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Leaching and indirect mineral carbonation performance of coal fly ash-water solution system

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  • Han, Sang-Jun
  • Im, Hye Jin
  • Wee, Jung-Ho

Abstract

The leaching and carbonation performances of indirect mineral carbonation are investigated using coal fly ash (FA) as the raw source and water as the solvent. The reactions were conducted at ambient temperature and pressure with a gas mixture comprised of 15 and 33mol% CO2. The overall CO2 storage and mineral carbonation capacities of FA suspended solution in which alkaline components had been previously leached for 2h (2S33) were 31.06 and 17.36mg CO2/g FA, respectively. The mineral carbonation capacity of FA in 2S33 was 18% of the theoretical value and its mineral carbonation storage capacity ratio was 55.9%. The performance of 2S33 was higher than that of its filtrate because the alkaline components were leached from the suspended FA simultaneously with the mineral carbonation. Submicrometer-sized particles were present in raw FA and their size was reduced by stirring during the leaching, as well as slightly increased, compared to the original raw FA, due to the carbonation. These submicro FA particles strongly affected the performance of the mineral carbonation of the FA-water solution.

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  • Han, Sang-Jun & Im, Hye Jin & Wee, Jung-Ho, 2015. "Leaching and indirect mineral carbonation performance of coal fly ash-water solution system," Applied Energy, Elsevier, vol. 142(C), pages 274-282.
    • Handle: RePEc:eee:appene:v:142:y:2015:i:c:p:274-282
    DOI: 10.1016/j.apenergy.2014.12.074
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    1. Wee, Jung-Ho, 2013. "A review on carbon dioxide capture and storage technology using coal fly ash," Applied Energy, Elsevier, vol. 106(C), pages 143-151.
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    5. Pan, Shu-Yuan & Lorente Lafuente, Ana Maria & Chiang, Pen-Chi, 2016. "Engineering, environmental and economic performance evaluation of high-gravity carbonation process for carbon capture and utilization," Applied Energy, Elsevier, vol. 170(C), pages 269-277.
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    7. Li, Hongwei & Zhang, Rongjun & Wang, Tianye & Wu, Yu & Xu, Run & Wang, Qiang & Tang, Zhigang, 2022. "Performance evaluation and environment risk assessment of steel slag enhancement for seawater to capture CO2," Energy, Elsevier, vol. 238(PB).
    8. Hosseini, Tahereh & Haque, Nawshad & Selomulya, Cordelia & Zhang, Lian, 2016. "Mineral carbonation of Victorian brown coal fly ash using regenerative ammonium chloride – Process simulation and techno-economic analysis," Applied Energy, Elsevier, vol. 175(C), pages 54-68.
    9. Ren, Shan & Aldahri, Tahani & Liu, Weizao & Liang, Bin, 2021. "CO2 mineral sequestration by using blast furnace slag: From batch to continuous experiments," Energy, Elsevier, vol. 214(C).
    10. Lei Wang & Yuemei Tang & Yu Gong & Xiang Shao & Xiaochen Lin & Weili Xu & Yifan Zhu & Yongming Ju & Lili Shi & Dorota Kołodyńska, 2023. "Remediation of Micro-Pollution in an Alkaline Washing Solution of Fly Ash Using Simulated Exhaust Gas: Parameters and Mechanism," Sustainability, MDPI, vol. 15(7), pages 1-15, March.

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