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Ion sieving in graphene oxide membranes via cationic control of interlayer spacing

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  • Liang Chen

    (Shanghai Applied Radiation Institute, Shanghai University
    Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences
    Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F University)

  • Guosheng Shi

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Jie Shen

    (State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University)

  • Bingquan Peng

    (Shanghai Applied Radiation Institute, Shanghai University)

  • Bowu Zhang

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Yuzhu Wang

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Fenggang Bian

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Jiajun Wang

    (Shanghai Applied Radiation Institute, Shanghai University)

  • Deyuan Li

    (Shanghai Applied Radiation Institute, Shanghai University
    Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Zhe Qian

    (Shanghai Applied Radiation Institute, Shanghai University)

  • Gang Xu

    (Shanghai Applied Radiation Institute, Shanghai University)

  • Gongping Liu

    (State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University)

  • Jianrong Zeng

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Lijuan Zhang

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Yizhou Yang

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Guoquan Zhou

    (Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F University)

  • Minghong Wu

    (Shanghai Applied Radiation Institute, Shanghai University)

  • Wanqin Jin

    (State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University)

  • Jingye Li

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

  • Haiping Fang

    (Key Laboratory of Interfacial Physics and Technology and Shanghai Synchrotron Radiation Facility, Shanghai Institute of Applied Physics, Chinese Academy of Sciences)

Abstract

Cations are used to control the interlayer spacing of graphene oxide membranes, enabling efficient and selective sieving of hydrated cations.

Suggested Citation

  • Liang Chen & Guosheng Shi & Jie Shen & Bingquan Peng & Bowu Zhang & Yuzhu Wang & Fenggang Bian & Jiajun Wang & Deyuan Li & Zhe Qian & Gang Xu & Gongping Liu & Jianrong Zeng & Lijuan Zhang & Yizhou Yan, 2017. "Ion sieving in graphene oxide membranes via cationic control of interlayer spacing," Nature, Nature, vol. 550(7676), pages 380-383, October.
    • Handle: RePEc:nat:nature:v:550:y:2017:i:7676:d:10.1038_nature24044
    DOI: 10.1038/nature24044
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    Cited by:

