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Multi-angular polarimetric remote sensing to pinpoint global aerosol absorption and direct radiative forcing

Author

Listed:
  • Cheng Chen

    (Univ. Lille, CNRS, UMR 8518 - LOA - Laboratoire d’Optique Atmosphérique
    GRASP-SAS, Univ. Lille)

  • Oleg Dubovik

    (Univ. Lille, CNRS, UMR 8518 - LOA - Laboratoire d’Optique Atmosphérique)

  • Gregory L. Schuster

    (NASA Langley Research Center)

  • Mian Chin

    (NASA Goddard Space Flight Center)

  • Daven K. Henze

    (University of Colorado)

  • Tatyana Lapyonok

    (Univ. Lille, CNRS, UMR 8518 - LOA - Laboratoire d’Optique Atmosphérique)

  • Zhengqiang Li

    (Chinese Academy of Sciences)

  • Yevgeny Derimian

    (Univ. Lille, CNRS, UMR 8518 - LOA - Laboratoire d’Optique Atmosphérique)

  • Ying Zhang

    (Chinese Academy of Sciences)

Abstract

Quantitative estimations of atmospheric aerosol absorption are rather uncertain due to the lack of reliable information about the global distribution. Because the information about aerosol properties is commonly provided by single-viewing photometric satellite sensors that are not sensitive to aerosol absorption. Consequently, the uncertainty in aerosol radiative forcing remains one of the largest in the Assessment Reports of the Intergovernmental Panel on Climate Change (IPCC AR5 and AR6). Here, we use multi-angular polarimeters (MAP) to provide constraints on emission of absorbing aerosol species and estimate global aerosol absorption optical depth (AAOD) and its climate effect. Our estimate of modern-era mid-visible AAOD is 0.0070 that is higher than IPCC by a factor of 1.3-1.8. The black carbon instantaneous direct radiative forcing (BC DRF) is +0.33 W/m2 [+0.17, +0.54]. The MAP constraint narrows the 95% confidence interval of BC DRF by a factor of 2 and boosts confidence in its spatial distribution.

Suggested Citation

  • Cheng Chen & Oleg Dubovik & Gregory L. Schuster & Mian Chin & Daven K. Henze & Tatyana Lapyonok & Zhengqiang Li & Yevgeny Derimian & Ying Zhang, 2022. "Multi-angular polarimetric remote sensing to pinpoint global aerosol absorption and direct radiative forcing," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-35147-y
    DOI: 10.1038/s41467-022-35147-y
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    References listed on IDEAS

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    1. Yoram J. Kaufman & Didier Tanré & Olivier Boucher, 2002. "A satellite view of aerosols in the climate system," Nature, Nature, vol. 419(6903), pages 215-223, September.
    2. Mark Z. Jacobson, 2001. "Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols," Nature, Nature, vol. 409(6821), pages 695-697, February.
    3. Nicolas Bellouin & Olivier Boucher & Jim Haywood & M. Shekar Reddy, 2005. "Global estimate of aerosol direct radiative forcing from satellite measurements," Nature, Nature, vol. 438(7071), pages 1138-1141, December.
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