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Chiral and flat-band magnetic quasiparticles in ferromagnetic and metallic kagome layers

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Listed:
  • S. X. M. Riberolles

    (Ames National Laboratory)

  • Tyler J. Slade

    (Ames National Laboratory)

  • Tianxiong Han

    (Ames National Laboratory
    Iowa State University)

  • Bing Li

    (Ames National Laboratory
    Iowa State University)

  • D. L. Abernathy

    (Oak Ridge National Laboratory)

  • P. C. Canfield

    (Ames National Laboratory
    Iowa State University)

  • B. G. Ueland

    (Ames National Laboratory)

  • P. P. Orth

    (Ames National Laboratory
    Iowa State University)

  • Liqin Ke

    (Ames National Laboratory)

  • R. J. McQueeney

    (Ames National Laboratory
    Iowa State University)

Abstract

Magnetic kagome metals are a promising platform to develop unique quantum transport and optical phenomena caused by the interplay between topological electronic bands, strong correlations, and magnetic order. This interplay may result in exotic quasiparticles that describe the coupled electronic and spin excitations on the frustrated kagome lattice. Here, we observe novel elementary magnetic excitations within the ferromagnetic Mn kagome layers in TbMn6Sn6 using inelastic neutron scattering. We observe sharp, collective acoustic magnons and identify flat-band magnons that are localized to a hexagonal plaquette due to the special geometry of the kagome layer. Surprisingly, we observe another type of elementary magnetic excitation; a chiral magnetic quasiparticle that is also localized on a hexagonal plaquette. The short lifetime of localized flat-band and chiral quasiparticles suggest that they are hybrid excitations that decay into electronic states.

Suggested Citation

  • S. X. M. Riberolles & Tyler J. Slade & Tianxiong Han & Bing Li & D. L. Abernathy & P. C. Canfield & B. G. Ueland & P. P. Orth & Liqin Ke & R. J. McQueeney, 2024. "Chiral and flat-band magnetic quasiparticles in ferromagnetic and metallic kagome layers," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-45841-8
    DOI: 10.1038/s41467-024-45841-8
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    1. Xiang Chen & Igor Krivenko & Matthew B. Stone & Alexander I. Kolesnikov & Thomas Wolf & Dmitry Reznik & Kevin S. Bedell & Frank Lechermann & Stephen D. Wilson, 2020. "Unconventional Hund metal in a weak itinerant ferromagnet," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
    2. Ella Lachman & Ryan A. Murphy & Nikola Maksimovic & Robert Kealhofer & Shannon Haley & Ross D. McDonald & Jeffrey R. Long & James G. Analytis, 2020. "Exchange biased anomalous Hall effect driven by frustration in a magnetic kagome lattice," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
    3. C. Mielke & D. Das & J.-X. Yin & H. Liu & R. Gupta & Y.-X. Jiang & M. Medarde & X. Wu & H. C. Lei & J. Chang & Pengcheng Dai & Q. Si & H. Miao & R. Thomale & T. Neupert & Y. Shi & R. Khasanov & M. Z. , 2022. "Time-reversal symmetry-breaking charge order in a kagome superconductor," Nature, Nature, vol. 602(7896), pages 245-250, February.
    4. Jia-Xin Yin & Biao Lian & M. Zahid Hasan, 2022. "Topological kagome magnets and superconductors," Nature, Nature, vol. 612(7941), pages 647-657, December.
    5. Minyong Han & Hisashi Inoue & Shiang Fang & Caolan John & Linda Ye & Mun K. Chan & David Graf & Takehito Suzuki & Madhav Prasad Ghimire & Won Joon Cho & Efthimios Kaxiras & Joseph G. Checkelsky, 2021. "Evidence of two-dimensional flat band at the surface of antiferromagnetic kagome metal FeSn," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    6. Z. Guguchia & J. A. T. Verezhak & D. J. Gawryluk & S. S. Tsirkin & J.-X. Yin & I. Belopolski & H. Zhou & G. Simutis & S.-S. Zhang & T. A. Cochran & G. Chang & E. Pomjakushina & L. Keller & Z. Skrzeczk, 2020. "Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet," Nature Communications, Nature, vol. 11(1), pages 1-9, December.
    7. R. Okuma & D. Nakamura & T. Okubo & A. Miyake & A. Matsuo & K. Kindo & M. Tokunaga & N. Kawashima & S. Takeyama & Z. Hiroi, 2019. "A series of magnon crystals appearing under ultrahigh magnetic fields in a kagomé antiferromagnet," Nature Communications, Nature, vol. 10(1), pages 1-7, December.
    8. Linda Ye & Mingu Kang & Junwei Liu & Felix von Cube & Christina R. Wicker & Takehito Suzuki & Chris Jozwiak & Aaron Bostwick & Eli Rotenberg & David C. Bell & Liang Fu & Riccardo Comin & Joseph G. Che, 2018. "Massive Dirac fermions in a ferromagnetic kagome metal," Nature, Nature, vol. 555(7698), pages 638-642, March.
    9. Linda Ye & Mun K. Chan & Ross D. McDonald & David Graf & Mingu Kang & Junwei Liu & Takehito Suzuki & Riccardo Comin & Liang Fu & Joseph G. Checkelsky, 2019. "de Haas-van Alphen effect of correlated Dirac states in kagome metal Fe3Sn2," Nature Communications, Nature, vol. 10(1), pages 1-8, December.
    10. Jia-Xin Yin & Wenlong Ma & Tyler A. Cochran & Xitong Xu & Songtian S. Zhang & Hung-Ju Tien & Nana Shumiya & Guangming Cheng & Kun Jiang & Biao Lian & Zhida Song & Guoqing Chang & Ilya Belopolski & Dan, 2020. "Quantum-limit Chern topological magnetism in TbMn6Sn6," Nature, Nature, vol. 583(7817), pages 533-536, July.
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