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Innovative synthesis and comprehensive electrochemical evaluation of FeVO4 for enhanced sodium-ion battery performance

Author

Listed:
  • Yin, Xinxin
  • Wu, Donghai
  • Lu, Zhenjiang
  • Xie, Jing
  • Hu, Jindou
  • Tang, Mingxuan
  • Ma, Huan
  • Zhang, Xuntao
  • Cao, Yali

Abstract

Sodium-ion batteries (SIBs) are emerging as a viable alternative to the more costly and resource-constrained lithium-ion batteries (LIBs), especially in meeting the increasing need for large-scale energy storage. A significant challenge for SIBs lies in the exploration of the advanced anode materials. FeVO4 (FVO) nanoparticles were synthesized through both wet chemical and solid-phase methods by using citric acid monohydrate and ferric nitrate nonahydrate as blowing agents. XRD and TEM characterization reveals the presence of a large (101) interlayer spacing (∼4.46 Å) that accommodates the insertion and extraction of sodium ions (Na+). As anode material for storing Na+, FVO demonstrates an impressive discharge capacity of 326.5 mAh g−1 when cycling at a rate of 0.1 A g−1 over 300 cycles. In addition, the NaFePO4||FeVO4 full cell provides a discharge specific capacity of 102.8 mAh g−1 at 0.1C (1C = 154 mAg−1). The dynamic properties of the FVO/Na battery are revealed by pseudo-capacitance analysis and GITT tests. Meanwhile, the storage mechanism of Na+ is further analyzed by XPS, TEM, in-situ XRD and density functional theory calculations. Overall, this work presents new insights into the application of FeVO4 in SIBs and also demonstrates the competitive potential of FeVO4 for energy storage.

Suggested Citation

  • Yin, Xinxin & Wu, Donghai & Lu, Zhenjiang & Xie, Jing & Hu, Jindou & Tang, Mingxuan & Ma, Huan & Zhang, Xuntao & Cao, Yali, 2024. "Innovative synthesis and comprehensive electrochemical evaluation of FeVO4 for enhanced sodium-ion battery performance," Applied Energy, Elsevier, vol. 373(C).
    • Handle: RePEc:eee:appene:v:373:y:2024:i:c:s0306261924012558
    DOI: 10.1016/j.apenergy.2024.123872
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    References listed on IDEAS

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    1. Yang Wen & Kai He & Yujie Zhu & Fudong Han & Yunhua Xu & Isamu Matsuda & Yoshitaka Ishii & John Cumings & Chunsheng Wang, 2014. "Expanded graphite as superior anode for sodium-ion batteries," Nature Communications, Nature, vol. 5(1), pages 1-10, September.
    2. Gupta, Yamini & Siwatch, Poonam & Karwasra, Reetika & Sharma, Kriti & Tripathi, S.K., 2024. "Recent progress of layered structured P2- and O3- type transition metal oxides as cathode material for sodium-ion batteries," Renewable and Sustainable Energy Reviews, Elsevier, vol. 192(C).
    3. Lin, Yu-Hsiu & Shen, Ting-Yu, 2023. "Novel cell screening and prognosing based on neurocomputing-based multiday-ahead time-series forecasting for predictive maintenance of battery modules in frequency regulation-energy storage systems," Applied Energy, Elsevier, vol. 351(C).
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