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Encoding multistate charge order and chirality in endotaxial heterostructures

Author

Listed:
  • Samra Husremović

    (University of California)

  • Berit H. Goodge

    (University of California
    Max-Planck-Institute for Chemical Physics of Solids)

  • Matthew P. Erodici

    (University of California)

  • Katherine Inzani

    (University of Nottingham, University Park)

  • Alberto Mier

    (University of California)

  • Stephanie M. Ribet

    (Lawrence Berkeley National Laboratory
    Northwestern University
    Northwestern University)

  • Karen C. Bustillo

    (Lawrence Berkeley National Laboratory)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Colin Ophus

    (Lawrence Berkeley National Laboratory)

  • Sinéad M. Griffin

    (Lawrence Berkeley National Laboratory
    Lawrence Berkeley National Laboratory)

  • D. Kwabena Bediako

    (University of California
    Lawrence Berkeley National Laboratory)

Abstract

High-density phase change memory (PCM) storage is proposed for materials with multiple intermediate resistance states, which have been observed in 1T-TaS2 due to charge density wave (CDW) phase transitions. However, the metastability responsible for this behavior makes the presence of multistate switching unpredictable in TaS2 devices. Here, we demonstrate the fabrication of nanothick verti-lateral H-TaS2/1T-TaS2 heterostructures in which the number of endotaxial metallic H-TaS2 monolayers dictates the number of resistance transitions in 1T-TaS2 lamellae near room temperature. Further, we also observe optically active heterochirality in the CDW superlattice structure, which is modulated in concert with the resistivity steps, and we show how strain engineering can be used to nucleate these polytype conversions. This work positions the principle of endotaxial heterostructures as a promising conceptual framework for reliable, non-volatile, and multi-level switching of structure, chirality, and resistance.

Suggested Citation

  • Samra Husremović & Berit H. Goodge & Matthew P. Erodici & Katherine Inzani & Alberto Mier & Stephanie M. Ribet & Karen C. Bustillo & Takashi Taniguchi & Kenji Watanabe & Colin Ophus & Sinéad M. Griffi, 2023. "Encoding multistate charge order and chirality in endotaxial heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41780-y
    DOI: 10.1038/s41467-023-41780-y
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    References listed on IDEAS

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    1. Quirin Stahl & Maximilian Kusch & Florian Heinsch & Gaston Garbarino & Norman Kretzschmar & Kerstin Hanff & Kai Rossnagel & Jochen Geck & Tobias Ritschel, 2020. "Collapse of layer dimerization in the photo-induced hidden state of 1T-TaS2," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
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    Cited by:

    1. Suk Hyun Sung & Nishkarsh Agarwal & Ismail El Baggari & Patrick Kezer & Yin Min Goh & Noah Schnitzer & Jeremy M. Shen & Tony Chiang & Yu Liu & Wenjian Lu & Yuping Sun & Lena F. Kourkoutis & John T. He, 2024. "Endotaxial stabilization of 2D charge density waves with long-range order," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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