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Advancing catalytic fast pyrolysis through integrated multiscale modeling and experimentation: Challenges, progress, and perspectives

Author

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  • Peter N. Ciesielski
  • M. Brennan Pecha
  • Vivek S. Bharadwaj
  • Calvin Mukarakate
  • G. Jeremy Leong
  • Branden Kappes
  • Michael F. Crowley
  • Seonah Kim
  • Thomas D. Foust
  • Mark R. Nimlos

Abstract

Catalytic fast pyrolysis (CFP) is a conversion process that integrates rapid thermochemical depolymerization of solid feedstocks with catalytic transformation to yield small molecules for fuel and chemical products. This process is well‐suited for the conversion of nonfossil feedstocks such as biomass and waste plastics, and thereby holds great potential for the production of renewable commodities. In spite of many technological developments in various aspects of CFP achieved over decades of research, this technology has yet to attain commercial success for the production of fuels and chemicals from renewable feedstocks. Effective CFP processes require careful coordination of chemical and physical phenomena that span very large length and time scales. A broad spectrum of scientific progress in both pyrolysis and catalytic upgrading has provided the foundation for successful deployment of CFP, although additional progress in process‐scale integration is yet required for commercial realization. Modeling and simulation tools provide an important framework wherein the CFP technologies by be better understood and evaluated from a holistic perspective. Here we provide a detailed description of the multiscale phenomena underlying CFP, describe challenges and associated technical progress, and suggest strategies for an integrated approach to advance this technology toward commercialization. This article is categorized under: Bioenergy > Systems and Infrastructure Bioenergy > Science and Materials

Suggested Citation

  • Peter N. Ciesielski & M. Brennan Pecha & Vivek S. Bharadwaj & Calvin Mukarakate & G. Jeremy Leong & Branden Kappes & Michael F. Crowley & Seonah Kim & Thomas D. Foust & Mark R. Nimlos, 2018. "Advancing catalytic fast pyrolysis through integrated multiscale modeling and experimentation: Challenges, progress, and perspectives," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 7(4), July.
  • Handle: RePEc:bla:wireae:v:7:y:2018:i:4:n:e297
    DOI: 10.1002/wene.297
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    References listed on IDEAS

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    1. Bergthorson, Jeffrey M. & Thomson, Murray J., 2015. "A review of the combustion and emissions properties of advanced transportation biofuels and their impact on existing and future engines," Renewable and Sustainable Energy Reviews, Elsevier, vol. 42(C), pages 1393-1417.
    2. I. A. Vasalos & A. A. Lappas & E. P. Kopalidou & K. G. Kalogiannis, 2016. "Biomass catalytic pyrolysis: process design and economic analysis," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 5(3), pages 370-383, May.
    3. Collard, François-Xavier & Blin, Joël, 2014. "A review on pyrolysis of biomass constituents: Mechanisms and composition of the products obtained from the conversion of cellulose, hemicelluloses and lignin," Renewable and Sustainable Energy Reviews, Elsevier, vol. 38(C), pages 594-608.
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    1. Gorugantu SriBala & Hans‐Heinrich Carstensen & Kevin M. Van Geem & Guy B. Marin, 2019. "Measuring biomass fast pyrolysis kinetics: State of the art," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 8(2), March.

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