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Circularly polarized electroluminescence from a single-crystal organic microcavity light-emitting diode based on photonic spin-orbit interactions

Author

Listed:
  • Jichao Jia

    (Capital Normal University)

  • Xue Cao

    (Capital Normal University)

  • Xuekai Ma

    (Universität Paderborn)

  • Jianbo De

    (Tianjin University, and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin))

  • Jiannian Yao

    (Tianjin University, and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin))

  • Stefan Schumacher

    (Universität Paderborn
    University of Arizona)

  • Qing Liao

    (Capital Normal University)

  • Hongbing Fu

    (Capital Normal University)

Abstract

Circularly polarized (CP) electroluminescence from organic light-emitting diodes (OLEDs) has aroused considerable attention for their potential in future display and photonic technologies. The development of CP-OLEDs relies largely on chiral-emitters, which not only remain rare owing to difficulties in design and synthesis but also limit the performance of electroluminescence. When the polarization (pseudospin) degrees of freedom of a photon interact with its orbital angular momentum, photonic spin-orbit interaction (SOI) emerges such as Rashba-Dresselhaus (RD) effect. Here, we demonstrate a chiral-emitter-free microcavity CP-OLED with a high dissymmetry factor (gEL) and high luminance by embedding a thin two-dimensional organic single crystal (2D-OSC) between two silver layers which serve as two metallic mirrors forming a microcavity and meanwhile also as two electrodes in an OLED architecture. In the presence of the RD effect, the SOIs in the birefringent 2D-OSC microcavity result in a controllable spin-splitting with CP dispersions. Thanks to the high emission efficiency and high carrier mobility of the OSC, chiral-emitter-free CP-OLEDs have been demonstrated exhibiting a high gEL of 1.1 and a maximum luminance of about 60000 cd/m2, which places our device among the best performing CP-OLEDs. This strategy opens an avenue for practical applications towards on-chip microcavity CP-OLEDs.

Suggested Citation

  • Jichao Jia & Xue Cao & Xuekai Ma & Jianbo De & Jiannian Yao & Stefan Schumacher & Qing Liao & Hongbing Fu, 2023. "Circularly polarized electroluminescence from a single-crystal organic microcavity light-emitting diode based on photonic spin-orbit interactions," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-022-35745-w
    DOI: 10.1038/s41467-022-35745-w
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    References listed on IDEAS

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    1. Kerry J. Vahala, 2003. "Optical microcavities," Nature, Nature, vol. 424(6950), pages 839-846, August.
    2. Zongsu Han & Kunyu Wang & Yifan Guo & Wenjie Chen & Jiale Zhang & Xinran Zhang & Giuliano Siligardi & Sihai Yang & Zhen Zhou & Pingchuan Sun & Wei Shi & Peng Cheng, 2019. "Cation-induced chirality in a bifunctional metal-organic framework for quantitative enantioselective recognition," Nature Communications, Nature, vol. 10(1), pages 1-7, December.
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    Cited by:

    1. Ufuk Kilic & Matthew Hilfiker & Shawn Wimer & Alexander Ruder & Eva Schubert & Mathias Schubert & Christos Argyropoulos, 2024. "Controlling the broadband enhanced light chirality with L-shaped dielectric metamaterials," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    2. Mingjian Zeng & Weiguang Wang & Shuman Zhang & Zhisheng Gao & Yingmeng Yan & Yitong Liu & Yulong Qi & Xin Yan & Wei Zhao & Xin Zhang & Ningning Guo & Huanhuan Li & Hui Li & Gaozhan Xie & Ye Tao & Runf, 2024. "Enabling robust blue circularly polarized organic afterglow through self-confining isolated chiral chromophore," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

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