IDEAS home Printed from https://ideas.repec.org/a/eee/energy/v300y2024ics0360544224013331.html
   My bibliography  Save this article

A comparative study on multidimensional signal evolution during thermal runaway of lithium-ion batteries with various cathode materials

Author

Listed:
  • Li, Kuijie
  • Gao, Xinlei
  • Peng, Shijian
  • Wang, Shengshi
  • Zhang, Weixin
  • Liu, Peng
  • Wu, Weixiong
  • Wang, Huizhi
  • Wang, Yu
  • Feng, Xuning
  • Cao, Yuan-cheng
  • Wen, Jinyu
  • Cheng, Shijie
  • Ouyang, Minggao

Abstract

Cathode materials significantly affect the failure behavior of lithium-ion batteries, but there is a lack of comparative research on the multidimensional signal evolution for batteries with various cathode materials when subjected to thermal runaway (TR). This study investigates the effect of cathode materials on battery safety properties by conducting overheating and overcharging abuse experiments on LiNixCoyMn(1-x-y)O2 (NCM 523, 622, and 811) as well as LiFePO4 (LFP) batteries. The multidimensional signals, including expansion force, gas concentrations, temperature, and voltage, are comprehensively and quantitatively analyzed. The results demonstrate that expansion force shows the earliest anomalies regardless of the cathode material in both abuse conditions. Gas can be detected after venting, followed by significant anomalies in voltage and temperature. Additionally, under overheating conditions, LFP cells exhibit the longest TR warning time of 677 s. However, the force anomaly-based warning method is more suitable for low-nickel NCM cells under overcharging scenarios. Specifically, NCM 523 cells achieve an overcharging warning time of 992 s at temperatures as low as 42.9 °C, and hold the highest venting force of 9859 N and venting temperature at 114.1 °C. On this basis, a hierarchical warning strategy based on multidimensional signal fusion is proposed. This study provides valuable insights into TR early warning and safety management in LIBs with different cathode materials.

