IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-41780-y.html
   My bibliography  Save this article

Encoding multistate charge order and chirality in endotaxial heterostructures

Author

Listed:
  • Samra Husremović

    (University of California)

  • Berit H. Goodge

    (University of California
    Max-Planck-Institute for Chemical Physics of Solids)

  • Matthew P. Erodici

    (University of California)

  • Katherine Inzani

    (University of Nottingham, University Park)

  • Alberto Mier

    (University of California)

  • Stephanie M. Ribet

    (Lawrence Berkeley National Laboratory
    Northwestern University
    Northwestern University)

  • Karen C. Bustillo

    (Lawrence Berkeley National Laboratory)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Colin Ophus

    (Lawrence Berkeley National Laboratory)

  • Sinéad M. Griffin

    (Lawrence Berkeley National Laboratory
    Lawrence Berkeley National Laboratory)

  • D. Kwabena Bediako

    (University of California
    Lawrence Berkeley National Laboratory)

Abstract

High-density phase change memory (PCM) storage is proposed for materials with multiple intermediate resistance states, which have been observed in 1T-TaS2 due to charge density wave (CDW) phase transitions. However, the metastability responsible for this behavior makes the presence of multistate switching unpredictable in TaS2 devices. Here, we demonstrate the fabrication of nanothick verti-lateral H-TaS2/1T-TaS2 heterostructures in which the number of endotaxial metallic H-TaS2 monolayers dictates the number of resistance transitions in 1T-TaS2 lamellae near room temperature. Further, we also observe optically active heterochirality in the CDW superlattice structure, which is modulated in concert with the resistivity steps, and we show how strain engineering can be used to nucleate these polytype conversions. This work positions the principle of endotaxial heterostructures as a promising conceptual framework for reliable, non-volatile, and multi-level switching of structure, chirality, and resistance.

