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Widespread 2013-2020 decreases and reduction challenges of organic aerosol in China

Author

Listed:
  • Qi Chen

    (Peking University
    Peking University)

  • Ruqian Miao

    (Peking University)

  • Guannan Geng

    (Tsinghua University)

  • Manish Shrivastava

    (Pacific Northwest National Laboratory)

  • Xu Dao

    (China National Environmental Monitoring Centre)

  • Bingye Xu

    (Zhejiang Province Environment Monitoring Centre)

  • Jiaqi Sun

    (China National Environmental Monitoring Centre)

  • Xian Zhang

    (China National Environmental Monitoring Centre)

  • Mingyuan Liu

    (China National Environmental Monitoring Centre)

  • Guigang Tang

    (China National Environmental Monitoring Centre)

  • Qian Tang

    (Zhejiang Province Environment Monitoring Centre)

  • Hanwen Hu

    (Tsinghua University)

  • Ru-Jin Huang

    (Chinese Academy of Sciences)

  • Hao Wang

    (Peking University)

  • Yan Zheng

    (Peking University)

  • Yue Qin

    (Peking University
    Peking University)

  • Song Guo

    (Peking University
    Peking University)

  • Min Hu

    (Peking University
    Peking University)

  • Tong Zhu

    (Peking University
    Peking University)

Abstract

High concentrations of organic aerosol (OA) occur in Asian countries, leading to great health burdens. Clean air actions have resulted in significant emission reductions of air pollutants in China. However, long-term nation-wide trends in OA and their causes remain unknown. Here, we present both observational and model evidence demonstrating widespread decreases with a greater reduction in primary OA than in secondary OA (SOA) in China during the period of 2013 to 2020. Most of the decline is attributed to reduced residential fuel burning while the interannual variability in SOA may have been driven by meteorological variations. We find contrasting effects of reducing NOx and SO2 on SOA production which may have led to slight overall increases in SOA. Our findings highlight the importance of clean energy replacements in multiple sectors on achieving air-quality targets because of high OA precursor emissions and fluctuating chemical and meteorological conditions.

Suggested Citation

  • Qi Chen & Ruqian Miao & Guannan Geng & Manish Shrivastava & Xu Dao & Bingye Xu & Jiaqi Sun & Xian Zhang & Mingyuan Liu & Guigang Tang & Qian Tang & Hanwen Hu & Ru-Jin Huang & Hao Wang & Yan Zheng & Yu, 2024. "Widespread 2013-2020 decreases and reduction challenges of organic aerosol in China," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-48902-0
    DOI: 10.1038/s41467-024-48902-0
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    References listed on IDEAS

    as
    1. Ru-Jin Huang & Yanlin Zhang & Carlo Bozzetti & Kin-Fai Ho & Jun-Ji Cao & Yongming Han & Kaspar R. Daellenbach & Jay G. Slowik & Stephen M. Platt & Francesco Canonaco & Peter Zotter & Robert Wolf & Sim, 2014. "High secondary aerosol contribution to particulate pollution during haze events in China," Nature, Nature, vol. 514(7521), pages 218-222, October.
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