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Two-dimensional charge order stabilized in clean polytype heterostructures

Author

Listed:
  • Suk Hyun Sung

    (University of Michigan)

  • Noah Schnitzer

    (Cornell University
    Kavli Institute at Cornell for Nanoscale Science)

  • Steve Novakov

    (University of Michigan)

  • Ismail El Baggari

    (Cornell University
    Rowland Institute at Harvard)

  • Xiangpeng Luo

    (University of Michigan)

  • Jiseok Gim

    (University of Michigan)

  • Nguyen M. Vu

    (University of Michigan)

  • Zidong Li

    (University of Michigan)

  • Todd H. Brintlinger

    (U.S. Naval Research Laboratory)

  • Yu Liu

    (Chinese Academy of Sciences)

  • Wenjian Lu

    (Chinese Academy of Sciences)

  • Yuping Sun

    (Chinese Academy of Sciences
    Chinese Academy of Sciences
    Nanjing University)

  • Parag B. Deotare

    (University of Michigan
    University of Michigan)

  • Kai Sun

    (University of Michigan)

  • Liuyan Zhao

    (University of Michigan)

  • Lena F. Kourkoutis

    (Kavli Institute at Cornell for Nanoscale Science
    Cornell University)

  • John T. Heron

    (University of Michigan
    University of Michigan)

  • Robert Hovden

    (University of Michigan
    University of Michigan)

Abstract

Compelling evidence suggests distinct correlated electron behavior may exist only in clean 2D materials such as 1T-TaS2. Unfortunately, experiment and theory suggest that extrinsic disorder in free standing 2D layers disrupts correlation-driven quantum behavior. Here we demonstrate a route to realizing fragile 2D quantum states through endotaxial polytype engineering of van der Waals materials. The true isolation of 2D charge density waves (CDWs) between metallic layers stabilizes commensurate long-range order and lifts the coupling between neighboring CDW layers to restore mirror symmetries via interlayer CDW twinning. The twinned-commensurate charge density wave (tC-CDW) reported herein has a single metal–insulator phase transition at ~350 K as measured structurally and electronically. Fast in-situ transmission electron microscopy and scanned nanobeam diffraction map the formation of tC-CDWs. This work introduces endotaxial polytype engineering of van der Waals materials to access latent 2D ground states distinct from conventional 2D fabrication.

Suggested Citation

  • Suk Hyun Sung & Noah Schnitzer & Steve Novakov & Ismail El Baggari & Xiangpeng Luo & Jiseok Gim & Nguyen M. Vu & Zidong Li & Todd H. Brintlinger & Yu Liu & Wenjian Lu & Yuping Sun & Parag B. Deotare &, 2022. "Two-dimensional charge order stabilized in clean polytype heterostructures," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-021-27947-5
    DOI: 10.1038/s41467-021-27947-5
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    References listed on IDEAS

    as
    1. Efrén Navarro-Moratalla & Joshua O. Island & Samuel Mañas-Valero & Elena Pinilla-Cienfuegos & Andres Castellanos-Gomez & Jorge Quereda & Gabino Rubio-Bollinger & Luca Chirolli & Jose Angel Silva-Guill, 2016. "Enhanced superconductivity in atomically thin TaS2," Nature Communications, Nature, vol. 7(1), pages 1-7, April.
    2. R. Ang & Z. C. Wang & C. L. Chen & J. Tang & N. Liu & Y. Liu & W. J. Lu & Y. P. Sun & T. Mori & Y. Ikuhara, 2015. "Atomistic origin of an ordered superstructure induced superconductivity in layered chalcogenides," Nature Communications, Nature, vol. 6(1), pages 1-6, May.
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    Cited by:

    1. Samra Husremović & Berit H. Goodge & Matthew P. Erodici & Katherine Inzani & Alberto Mier & Stephanie M. Ribet & Karen C. Bustillo & Takashi Taniguchi & Kenji Watanabe & Colin Ophus & Sinéad M. Griffi, 2023. "Encoding multistate charge order and chirality in endotaxial heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    2. Myeongjin Jang & Sol Lee & Fernando Cantos-Prieto & Ivona Košić & Yue Li & Arthur R. C. McCray & Min-Hyoung Jung & Jun-Yeong Yoon & Loukya Boddapati & Francis Leonard Deepak & Hu Young Jeong & Charuda, 2024. "Direct observation of twisted stacking domains in the van der Waals magnet CrI3," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. Hongguang Wang & Jiawei Zhang & Chen Shen & Chao Yang & Kathrin Küster & Julia Deuschle & Ulrich Starke & Hongbin Zhang & Masahiko Isobe & Dennis Huang & Peter A. van Aken & Hidenori Takagi, 2024. "Direct visualization of stacking-selective self-intercalation in epitaxial Nb1+xSe2 films," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Suk Hyun Sung & Nishkarsh Agarwal & Ismail El Baggari & Patrick Kezer & Yin Min Goh & Noah Schnitzer & Jeremy M. Shen & Tony Chiang & Yu Liu & Wenjian Lu & Yuping Sun & Lena F. Kourkoutis & John T. He, 2024. "Endotaxial stabilization of 2D charge density waves with long-range order," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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