Suggested Citation

  • Samra Husremović & Berit H. Goodge & Matthew P. Erodici & Katherine Inzani & Alberto Mier & Stephanie M. Ribet & Karen C. Bustillo & Takashi Taniguchi & Kenji Watanabe & Colin Ophus & Sinéad M. Griffi, 2023. "Encoding multistate charge order and chirality in endotaxial heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41780-y
    DOI: 10.1038/s41467-023-41780-y
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-41780-y
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-023-41780-y?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Quirin Stahl & Maximilian Kusch & Florian Heinsch & Gaston Garbarino & Norman Kretzschmar & Kerstin Hanff & Kai Rossnagel & Jochen Geck & Tobias Ritschel, 2020. "Collapse of layer dimerization in the photo-induced hidden state of 1T-TaS2," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
    2. Suk Hyun Sung & Noah Schnitzer & Steve Novakov & Ismail El Baggari & Xiangpeng Luo & Jiseok Gim & Nguyen M. Vu & Zidong Li & Todd H. Brintlinger & Yu Liu & Wenjian Lu & Yuping Sun & Parag B. Deotare &, 2022. "Two-dimensional charge order stabilized in clean polytype heterostructures," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    3. Yan Zhao & Zhengwei Nie & Hao Hong & Xia Qiu & Shiyi Han & Yue Yu & Mengxi Liu & Xiaohui Qiu & Kaihui Liu & Sheng Meng & Lianming Tong & Jin Zhang, 2023. "Spectroscopic visualization and phase manipulation of chiral charge density waves in 1T-TaS2," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    4. I. Vaskivskyi & I. A. Mihailovic & S. Brazovskii & J. Gospodaric & T. Mertelj & D. Svetin & P. Sutar & D. Mihailovic, 2016. "Fast electronic resistance switching involving hidden charge density wave states," Nature Communications, Nature, vol. 7(1), pages 1-6, September.
    5. Xuan Song & Liwei Liu & Yaoyao Chen & Han Yang & Zeping Huang & Baofei Hou & Yanhui Hou & Xu Han & Huixia Yang & Quanzhen Zhang & Teng Zhang & Jiadong Zhou & Yuan Huang & Yu Zhang & Hong-Jun Gao & Yel, 2022. "Atomic-scale visualization of chiral charge density wave superlattices and their reversible switching," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Suk Hyun Sung & Nishkarsh Agarwal & Ismail El Baggari & Patrick Kezer & Yin Min Goh & Noah Schnitzer & Jeremy M. Shen & Tony Chiang & Yu Liu & Wenjian Lu & Yuping Sun & Lena F. Kourkoutis & John T. He, 2024. "Endotaxial stabilization of 2D charge density waves with long-range order," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Suk Hyun Sung & Nishkarsh Agarwal & Ismail El Baggari & Patrick Kezer & Yin Min Goh & Noah Schnitzer & Jeremy M. Shen & Tony Chiang & Yu Liu & Wenjian Lu & Yuping Sun & Lena F. Kourkoutis & John T. He, 2024. "Endotaxial stabilization of 2D charge density waves with long-range order," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Yan Zhao & Zhengwei Nie & Hao Hong & Xia Qiu & Shiyi Han & Yue Yu & Mengxi Liu & Xiaohui Qiu & Kaihui Liu & Sheng Meng & Lianming Tong & Jin Zhang, 2023. "Spectroscopic visualization and phase manipulation of chiral charge density waves in 1T-TaS2," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    3. Anze Mraz & Michele Diego & Andrej Kranjec & Jaka Vodeb & Peter Karpov & Yaroslav Gerasimenko & Jan Ravnik & Yevhenii Vaskivskyi & Rok Venturini & Viktor Kabanov & Benjamin Lipovšek & Marko Topič & Ig, 2023. "Manipulation of fractionalized charge in the metastable topologically entangled state of a doped Wigner crystal," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    4. Dohyun Kim & Eui-Cheol Shin & Yongjoon Lee & Young Hee Lee & Mali Zhao & Yong-Hyun Kim & Heejun Yang, 2022. "Atomic-scale thermopower in charge density wave states," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    5. Seyeong Cha & Giyeok Lee & Sol Lee & Sae Hee Ryu & Yeongsup Sohn & Gijeong An & Changmo Kang & Minsu Kim & Kwanpyo Kim & Aloysius Soon & Keun Su Kim, 2023. "Order-disorder phase transition driven by interlayer sliding in lead iodides," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    6. Yihao Wang & Zhihao Li & Xuan Luo & Jingjing Gao & Yuyan Han & Jialiang Jiang & Jin Tang & Huanxin Ju & Tongrui Li & Run Lv & Shengtao Cui & Yingguo Yang & Yuping Sun & Junfa Zhu & Xingyu Gao & Wenjia, 2024. "Dualistic insulator states in 1T-TaS2 crystals," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    7. Jaka Vodeb & Michele Diego & Yevhenii Vaskivskyi & Leonard Logaric & Yaroslav Gerasimenko & Viktor Kabanov & Benjamin Lipovsek & Marko Topic & Dragan Mihailovic, 2024. "Non-equilibrium quantum domain reconfiguration dynamics in a two-dimensional electronic crystal and a quantum annealer," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    8. Myeongjin Jang & Sol Lee & Fernando Cantos-Prieto & Ivona Košić & Yue Li & Arthur R. C. McCray & Min-Hyoung Jung & Jun-Yeong Yoon & Loukya Boddapati & Francis Leonard Deepak & Hu Young Jeong & Charuda, 2024. "Direct observation of twisted stacking domains in the van der Waals magnet CrI3," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    9. James L. Hart & Saif Siddique & Noah Schnitzer & Stephen D. Funni & Lena F. Kourkoutis & Judy J. Cha, 2023. "In operando cryo-STEM of pulse-induced charge density wave switching in TaS2," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    10. Yun Cheng & Alfred Zong & Jun Li & Wei Xia & Shaofeng Duan & Wenxuan Zhao & Yidian Li & Fengfeng Qi & Jun Wu & Lingrong Zhao & Pengfei Zhu & Xiao Zou & Tao Jiang & Yanfeng Guo & Lexian Yang & Dong Qia, 2022. "Light-induced dimension crossover dictated by excitonic correlations," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    11. Sung-Hoon Lee & Doohee Cho, 2023. "Charge density wave surface reconstruction in a van der Waals layered material," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    12. Hongguang Wang & Jiawei Zhang & Chen Shen & Chao Yang & Kathrin Küster & Julia Deuschle & Ulrich Starke & Hongbin Zhang & Masahiko Isobe & Dennis Huang & Peter A. van Aken & Hidenori Takagi, 2024. "Direct visualization of stacking-selective self-intercalation in epitaxial Nb1+xSe2 films," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    13. Nguyen Nhat Quyen & Wen-Yen Tzeng & Chih-En Hsu & I-An Lin & Wan-Hsin Chen & Hao-Hsiang Jia & Sheng-Chiao Wang & Cheng-En Liu & Yu-Sheng Chen & Wei-Liang Chen & Ta-Lei Chou & I-Ta Wang & Chia-Nung Kuo, 2024. "Three-dimensional ultrafast charge-density-wave dynamics in CuTe," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    14. Quanzhen Zhang & Wen-Yu He & Yu Zhang & Yaoyao Chen & Liangguang Jia & Yanhui Hou & Hongyan Ji & Huixia Yang & Teng Zhang & Liwei Liu & Hong-Jun Gao & Thomas A. Jung & Yeliang Wang, 2024. "Quantum spin liquid signatures in monolayer 1T-NbSe2," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41780-y. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.