Suggested Citation

  • Li, Kuijie & Gao, Xinlei & Peng, Shijian & Wang, Shengshi & Zhang, Weixin & Liu, Peng & Wu, Weixiong & Wang, Huizhi & Wang, Yu & Feng, Xuning & Cao, Yuan-cheng & Wen, Jinyu & Cheng, Shijie & Ouyang, M, 2024. "A comparative study on multidimensional signal evolution during thermal runaway of lithium-ion batteries with various cathode materials," Energy, Elsevier, vol. 300(C).
    • Handle: RePEc:eee:energy:v:300:y:2024:i:c:s0360544224013331
    DOI: 10.1016/j.energy.2024.131560
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0360544224013331
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.energy.2024.131560?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Hu, Jian & Tang, Xiaojie & Zhu, Xiaolong & Liu, Tong & Wang, Xishi, 2024. "Suppression of thermal runaway induced by thermal abuse in large-capacity lithium-ion batteries with water mist," Energy, Elsevier, vol. 286(C).
    2. Li, Kuijie & Chen, Long & Gao, Xinlei & Lu, Yao & Wang, Depeng & Zhang, Weixin & Wu, Weixiong & Han, Xuebing & Cao, Yuan-cheng & Wen, Jinyu & Cheng, Shijie & Ouyang, Minggao, 2024. "Implementing expansion force-based early warning in LiFePO4 batteries with various states of charge under thermal abuse scenarios," Applied Energy, Elsevier, vol. 362(C).
    3. Feng, Xuning & Lu, Languang & Ouyang, Minggao & Li, Jiangqiu & He, Xiangming, 2016. "A 3D thermal runaway propagation model for a large format lithium ion battery module," Energy, Elsevier, vol. 115(P1), pages 194-208.
    4. Ouyang, Nan & Zhang, Wencan & Yin, Xiuxing & Li, Xingyao & Xie, Yi & He, Hancheng & Long, Zhuoru, 2023. "A data-driven method for predicting thermal runaway propagation of battery modules considering uncertain conditions," Energy, Elsevier, vol. 273(C).
    5. Xu, Chengshan & Wang, Huaibin & Jiang, Fachao & Feng, Xuning & Lu, Languang & Jin, Changyong & Zhang, Fangshu & Huang, Wensheng & Zhang, Mengqi & Ouyang, Minggao, 2023. "Modelling of thermal runaway propagation in lithium-ion battery pack using reduced-order model," Energy, Elsevier, vol. 268(C).
    6. Mao, Ning & Zhang, Teng & Wang, Zhirong & Gadkari, Siddharth & Wang, Junling & He, Tengfei & Gao, Tianfeng & Cai, Qiong, 2023. "Revealing the thermal stability and component heat contribution ratio of overcharged lithium-ion batteries during thermal runaway," Energy, Elsevier, vol. 263(PD).
    7. Jia, Zhuangzhuang & Huang, Zonghou & Zhai, Hongju & Qin, Pen & Zhang, Yue & Li, Yawen & Wang, Qingsong, 2022. "Experimental investigation on thermal runaway propagation of 18,650 lithium-ion battery modules with two cathode materials at low pressure," Energy, Elsevier, vol. 251(C).
    8. Zhang, Yue & Cheng, Siyuan & Mei, Wenxin & Jiang, Lihua & Jia, Zhuangzhuang & Cheng, Zhixiang & Sun, Jinhua & Wang, Qingsong, 2023. "Understanding of thermal runaway mechanism of LiFePO4 battery in-depth by three-level analysis," Applied Energy, Elsevier, vol. 336(C).
    9. Wei, Gang & Huang, Ranjun & Zhang, Guangxu & Jiang, Bo & Zhu, Jiangong & Guo, Yangyang & Han, Guangshuai & Wei, Xuezhe & Dai, Haifeng, 2023. "A comprehensive insight into the thermal runaway issues in the view of lithium-ion battery intrinsic safety performance and venting gas explosion hazards," Applied Energy, Elsevier, vol. 349(C).
    10. Chen, Siqi & Wei, Xuezhe & Zhang, Guangxu & Rui, Xinyu & Xu, Chengshan & Feng, Xuning & Dai, Haifeng & Ouyang, Minggao, 2023. "Active and passive safety enhancement for batteries from force perspective," Renewable and Sustainable Energy Reviews, Elsevier, vol. 187(C).
    11. He, C.X. & Yue, Q.L. & Chen, Q. & Zhao, T.S., 2022. "Modeling thermal runaway of lithium-ion batteries with a venting process," Applied Energy, Elsevier, vol. 327(C).
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Li, Kuijie & Chen, Long & Gao, Xinlei & Lu, Yao & Wang, Depeng & Zhang, Weixin & Wu, Weixiong & Han, Xuebing & Cao, Yuan-cheng & Wen, Jinyu & Cheng, Shijie & Ouyang, Minggao, 2024. "Implementing expansion force-based early warning in LiFePO4 batteries with various states of charge under thermal abuse scenarios," Applied Energy, Elsevier, vol. 362(C).
    2. Zhang, Yue & Song, Laifeng & Tian, Jiamin & Mei, Wenxin & Jiang, Lihua & Sun, Jinhua & Wang, Qingsong, 2024. "Modeling the propagation of internal thermal runaway in lithium-ion battery," Applied Energy, Elsevier, vol. 362(C).
    3. Wang, Gongquan & Ping, Ping & Peng, Rongqi & Lv, Hongpeng & Zhao, Hengle & Gao, Wei & Kong, Depeng, 2023. "A semi reduced-order model for multi-scale simulation of fire propagation of lithium-ion batteries in energy storage system," Renewable and Sustainable Energy Reviews, Elsevier, vol. 186(C).
    4. Xu, Chengshan & Wang, Huaibin & Jiang, Fachao & Feng, Xuning & Lu, Languang & Jin, Changyong & Zhang, Fangshu & Huang, Wensheng & Zhang, Mengqi & Ouyang, Minggao, 2023. "Modelling of thermal runaway propagation in lithium-ion battery pack using reduced-order model," Energy, Elsevier, vol. 268(C).
