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Quantum-limit Chern topological magnetism in TbMn6Sn6

Author

Listed:
  • Jia-Xin Yin

    (Princeton University)

  • Wenlong Ma

    (Peking University)

  • Tyler A. Cochran

    (Princeton University)

  • Xitong Xu

    (Peking University)

  • Songtian S. Zhang

    (Princeton University)

  • Hung-Ju Tien

    (National Cheng Kung University)

  • Nana Shumiya

    (Princeton University)

  • Guangming Cheng

    (Princeton University)

  • Kun Jiang

    (Boston College)

  • Biao Lian

    (Princeton University)

  • Zhida Song

    (Princeton University)

  • Guoqing Chang

    (Princeton University)

  • Ilya Belopolski

    (Princeton University)

  • Daniel Multer

    (Princeton University)

  • Maksim Litskevich

    (Princeton University)

  • Zi-Jia Cheng

    (Princeton University)

  • Xian P. Yang

    (Princeton University)

  • Bianca Swidler

    (Princeton University)

  • Huibin Zhou

    (Peking University)

  • Hsin Lin

    (Academia Sinica)

  • Titus Neupert

    (University of Zurich)

  • Ziqiang Wang

    (Boston College)

  • Nan Yao

    (Princeton University)

  • Tay-Rong Chang

    (National Cheng Kung University
    Center for Quantum Frontiers of Research and Technology (QFort)
    National Center for Theoretical Sciences)

  • Shuang Jia

    (Peking University
    University of Chinese Academy of Sciences
    Beijing Academy of Quantum Information Sciences)

  • M. Zahid Hasan

    (Princeton University
    Lawrence Berkeley National Laboratory)

Abstract

The quantum-level interplay between geometry, topology and correlation is at the forefront of fundamental physics1–15. Kagome magnets are predicted to support intrinsic Chern quantum phases owing to their unusual lattice geometry and breaking of time-reversal symmetry14,15. However, quantum materials hosting ideal spin–orbit-coupled kagome lattices with strong out-of-plane magnetization are lacking16–21. Here, using scanning tunnelling microscopy, we identify a new topological kagome magnet, TbMn6Sn6, that is close to satisfying these criteria. We visualize its effectively defect-free, purely manganese-based ferromagnetic kagome lattice with atomic resolution. Remarkably, its electronic state shows distinct Landau quantization on application of a magnetic field, and the quantized Landau fan structure features spin-polarized Dirac dispersion with a large Chern gap. We further demonstrate the bulk–boundary correspondence between the Chern gap and the topological edge state, as well as the Berry curvature field correspondence of Chern gapped Dirac fermions. Our results point to the realization of a quantum-limit Chern phase in TbMn6Sn6, and may enable the observation of topological quantum phenomena in the RMn6Sn6 (where R is a rare earth element) family with a variety of magnetic structures. Our visualization of the magnetic bulk–boundary–Berry correspondence covering real space and momentum space demonstrates a proof-of-principle method for revealing topological magnets.

Suggested Citation

  • Jia-Xin Yin & Wenlong Ma & Tyler A. Cochran & Xitong Xu & Songtian S. Zhang & Hung-Ju Tien & Nana Shumiya & Guangming Cheng & Kun Jiang & Biao Lian & Zhida Song & Guoqing Chang & Ilya Belopolski & Dan, 2020. "Quantum-limit Chern topological magnetism in TbMn6Sn6," Nature, Nature, vol. 583(7817), pages 533-536, July.
  • Handle: RePEc:nat:nature:v:583:y:2020:i:7817:d:10.1038_s41586-020-2482-7
    DOI: 10.1038/s41586-020-2482-7
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    Cited by:

