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Lanthana-doped ceria as active support for oxygen carriers in chemical looping combustion

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  • Bhavsar, Saurabh
  • Isenberg, Natalie
  • More, Amey
  • Veser, Götz

Abstract

The redox properties and oxygen buffering capacity of reducible oxides, such as ceria, make them interesting support materials for oxygen carriers in Chemical Looping Combustion (CLC), an emerging clean combustion technology. However, the effectiveness of reducible oxides for redox applications depends crucially on oxygen mobility in the oxide lattice. In the present work, we demonstrate that addition of an aliovalent dopant (La) strongly enhances oxygen mobility in ceria, resulting in multiple performance benefits. A series of La-doped ceria (LaxCe1−xO2−x/2, 0

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  • Bhavsar, Saurabh & Isenberg, Natalie & More, Amey & Veser, Götz, 2016. "Lanthana-doped ceria as active support for oxygen carriers in chemical looping combustion," Applied Energy, Elsevier, vol. 168(C), pages 236-247.
    • Handle: RePEc:eee:appene:v:168:y:2016:i:c:p:236-247
    DOI: 10.1016/j.apenergy.2016.01.073
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    References listed on IDEAS

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    1. Do, Jeong Yeon & Son, Namgyu & Park, No-Kuk & Kwak, Byeong Sub & Baek, Jeom-In & Ryu, Ho-Jung & Kang, Misook, 2018. "Reliable oxygen transfer in MgAl2O4 spinel through the reversible formation of oxygen vacancies by Cu2+/Fe3+ anchoring," Applied Energy, Elsevier, vol. 219(C), pages 138-150.
    2. Qiu, Yu & Zhang, Shuai & Cui, Dongxu & Li, Min & Zeng, Jimin & Zeng, Dewang & Xiao, Rui, 2019. "Enhanced hydrogen production performance at intermediate temperatures through the synergistic effects of binary oxygen carriers," Applied Energy, Elsevier, vol. 252(C), pages 1-1.
    3. Jo, Seung Won & Im, Younghwan & Do, Jeong Yeon & Park, No-Kuk & Lee, Tae Jin & Lee, Sang Tae & Cha, Moon Soon & Jeon, Min-Kyu & Kang, Misook, 2017. "Synergies between Ni, Co, and Mn ions in trimetallic Ni1-xCoxMnO4 catalysts for effective hydrogen production from propane steam reforming," Renewable Energy, Elsevier, vol. 113(C), pages 248-256.

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