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Self-rolling of vanadium dioxide nanomembranes for enhanced multi-level solar modulation

Author

Listed:
  • Xing Li

    (Fudan University
    Yiwu Research Institute of Fudan University
    Fudan University)

  • Cuicui Cao

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Chang Liu

    (Fudan University
    Yiwu Research Institute of Fudan University
    Fudan University)

  • Wenhao He

    (Fudan University)

  • Kaibo Wu

    (Fudan University
    Yiwu Research Institute of Fudan University)

  • Yang Wang

    (Fudan University
    Yiwu Research Institute of Fudan University
    Fudan University)

  • Borui Xu

    (Fudan University
    Yiwu Research Institute of Fudan University)

  • Ziao Tian

    (Chinese Academy of Sciences)

  • Enming Song

    (Fudan University
    Fudan University)

  • Jizhai Cui

    (Fudan University
    Yiwu Research Institute of Fudan University
    Fudan University)

  • Gaoshan Huang

    (Fudan University
    Yiwu Research Institute of Fudan University
    Fudan University)

  • Changlin Zheng

    (Fudan University)

  • Zengfeng Di

    (Chinese Academy of Sciences)

  • Xun Cao

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Yongfeng Mei

    (Fudan University
    Yiwu Research Institute of Fudan University
    Fudan University
    Fudan University)

Abstract

Thermochromic window develops as a competitive solution for carbon emissions due to comprehensive advantages of its passivity and effective utilization of energy. How to further enhance the solar modulation ( $${\triangle T}_{{{{{{{\rm{sol}}}}}}}}$$ △ T sol ) of thermochromic windows while ensuring high luminous transmittance ( $${T}_{{{{{{{\rm{lum}}}}}}}}$$ T lum ) becomes the latest challenge to touch the limit of energy efficiency. Here, we show a smart window combining mechanochromism with thermochromism by self-rolling of vanadium dioxide (VO2) nanomembranes to enhance multi-level solar modulation. The mechanochromism is introduced by the temperature-controlled regulation of curvature of rolled-up smart window, which benefits from effective strain adjustment in VO2 nanomembranes upon the phase transition. Under geometry design and optimization, the rolled-up smart window with high $${\triangle T}_{{{{\rm{sol}}}}}$$ △ T sol and $${T}_{{{{{{\rm{lum}}}}}}}$$ T lum is achieved for the modulation of indoor temperature self-adapted to seasons and climate. Furthermore, such rolled-up smart window enables high infrared reflectance after triggered phase transition and acts as a smart lens protective cover for strong radiation. This work supports the feasibility of self-rolling technology in smart windows and lens protection, which promises broad interest and practical applications of self-adapting devices and systems for smart building, intelligent sensors and actuators with the perspective of energy efficiency.

Suggested Citation

  • Xing Li & Cuicui Cao & Chang Liu & Wenhao He & Kaibo Wu & Yang Wang & Borui Xu & Ziao Tian & Enming Song & Jizhai Cui & Gaoshan Huang & Changlin Zheng & Zengfeng Di & Xun Cao & Yongfeng Mei, 2022. "Self-rolling of vanadium dioxide nanomembranes for enhanced multi-level solar modulation," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-35513-w
    DOI: 10.1038/s41467-022-35513-w
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    References listed on IDEAS

    as
    1. Lei Zhao & Xuhui Lee & Ronald B. Smith & Keith Oleson, 2014. "Strong contributions of local background climate to urban heat islands," Nature, Nature, vol. 511(7508), pages 216-219, July.
    2. Borui Xu & Xinyuan Zhang & Ziao Tian & Di Han & Xingce Fan & Yimeng Chen & Zengfeng Di & Teng Qiu & Yongfeng Mei, 2019. "Microdroplet-guided intercalation and deterministic delamination towards intelligent rolling origami," Nature Communications, Nature, vol. 10(1), pages 1-10, December.
    3. Wang, Shancheng & Owusu, Kwadwo Asare & Mai, Liqiang & Ke, Yujie & Zhou, Yang & Hu, Peng & Magdassi, Shlomo & Long, Yi, 2018. "Vanadium dioxide for energy conservation and energy storage applications: Synthesis and performance improvement," Applied Energy, Elsevier, vol. 211(C), pages 200-217.
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