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Cobalt carbide nanoprisms for direct production of lower olefins from syngas

Author

Listed:
  • Liangshu Zhong

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

  • Fei Yu

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences
    School of Environmental and Chemical Engineering, Shanghai University)

  • Yunlei An

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences
    School of Environmental and Chemical Engineering, Shanghai University)

  • Yonghui Zhao

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

  • Yuhan Sun

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences
    School of Physical Science and Technology, ShanghaiTech University)

  • Zhengjia Li

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences
    School of Chemistry and Molecular Engineering, East China Normal University)

  • Tiejun Lin

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

  • Yanjun Lin

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

  • Xingzhen Qi

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

  • Yuanyuan Dai

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences
    University of the Chinese Academy of Sciences)

  • Lin Gu

    (Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences)

  • Jinsong Hu

    (University of the Chinese Academy of Sciences
    Beijing National Laboratory for Molecular Sciences, Key Laboratory of Molecular Nanostructure and Nanotechnology, Institute of Chemistry, Chinese Academy of Sciences)

  • Shifeng Jin

    (Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences)

  • Qun Shen

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

  • Hui Wang

    (CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute, Chinese Academy of Sciences)

Abstract

Lower olefins are hydrocarbons that are widely used in the chemical industry, and can be generated from syngas by the ‘Fischer–Tropsch to olefins’ process; here, a new catalyst is described that can generate lower olefins from syngas with high selectivity, with little formation of undesirable methane.

Suggested Citation

  • Liangshu Zhong & Fei Yu & Yunlei An & Yonghui Zhao & Yuhan Sun & Zhengjia Li & Tiejun Lin & Yanjun Lin & Xingzhen Qi & Yuanyuan Dai & Lin Gu & Jinsong Hu & Shifeng Jin & Qun Shen & Hui Wang, 2016. "Cobalt carbide nanoprisms for direct production of lower olefins from syngas," Nature, Nature, vol. 538(7623), pages 84-87, October.
    • Handle: RePEc:nat:nature:v:538:y:2016:i:7623:d:10.1038_nature19786
    DOI: 10.1038/nature19786
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    Cited by:

    1. Fei Qian & Jiawei Bai & Yi Cai & Hui Yang & Xue-Min Cao & Xingchen Liu & Xing-Wu Liu & Yong Yang & Yong-Wang Li & Ding Ma & Xiao-Dong Wen, 2024. "Stabilized ε-Fe2C catalyst with Mn tuning to suppress C1 byproduct selectivity for high-temperature olefin synthesis," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    2. Xiaofeng Gao & Ling Zhu & Feng Yang & Lei Zhang & Wenhao Xu & Xian Zhou & Yongkang Huang & Houhong Song & Lili Lin & Xiaodong Wen & Ding Ma & Siyu Yao, 2023. "Subsurface nickel boosts the low-temperature performance of a boron oxide overlayer in propane oxidative dehydrogenation," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    3. Hailing Yu & Caiqi Wang & Xin Xin & Yao Wei & Shenggang Li & Yunlei An & Fanfei Sun & Tiejun Lin & Liangshu Zhong, 2024. "Engineering ZrO2–Ru interface to boost Fischer-Tropsch synthesis to olefins," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Wenlong Wu & Jiahua Luo & Jiankang Zhao & Menglin Wang & Lei Luo & Sunpei Hu & Bingxuan He & Chao Ma & Hongliang Li & Jie Zeng, 2024. "Facet sensitivity of iron carbides in Fischer-Tropsch synthesis," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    5. Yanfei Xu & Zhenxuan Zhang & Ke Wu & Jungang Wang & Bo Hou & Ruoting Shan & Ling Li & Mingyue Ding, 2024. "Effects of surface hydrophobization on the phase evolution behavior of iron-based catalyst during Fischer–Tropsch synthesis," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    6. Wang, Danfeng & Gu, Yu & Chen, Qianqian & Tang, Zhiyong, 2023. "Direct conversion of syngas to alpha olefins via Fischer–Tropsch synthesis: Process development and comparative techno-economic-environmental analysis," Energy, Elsevier, vol. 263(PE).
    7. Chuanhao Wang & Junjie Du & Lin Zeng & Zhongling Li & Yizhou Dai & Xu Li & Zijun Peng & Wenlong Wu & Hongliang Li & Jie Zeng, 2023. "Direct synthesis of extra-heavy olefins from carbon monoxide and water," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    8. Zhao, Zhitong & Chong, Katie & Jiang, Jingyang & Wilson, Karen & Zhang, Xiaochen & Wang, Feng, 2018. "Low-carbon roadmap of chemical production: A case study of ethylene in China," Renewable and Sustainable Energy Reviews, Elsevier, vol. 97(C), pages 580-591.
    9. Na Li & Yifeng Zhu & Feng Jiao & Xiulian Pan & Qike Jiang & Jun Cai & Yifan Li & Wei Tong & Changqi Xu & Shengcheng Qu & Bing Bai & Dengyun Miao & Zhi Liu & Xinhe Bao, 2022. "Steering the reaction pathway of syngas-to-light olefins with coordination unsaturated sites of ZnGaOx spinel," Nature Communications, Nature, vol. 13(1), pages 1-8, December.

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