    1. Xitong Xu & Jia-Xin Yin & Wenlong Ma & Hung-Ju Tien & Xiao-Bin Qiang & P. V. Sreenivasa Reddy & Huibin Zhou & Jie Shen & Hai-Zhou Lu & Tay-Rong Chang & Zhe Qu & Shuang Jia, 2022. "Topological charge-entropy scaling in kagome Chern magnet TbMn6Sn6," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    2. He Wang & Yanzhao Liu & Ming Gong & Hua Jiang & Xiaoyue Gao & Wenlong Ma & Jiawei Luo & Haoran Ji & Jun Ge & Shuang Jia & Peng Gao & Ziqiang Wang & X. C. Xie & Jian Wang, 2023. "Emergent superconductivity in topological-kagome-magnet/metal heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    3. Heda Zhang & Jahyun Koo & Chunqiang Xu & Milos Sretenovic & Binghai Yan & Xianglin Ke, 2022. "Exchange-biased topological transverse thermoelectric effects in a Kagome ferrimagnet," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    4. Huimin Zhang & Basu Dev Oli & Qiang Zou & Xu Guo & Zhengfei Wang & Lian Li, 2023. "Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    5. H. Miao & T. T. Zhang & H. X. Li & G. Fabbris & A. H. Said & R. Tartaglia & T. Yilmaz & E. Vescovo & J.-X. Yin & S. Murakami & X. L. Feng & K. Jiang & X. L. Wu & A. F. Wang & S. Okamoto & Y. L. Wang &, 2023. "Signature of spin-phonon coupling driven charge density wave in a kagome magnet," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    6. S. X. M. Riberolles & Tyler J. Slade & Tianxiong Han & Bing Li & D. L. Abernathy & P. C. Canfield & B. G. Ueland & P. P. Orth & Liqin Ke & R. J. McQueeney, 2024. "Chiral and flat-band magnetic quasiparticles in ferromagnetic and metallic kagome layers," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    7. Boqin Song & Tianping Ying & Xianxin Wu & Wei Xia & Qiangwei Yin & Qinghua Zhang & Yanpeng Song & Xiaofan Yang & Jiangang Guo & Lin Gu & Xiaolong Chen & Jiangping Hu & Andreas P. Schnyder & Hechang Le, 2023. "Anomalous enhancement of charge density wave in kagome superconductor CsV3Sb5 approaching the 2D limit," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    8. Zheng Ren & Jianwei Huang & Hengxin Tan & Ananya Biswas & Aki Pulkkinen & Yichen Zhang & Yaofeng Xie & Ziqin Yue & Lei Chen & Fang Xie & Kevin Allen & Han Wu & Qirui Ren & Anil Rajapitamahuni & Asish , 2024. "Persistent flat band splitting and strong selective band renormalization in a kagome magnet thin film," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    9. Rui Lou & Liqin Zhou & Wenhua Song & Alexander Fedorov & Zhijun Tu & Bei Jiang & Qi Wang & Man Li & Zhonghao Liu & Xuezhi Chen & Oliver Rader & Bernd Büchner & Yujie Sun & Hongming Weng & Hechang Lei , 2024. "Orbital-selective effect of spin reorientation on the Dirac fermions in a non-charge-ordered kagome ferromagnet Fe3Ge," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    10. Ziyuan Chen & Xueliang Wu & Shiming Zhou & Jiakang Zhang & Ruotong Yin & Yuanji Li & Mingzhe Li & Jiashuo Gong & Mingquan He & Yisheng Chai & Xiaoyuan Zhou & Yilin Wang & Aifeng Wang & Ya-Jun Yan & Do, 2024. "Discovery of a long-ranged charge order with 1/4 Ge1-dimerization in an antiferromagnetic Kagome metal," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    11. Li Huang & Xianghua Kong & Qi Zheng & Yuqing Xing & Hui Chen & Yan Li & Zhixin Hu & Shiyu Zhu & Jingsi Qiao & Yu-Yang Zhang & Haixia Cheng & Zhihai Cheng & Xianggang Qiu & Enke Liu & Hechang Lei & Xia, 2023. "Discovery and construction of surface kagome electronic states induced by p-d electronic hybridization in Co3Sn2S2," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    12. S. X. M. Riberolles & Tyler J. Slade & R. L. Dally & P. M. Sarte & Bing Li & Tianxiong Han & H. Lane & C. Stock & H. Bhandari & N. J. Ghimire & D. L. Abernathy & P. C. Canfield & J. W. Lynn & B. G. Ue, 2023. "Orbital character of the spin-reorientation transition in TbMn6Sn6," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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