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Performance of Cu‐Fe‐based oxygen carrier in a CLC process based on fixed bed reactors

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  • Qiang Tian
  • Lixin Che
  • Bin Ding
  • Qianwei Wang
  • Qingquan Su

Abstract

To explore the application of chemical‐looping combustion (CLC) to the distributed medium‐ small‐scale hot water and steam gas‐fueled boilers, a CLC process based on two fixed bed reactors (FBRs) has been proposed. A Cu‐Fe‐based oxygen carrier (OC) was studied to meet the requirements for this process. Results showed that Cu30‐Fe50/Al20 was exothermic both in the reduction step and in the oxidation step, and showed a quite large operating temperature window of 600–900°C. At the lower temperature side, it showed good low temperature reactivity, and at the higher temperature side, it showed strong resistance to carbon deposition, agglomeration, and sintering. © 2017 Society of Chemical Industry and John Wiley & Sons, Ltd.

Suggested Citation

  • Qiang Tian & Lixin Che & Bin Ding & Qianwei Wang & Qingquan Su, 2017. "Performance of Cu‐Fe‐based oxygen carrier in a CLC process based on fixed bed reactors," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 7(4), pages 731-744, August.
    • Handle: RePEc:wly:greenh:v:7:y:2017:i:4:p:731-744
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    File URL: http://hdl.handle.net/10.1002/ghg.1684
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    References listed on IDEAS

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    1. Zhang, Shuai & Xiao, Rui & Zheng, Wenguang, 2014. "Comparative study between fluidized-bed and fixed-bed operation modes in pressurized chemical looping combustion of coal," Applied Energy, Elsevier, vol. 130(C), pages 181-189.
    2. Han, Lu & Bollas, George M., 2016. "Chemical-looping combustion in a reverse-flow fixed bed reactor," Energy, Elsevier, vol. 102(C), pages 669-681.
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    1. Tomasz Czakiert & Jaroslaw Krzywanski & Anna Zylka & Wojciech Nowak, 2022. "Chemical Looping Combustion: A Brief Overview," Energies, MDPI, vol. 15(4), pages 1-19, February.
    2. Qiang Tian & Lixin Che & Bin Ding & Qianwei Wang & Qingquan Su, 2018. "Performance of a Cu–Fe‐based oxygen carrier combined with a Ni‐based oxygen carrier in a chemical‐looping combustion process based on fixed‐bed reactors," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(3), pages 542-556, June.

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