    5. Ostanek, Jason K. & Li, Weisi & Mukherjee, Partha P. & Crompton, K.R. & Hacker, Christopher, 2020. "Simulating onset and evolution of thermal runaway in Li-ion cells using a coupled thermal and venting model," Applied Energy, Elsevier, vol. 268(C).
    6. Sheng Yang & Wenwei Wang & Cheng Lin & Weixiang Shen & Yiding Li, 2019. "Investigation of Internal Short Circuits of Lithium-Ion Batteries under Mechanical Abusive Conditions," Energies, MDPI, vol. 12(10), pages 1-16, May.
    7. Wei, Gang & Huang, Ranjun & Zhang, Guangxu & Jiang, Bo & Zhu, Jiangong & Guo, Yangyang & Han, Guangshuai & Wei, Xuezhe & Dai, Haifeng, 2023. "A comprehensive insight into the thermal runaway issues in the view of lithium-ion battery intrinsic safety performance and venting gas explosion hazards," Applied Energy, Elsevier, vol. 349(C).
    8. Jin, Changyong & Sun, Yuedong & Wang, Huaibin & Zheng, Yuejiu & Wang, Shuyu & Rui, Xinyu & Xu, Chengshan & Feng, Xuning & Wang, Hewu & Ouyang, Minggao, 2022. "Heating power and heating energy effect on the thermal runaway propagation characteristics of lithium-ion battery module: Experiments and modeling," Applied Energy, Elsevier, vol. 312(C).
    9. Luo, Pan & Gao, Kai & Hu, Lin & Chen, Bin & Zhang, Yuanjian, 2024. "Adaptive hybrid cooling strategy to mitigate battery thermal runaway considering natural convection in phase change material," Applied Energy, Elsevier, vol. 361(C).
    10. Meng, Jinhao & Cai, Lei & Stroe, Daniel-Ioan & Luo, Guangzhao & Sui, Xin & Teodorescu, Remus, 2019. "Lithium-ion battery state-of-health estimation in electric vehicle using optimized partial charging voltage profiles," Energy, Elsevier, vol. 185(C), pages 1054-1062.
    11. Ma, Mina & Wang, Yu & Duan, Qiangling & Wu, Tangqin & Sun, Jinhua & Wang, Qingsong, 2018. "Fault detection of the connection of lithium-ion power batteries in series for electric vehicles based on statistical analysis," Energy, Elsevier, vol. 164(C), pages 745-756.
    12. Coman, Paul T. & Darcy, Eric C. & Veje, Christian T. & White, Ralph E., 2017. "Numerical analysis of heat propagation in a battery pack using a novel technology for triggering thermal runaway," Applied Energy, Elsevier, vol. 203(C), pages 189-200.
    13. Meng, Lingyu & See, K.W. & Wang, Guofa & Wang, Yunpeng & Zhang, Yong & Zang, Caiyun & Xie, Bin, 2022. "Explosion-proof lithium-ion battery pack – In-depth investigation and experimental study on the design criteria," Energy, Elsevier, vol. 249(C).
    14. Xie, Jiekai & Luo, Yunjun & Zhang, Guoqing & Mo, Chongmao & Yang, Xiaoqing, 2024. "Compact design of integrated battery thermal management systems enabled by bi-functional heating-cooling plates and temperature-equalizing strategy," Renewable Energy, Elsevier, vol. 222(C).
    15. Zhu, Xiaoqing & Wang, Zhenpo & Wang, Yituo & Wang, Hsin & Wang, Cong & Tong, Lei & Yi, Mi, 2019. "Overcharge investigation of large format lithium-ion pouch cells with Li(Ni0.6Co0.2Mn0.2)O2 cathode for electric vehicles: Thermal runaway features and safety management method," Energy, Elsevier, vol. 169(C), pages 868-880.
    16. Yi, Yahui & Xia, Chengyu & Shi, Lei & Meng, Leifeng & Chi, Qifu & Qian, Liqin & Ma, Tiancai & Chen, Siqi, 2024. "Lithium-ion battery expansion mechanism and Gaussian process regression based state of charge estimation with expansion characteristics," Energy, Elsevier, vol. 292(C).
    17. Zhang, Liwen & Zhao, Peng & Xu, Meng & Wang, Xia, 2020. "Computational identification of the safety regime of Li-ion battery thermal runaway," Applied Energy, Elsevier, vol. 261(C).
    18. Jia, Zhuangzhuang & Song, Laifeng & Mei, Wenxin & Yu, Yin & Meng, Xiangdong & Jin, Kaiqiang & Sun, Jinhua & Wang, Qingsong, 2022. "The preload force effect on the thermal runaway and venting behaviors of large-format prismatic LiFePO4 batteries," Applied Energy, Elsevier, vol. 327(C).
    19. Xinyu Liu & Zhifu Zhou & Weitao Wu & Linsong Gao & Yang Li & Heng Huang & Zheng Huang & Yubai Li & Yongchen Song, 2022. "Three-Dimensional Modeling for the Internal Shorting Caused Thermal Runaway Process in 20Ah Lithium-Ion Battery," Energies, MDPI, vol. 15(19), pages 1-25, September.
    20. Ardani, M.I. & Patel, Y. & Siddiq, A. & Offer, G.J. & Martinez-Botas, R.F., 2018. "Combined experimental and numerical evaluation of the differences between convective and conductive thermal control on the performance of a lithium ion cell," Energy, Elsevier, vol. 144(C), pages 81-97.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:energy:v:300:y:2024:i:c:s0360544224013331. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.journals.elsevier.com/energy .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.