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Carbon dioxide removal using calcium aluminate carbonates on titanic oxide under warm-gas conditions

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  • Yu, Ching-tsung
  • Kuo, Huan-ting
  • Chen, Yi-ming

Abstract

This study presents a scale-up production method for Ti including Ca/Al sorbents and their CO2 sorption test under warm gas conditions by thermogravimetric (TG) analysis and fixed-bed reactor experiments. The Ca/Al/Tix sorbents are made by the precipitation-and-deposition method where Ca2+ and Al3+ ions are deposited via an alkaline solution of OH−/CO32− on TiO2 powder. The titanium dioxide binder facilitates CO2 capture and enhances the CO2 capacity and multicycle stability by adjusting the Ti/Ca ratio. The results showed that these sorbents exhibited excellent CO2 capture stability of 96–98% after ten cycles at 750°C by TG analysis. Characterization by XRD indicated that the reduction in the deterioration of the sorbent during the cycle test could possibly result from the formation of an anti-sintering compound such as CaTiO3 along with calcium aluminate hydroxides related to katoite. Using a reactor as test rig, the amount of sorbent and total capture weight was significantly increased. This TiO2-coated sample of Ca/Al/O–TiO2 provides a feasible route for the manufacture of cheap CO2 sorbents.

Suggested Citation

  • Yu, Ching-tsung & Kuo, Huan-ting & Chen, Yi-ming, 2016. "Carbon dioxide removal using calcium aluminate carbonates on titanic oxide under warm-gas conditions," Applied Energy, Elsevier, vol. 162(C), pages 1122-1130.
    • Handle: RePEc:eee:appene:v:162:y:2016:i:c:p:1122-1130
    DOI: 10.1016/j.apenergy.2014.12.046
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    References listed on IDEAS

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    1. Mario Sisinni & Andrea Di Carlo & Enrico Bocci & Andrea Micangeli & Vincenzo Naso, 2013. "Hydrogen-Rich Gas Production by Sorption Enhanced Steam Reforming of Woodgas Containing TAR over a Commercial Ni Catalyst and Calcined Dolomite as CO 2 Sorbent," Energies, MDPI, vol. 6(7), pages 1-15, July.
    2. Zhang, Yingying & Ji, Xiaoyan & Lu, Xiaohua, 2014. "Energy consumption analysis for CO2 separation from gas mixtures," Applied Energy, Elsevier, vol. 130(C), pages 237-243.
    3. Chen, Huichao & Zhao, Changsui & Yang, Yanmei & Zhang, Pingping, 2012. "CO2 capture and attrition performance of CaO pellets with aluminate cement under pressurized carbonation," Applied Energy, Elsevier, vol. 91(1), pages 334-340.
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    1. Han, Rui & Gao, Jihui & Wei, Siyu & Su, Yanlin & Sun, Fei & Zhao, Guangbo & Qin, Yukun, 2018. "Strongly coupled calcium carbonate/antioxidative graphite nanosheets composites with high cycling stability for thermochemical energy storage," Applied Energy, Elsevier, vol. 231(C), pages 412-422.
    2. Živković, Luka A. & Pohar, Andrej & Likozar, Blaž & Nikačević, Nikola M., 2016. "Kinetics and reactor modeling for CaO sorption-enhanced high-temperature water–gas shift (SE–WGS) reaction for hydrogen production," Applied Energy, Elsevier, vol. 178(C), pages 844-855.
    3. Antzaras, Andy N. & Lemonidou, Angeliki A., 2022. "Recent advances on materials and processes for intensified production of blue hydrogen," Renewable and Sustainable Energy Reviews, Elsevier, vol. 155(C).
    4. Shi, Jiewen & Li, Yingjie & Zhang, Qing & Ma, Xiaotong & Duan, Lunbo & Zhou, Xingang, 2017. "CO2 capture performance of a novel synthetic CaO/sepiolite sorbent at calcium looping conditions," Applied Energy, Elsevier, vol. 203(C), pages 412-421.

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    Keywords

    CaO; TiO2; CO2 capture;
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