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Study on the gasification of wastepaper/carbon dioxide catalyzed by molten carbonate salts

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  • Jin, Gong
  • Iwaki, Hiroyuki
  • Arai, Norio
  • Kitagawa, Kuniyuki

Abstract

This study focuses on waste paper gasification in carbon dioxide atmosphere with molten alkali carbonates including potassium, sodium, lithium carbonate or their intermixtures as catalyst. The molten catalysts is capable of facilitating a desired reaction (C+CO2→2CO), which was hardly feasible even at a high temperature of 973K if catalyst absences. It is that the catalysts which provides a gas–liquid interface between carbon and carbon dioxide, replacing original gas–solid, then allows the two reactants contact each other effectively. Further experimental results demonstrate that the intermixture carbonates exhibit strongly enhancement on catalytic activity than any carbonate salts in the form of single. The reaction rate depends on temperature evaluating manners, a rapid heating processes is favorable to the aimed reaction. With respect to recycling of carbon dioxide, the process provides a conversion in 30%.

Suggested Citation

  • Jin, Gong & Iwaki, Hiroyuki & Arai, Norio & Kitagawa, Kuniyuki, 2005. "Study on the gasification of wastepaper/carbon dioxide catalyzed by molten carbonate salts," Energy, Elsevier, vol. 30(7), pages 1192-1203.
    • Handle: RePEc:eee:energy:v:30:y:2005:i:7:p:1192-1203
    DOI: 10.1016/j.energy.2004.08.002
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    References listed on IDEAS

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    1. R. D. Cortright & R. R. Davda & J. A. Dumesic, 2002. "Hydrogen from catalytic reforming of biomass-derived hydrocarbons in liquid water," Nature, Nature, vol. 418(6901), pages 964-967, August.
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    1. Yuan, Hongyou & Wu, Shubin & Yin, Xiuli & Huang, Yanqin & Guo, Daliang & Wu, Chuangzhi, 2018. "Adjustment of biomass product gas to raise H2/CO ratio and remove tar over sodium titanate catalysts," Renewable Energy, Elsevier, vol. 115(C), pages 288-298.
    2. Chen, Wei-Hsin & Lin, Bo-Jhih, 2013. "Hydrogen and synthesis gas production from activated carbon and steam via reusing carbon dioxide," Applied Energy, Elsevier, vol. 101(C), pages 551-559.
    3. Backer, Michael & Gladen, Adam, 2023. "Impact of salt composition and temperature on low-temperature torrefaction of pine in molten nitrate salts," Energy, Elsevier, vol. 263(PE).
    4. Li, Jun & Xie, Yingpu & Zeng, Kuo & Flamant, Gilles & Yang, Haiping & Yang, Xinyi & Zhong, Dian & Du, Zhenyi & Chen, Hanping, 2020. "Biomass gasification in molten salt for syngas production," Energy, Elsevier, vol. 210(C).
    5. Anis, Samsudin & Zainal, Z.A., 2011. "Tar reduction in biomass producer gas via mechanical, catalytic and thermal methods: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(5), pages 2355-2377, June.
    6. Masnadi, Mohammad S. & Grace, John R. & Bi, Xiaotao T. & Lim, C. Jim & Ellis, Naoko & Li, Yong Hua & Watkinson, A. Paul, 2015. "From coal towards renewables: Catalytic/synergistic effects during steam co-gasification of switchgrass and coal in a pilot-scale bubbling fluidized bed," Renewable Energy, Elsevier, vol. 83(C), pages 918-930.
    7. Han, Jun & Kim, Heejoon, 2008. "The reduction and control technology of tar during biomass gasification/pyrolysis: An overview," Renewable and Sustainable Energy Reviews, Elsevier, vol. 12(2), pages 397-416, February.
    8. Masnadi, Mohammad S. & Grace, John R. & Bi, Xiaotao T. & Lim, C. Jim & Ellis, Naoko & Li, Yong Hua & Watkinson, A. Paul, 2015. "Single-fuel steam gasification of switchgrass and coal in a bubbling fluidized bed: A comprehensive parametric reference for co-gasification study," Energy, Elsevier, vol. 80(C), pages 133-147.
    9. Rizkiana, Jenny & Guan, Guoqing & Widayatno, Wahyu Bambang & Hao, Xiaogang & Wang, Zhongde & Zhang, Zhonglin & Abudula, Abuliti, 2015. "Oil production from mild pyrolysis of low-rank coal in molten salts media," Applied Energy, Elsevier, vol. 154(C), pages 944-950.
    10. Zhang, Shangzhong & Yoshikawa, Kunio & Nakagome, Hideki & Kamo, Tohru, 2013. "Kinetics of the steam gasification of a phenolic circuit board in the presence of carbonates," Applied Energy, Elsevier, vol. 101(C), pages 815-821.
    11. Hathaway, Brandon J. & Honda, Masanori & Kittelson, David B. & Davidson, Jane H., 2013. "Steam gasification of plant biomass using molten carbonate salts," Energy, Elsevier, vol. 49(C), pages 211-217.

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