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Vanadium dioxide for energy conservation and energy storage applications: Synthesis and performance improvement

Author

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  • Wang, Shancheng
  • Owusu, Kwadwo Asare
  • Mai, Liqiang
  • Ke, Yujie
  • Zhou, Yang
  • Hu, Peng
  • Magdassi, Shlomo
  • Long, Yi

Abstract

Vanadium dioxide (VO2) is one of the most widely studied inorganic phase change material for energy storage and energy conservation applications. Monoclinic VO2 [VO2(M)] changes from semiconducting phase to metallic rutile phase at near room temperature and the resultant abrupt suppressed infrared transmittance at high temperature makes it a potential candidate for thermochromic smart window application to cut the air-condition usage. Meanwhile proper electrical potential, stable structure and good interaction with lithium ions make metastable VO2 [VO2(B)] an attractive material for fabrication of electrodes for batteries and supercapacitors. However, some long-standing issues have plagued its usage. In thermochromic application, high transition temperature (τc), low luminous transmittance (Tlum) and undesirable solar modulation ability (△Tsol) are the key problems, while in energy storage applications, short cycling lifetime and complex three-dimension microstructure are the major challenges. The common methods to produce VO2 polymorph are physical vapour deposition (PVD), chemical vapour deposition (CVD), sol-gel synthesis, and hydrothermal method. CVD is an intensively studied method due to its ability to produce uniform films with precise stoichiometry, phase and morphology control. This paper reviews the various CVD techniques to produce VO2 with controlled phases and the ternary diagram shows the relationship between film stoichiometry and various process conditions. The difference between the various CVD systems are commented and the process window to produce VO2 are tabulated. Some strategies to improve VO2′s performance in both energy conservation and energy storage applications are discussed.

Suggested Citation

  • Wang, Shancheng & Owusu, Kwadwo Asare & Mai, Liqiang & Ke, Yujie & Zhou, Yang & Hu, Peng & Magdassi, Shlomo & Long, Yi, 2018. "Vanadium dioxide for energy conservation and energy storage applications: Synthesis and performance improvement," Applied Energy, Elsevier, vol. 211(C), pages 200-217.
    • Handle: RePEc:eee:appene:v:211:y:2018:i:c:p:200-217
    DOI: 10.1016/j.apenergy.2017.11.039
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    2. Zeng, Jimin & Liu, Lidong & Liang, Xiao & Chen, Shihe & Yuan, Jun, 2021. "Evaluating fuel consumption factor for energy conservation and carbon neutral on an industrial thermal power unit," Energy, Elsevier, vol. 232(C).
    3. Liu, Sai & Tso, Chi Yan & Du, Yu Wei & Chao, Luke Christopher & Lee, Hau Him & Ho, Tsz Chung & Leung, Michael Kwok Hi, 2021. "Bioinspired thermochromic transparent hydrogel wood with advanced optical regulation abilities and mechanical properties for windows," Applied Energy, Elsevier, vol. 297(C).
    4. Ke, Yujie & Tan, Yutong & Feng, Chengchen & Chen, Cong & Lu, Qi & Xu, Qiyang & Wang, Tao & Liu, Hai & Liu, Xinghai & Peng, Jinqing & Long, Yi, 2022. "Tetra-Fish-Inspired aesthetic thermochromic windows toward Energy-Saving buildings," Applied Energy, Elsevier, vol. 315(C).
    5. Shi, Yu & Eze, Chika & Xiong, Binyu & He, Weidong & Zhang, Han & Lim, T.M. & Ukil, A. & Zhao, Jiyun, 2019. "Recent development of membrane for vanadium redox flow battery applications: A review," Applied Energy, Elsevier, vol. 238(C), pages 202-224.
    6. Zhao, Xinpeng & Mofid, Sohrab Alex & Jelle, Bjørn Petter & Tan, Gang & Yin, Xiaobo & Yang, Ronggui, 2020. "Optically-switchable thermally-insulating VO2-aerogel hybrid film for window retrofits," Applied Energy, Elsevier, vol. 278(C).
    7. Wu, Yongjia & Gao, Yahui & Wang, Caixia & Chen, Qiong & Ming, Tingzhen, 2023. "The energy saving performance of the thermal diode composite wall in different climate regions," Renewable Energy, Elsevier, vol. 219(P1).

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