Elsevier, vol. 90(P1), pages 1075-1081.

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