IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-40136-w.html
   My bibliography  Save this article

Unlocking full and fast conversion in photocatalytic carbon dioxide reduction for applications in radio-carbonylation

Author

Listed:
  • Serena Monticelli

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Alex Talbot

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Philipp Gotico

    (Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell)

  • Fabien Caillé

    (Université Paris-Saclay, Inserm, CNRS, CEA, Laboratoire d’Imagerie Biomédicale Multimodale Paris-Saclay (BioMaps))

  • Olivier Loreau

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Antonio Vecchio

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Augustin Malandain

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Antoine Sallustrau

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Winfried Leibl

    (Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell)

  • Ally Aukauloo

    (Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell
    Université Paris-Saclay, CNRS, Institut de chimie moléculaire et des matériaux d’Orsay)

  • Frédéric Taran

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Zakaria Halime

    (Université Paris-Saclay, CNRS, Institut de chimie moléculaire et des matériaux d’Orsay)

  • Davide Audisio

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

Abstract

Harvesting sunlight to drive carbon dioxide (CO2) valorisation represents an ideal concept to support a sustainable and carbon-neutral economy. While the photochemical reduction of CO2 to carbon monoxide (CO) has emerged as a hot research topic, the full CO2-to-CO conversion remains an often-overlooked criterion that prevents a productive and direct valorisation of CO into high-value-added chemicals. Herein, we report a photocatalytic process that unlocks full and fast CO2-to-CO conversion (

Suggested Citation

  • Serena Monticelli & Alex Talbot & Philipp Gotico & Fabien Caillé & Olivier Loreau & Antonio Vecchio & Augustin Malandain & Antoine Sallustrau & Winfried Leibl & Ally Aukauloo & Frédéric Taran & Zakari, 2023. "Unlocking full and fast conversion in photocatalytic carbon dioxide reduction for applications in radio-carbonylation," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-40136-w
    DOI: 10.1038/s41467-023-40136-w
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-40136-w
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-023-40136-w?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Yuan-Sheng Xia & Meizhong Tang & Lei Zhang & Jiang Liu & Cheng Jiang & Guang-Kuo Gao & Long-Zhang Dong & Lan-Gui Xie & Ya-Qian Lan, 2022. "Tandem utilization of CO2 photoreduction products for the carbonylation of aryl iodides," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    2. Zutao Ouyang & Pietro Sciusco & Tong Jiao & Sarah Feron & Cheyenne Lei & Fei Li & Ranjeet John & Peilei Fan & Xia Li & Christopher A. Williams & Guangzhao Chen & Chenghao Wang & Jiquan Chen, 2022. "Albedo changes caused by future urbanization contribute to global warming," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    3. Rui Sang & Yuya Hu & Rauf Razzaq & Guillaume Mollaert & Hanan Atia & Ursula Bentrup & Muhammad Sharif & Helfried Neumann & Henrik Junge & Ralf Jackstell & Bert U. W. Maes & Matthias Beller, 2022. "A practical concept for catalytic carbonylations using carbon dioxide," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Annan Chen & Chuanfeng Zhao & Haotian Zhang & Yikun Yang & Jiefeng Li, 2024. "Surface albedo regulates aerosol direct climate effect," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    2. Junzhou Yu & Wenzheng Hu & Ting Deng, 2024. "Towards more resilient economy—analyzing the impact of new-type urbanization on urban economic resilience: mechanisms and spatial spillover boundaries," Economic Change and Restructuring, Springer, vol. 57(5), pages 1-41, October.
    3. Yuman Qin & Robin Cauwenbergh & Suman Pradhan & Rakesh Maiti & Philippe Franck & Shoubhik Das, 2023. "Straightforward synthesis of functionalized γ-Lactams using impure CO2 stream as the carbon source," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    4. Xianyu Deng & Jianjun Zhang & Kezhen Qi & Guijie Liang & Feiyan Xu & Jiaguo Yu, 2024. "Ultrafast electron transfer at the In2O3/Nb2O5 S-scheme interface for CO2 photoreduction," Nature Communications, Nature, vol. 15(1), pages 1-12, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-40136-w. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.