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    2. Weiwen Xin & Jingru Fu & Yongchao Qian & Lin Fu & Xiang-Yu Kong & Teng Ben & Lei Jiang & Liping Wen, 2022. "Biomimetic KcsA channels with ultra-selective K+ transport for monovalent ion sieving," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    3. Rezakazemi, Mashallah & Arabi Shamsabadi, Ahmad & Lin, Haiqing & Luis, Patricia & Ramakrishna, Seeram & Aminabhavi, Tejraj M., 2021. "Sustainable MXenes-based membranes for highly energy-efficient separations," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    4. Changwei Zhao & Yanjun Zhang & Yuewen Jia & Bojun Li & Wenjing Tang & Chuning Shang & Rui Mo & Pei Li & Shaomin Liu & Sui Zhang, 2023. "Polyamide membranes with nanoscale ordered structures for fast permeation and highly selective ion-ion separation," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    5. Zhipeng Wang & Liqin Huang & Xue Dong & Tong Wu & Qi Qing & Jing Chen & Yuexiang Lu & Chao Xu, 2023. "Ion sieving in graphene oxide membrane enables efficient actinides/lanthanides separation," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    6. Ri-Jian Mo & Shuang Chen & Li-Qiu Huang & Xin-Lei Ding & Saima Rafique & Xing-Hua Xia & Zhong-Qiu Li, 2024. "Regulating ion affinity and dehydration of metal-organic framework sub-nanochannels for high-precision ion separation," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    7. Zhen Zhang & Preeti Bhauriyal & Hafeesudeen Sahabudeen & Zhiyong Wang & Xiaohui Liu & Mike Hambsch & Stefan C. B. Mannsfeld & Renhao Dong & Thomas Heine & Xinliang Feng, 2022. "Cation-selective two-dimensional polyimine membranes for high-performance osmotic energy conversion," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    8. Shuangqiao Han & Junyong Zhu & Adam A. Uliana & Dongyang Li & Yatao Zhang & Lin Zhang & Yong Wang & Tao He & Menachem Elimelech, 2022. "Microporous organic nanotube assisted design of high performance nanofiltration membranes," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    9. Zongyao Zhou & Kangning Zhao & Heng-Yu Chi & Yueqing Shen & Shuqing Song & Kuang-Jung Hsu & Mojtaba Chevalier & Wenxiong Shi & Kumar Varoon Agrawal, 2024. "Electrochemical-repaired porous graphene membranes for precise ion-ion separation," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    10. Shuqi Xu & Alice J. Hutchinson & Mahdiar Taheri & Ben Corry & Juan F. Torres, 2024. "Thermodiffusive desalination," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    11. Rongming Xu & Yuan Kang & Weiming Zhang & Bingcai Pan & Xiwang Zhang, 2023. "Two-dimensional MXene membranes with biomimetic sub-nanochannels for enhanced cation sieving," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    12. Hongjian Wang & Yeming Zhai & Yang Li & Yu Cao & Benbing Shi & Runlai Li & Zingting Zhu & Haifei Jiang & Zheyuan Guo & Meidi Wang & Long Chen & Yawei Liu & Kai-Ge Zhou & Fusheng Pan & Zhongyi Jiang, 2022. "Covalent organic framework membranes for efficient separation of monovalent cations," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    13. Yang Wang & Tingting Lian & Nadezda V. Tarakina & Jiayin Yuan & Markus Antonietti, 2022. "Lamellar carbon nitride membrane for enhanced ion sieving and water desalination," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    14. Xinming Xia & Feng Zhou & Jing Xu & Zhongteng Wang & Jian Lan & Yan Fan & Zhikun Wang & Wei Liu & Junlang Chen & Shangshen Feng & Yusong Tu & Yizhou Yang & Liang Chen & Haiping Fang, 2022. "Unexpectedly efficient ion desorption of graphene-based materials," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    15. Quan Peng & Ruoyu Wang & Zilin Zhao & Shihong Lin & Ying Liu & Dianyu Dong & Zheng Wang & Yiman He & Yuzhang Zhu & Jian Jin & Lei Jiang, 2024. "Extreme Li-Mg selectivity via precise ion size differentiation of polyamide membrane," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    16. Yuanxi Yu & Chenxing Yang & Matteo Baggioli & Anthony E. Phillips & Alessio Zaccone & Lei Zhang & Ryoichi Kajimoto & Mitsutaka Nakamura & Dehong Yu & Liang Hong, 2022. "The ω3 scaling of the vibrational density of states in quasi-2D nanoconfined solids," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    17. Haiguang Zhang & Jiajian Xing & Gaoliang Wei & Xu Wang & Shuo Chen & Xie Quan, 2024. "Electrostatic-induced ion-confined partitioning in graphene nanolaminate membrane for breaking anion–cation co-transport to enhance desalination," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    18. Yuan Kang & Ting Hu & Yuqi Wang & Kaiqiang He & Zhuyuan Wang & Yvonne Hora & Wang Zhao & Rongming Xu & Yu Chen & Zongli Xie & Huanting Wang & Qinfen Gu & Xiwang Zhang, 2023. "Nanoconfinement enabled non-covalently decorated MXene membranes for ion-sieving," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    19. Nawapong Unsuree & Sorasak Phanphak & Pongthep Prajongtat & Aritsa Bunpheng & Kulpavee Jitapunkul & Pornpis Kongputhon & Pannaree Srinoi & Pawin Iamprasertkun & Wisit Hirunpinyopas, 2021. "A Review: Ion Transport of Two-Dimensional Materials in Novel Technologies from Macro to Nanoscopic Perspectives," Energies, MDPI, vol. 14(18), pages 1-38, September.
    20. Qian Zhang & Bo Gao & Ling Zhang & Xiaopeng Liu & Jixiang Cui & Yijun Cao & Hongbo Zeng & Qun Xu & Xinwei Cui & Lei Jiang, 2023. "Anomalous water molecular gating from atomic-scale graphene capillaries for precise and ultrafast molecular sieving," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    21. Xinyue Wen & Tobias Foller & Xiaoheng Jin & Tiziana Musso & Priyank Kumar & Rakesh Joshi, 2022. "Understanding water transport through graphene-based nanochannels via experimental control of slip length," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    22. Si-Hua Liu & Jun-Hao Zhou & Chunrui Wu & Peng Zhang & Xingzhong Cao & Jian-Ke Sun, 2024. "Sub-8 nm networked cage nanofilm with tunable nanofluidic channels for adaptive sieving," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    23. Hai Liu & Xinxi Huang & Yang Wang & Baian Kuang & Wanbin Li, 2024. "Nanowire-assisted electrochemical perforation of graphene oxide nanosheets for molecular separation," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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