IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-34377-4.html
   My bibliography  Save this article

Electronically phase separated nano-network in antiferromagnetic insulating LaMnO3/PrMnO3/CaMnO3 tricolor superlattice

Author

Listed:
  • Qiang Li

    (Fudan University
    Fudan University)

  • Tian Miao

    (Fudan University
    Xi’an Jiaotong University)

  • Huimin Zhang

    (Fudan University
    Fudan University
    Shanghai Qi Zhi Institute)

  • Weiyan Lin

    (Fudan University)

  • Wenhao He

    (Fudan University
    Fudan University)

  • Yang Zhong

    (Fudan University
    Fudan University
    Shanghai Qi Zhi Institute)

  • Lifen Xiang

    (Fudan University)

  • Lina Deng

    (Fudan University)

  • Biying Ye

    (Fudan University)

  • Qian Shi

    (Fudan University)

  • Yinyan Zhu

    (Fudan University
    Shanghai Qi Zhi Institute
    Fudan University)

  • Hangwen Guo

    (Fudan University
    Shanghai Qi Zhi Institute
    Fudan University)

  • Wenbin Wang

    (Fudan University
    Shanghai Qi Zhi Institute
    Fudan University)

  • Changlin Zheng

    (Fudan University
    Fudan University)

  • Lifeng Yin

    (Fudan University
    Fudan University
    Shanghai Qi Zhi Institute
    Fudan University)

  • Xiaodong Zhou

    (Fudan University
    Shanghai Qi Zhi Institute
    Fudan University)

  • Hongjun Xiang

    (Fudan University
    Fudan University
    Shanghai Qi Zhi Institute)

  • Jian Shen

    (Fudan University
    Fudan University
    Shanghai Qi Zhi Institute
    Fudan University)

Abstract

Strongly correlated materials often exhibit an electronic phase separation (EPS) phenomena whose domain pattern is random in nature. The ability to control the spatial arrangement of the electronic phases at microscopic scales is highly desirable for tailoring their macroscopic properties and/or designing novel electronic devices. Here we report the formation of EPS nanoscale network in a mono-atomically stacked LaMnO3/CaMnO3/PrMnO3 superlattice grown on SrTiO3 (STO) (001) substrate, which is known to have an antiferromagnetic (AFM) insulating ground state. The EPS nano-network is a consequence of an internal strain relaxation triggered by the structural domain formation of the underlying STO substrate at low temperatures. The same nanoscale network pattern can be reproduced upon temperature cycling allowing us to employ different local imaging techniques to directly compare the magnetic and transport state of a single EPS domain. Our results confirm the one-to-one correspondence between ferromagnetic (AFM) to metallic (insulating) state in manganite. It also represents a significant step in a paradigm shift from passively characterizing EPS in strongly correlated systems to actively engaging in its manipulation.

Suggested Citation

  • Qiang Li & Tian Miao & Huimin Zhang & Weiyan Lin & Wenhao He & Yang Zhong & Lifen Xiang & Lina Deng & Biying Ye & Qian Shi & Yinyan Zhu & Hangwen Guo & Wenbin Wang & Changlin Zheng & Lifeng Yin & Xiao, 2022. "Electronically phase separated nano-network in antiferromagnetic insulating LaMnO3/PrMnO3/CaMnO3 tricolor superlattice," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34377-4
    DOI: 10.1038/s41467-022-34377-4
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-34377-4
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-022-34377-4?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Sasikanth Manipatruni & Dmitri E. Nikonov & Chia-Ching Lin & Tanay A. Gosavi & Huichu Liu & Bhagwati Prasad & Yen-Lin Huang & Everton Bonturim & Ramamoorthy Ramesh & Ian A. Young, 2019. "Scalable energy-efficient magnetoelectric spin–orbit logic," Nature, Nature, vol. 565(7737), pages 35-42, January.
    2. Kai Du & Kai Zhang & Shuai Dong & Wengang Wei & Jian Shao & Jiebin Niu & Jinjie Chen & Yinyan Zhu & Hanxuan Lin & Xiaolu Yin & Sy-Hwang Liou & Lifeng Yin & Jian Shen, 2015. "Visualization of a ferromagnetic metallic edge state in manganite strips," Nature Communications, Nature, vol. 6(1), pages 1-5, May.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Freddie Hendriks & Rafael R. Rojas-Lopez & Bert Koopmans & Marcos H. D. Guimarães, 2024. "Electric control of optically-induced magnetization dynamics in a van der Waals ferromagnetic semiconductor," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    2. Piyush Agarwal & Lisen Huang & Sze Lim & Ranjan Singh, 2022. "Electric-field control of nonlinear THz spintronic emitters," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    3. Sajid Husain & Isaac Harris & Guanhui Gao & Xinyan Li & Peter Meisenheimer & Chuqiao Shi & Pravin Kavle & Chi Hun Choi & Tae Yeon Kim & Deokyoung Kang & Piush Behera & Didier Perrodin & Hua Guo & Jame, 2024. "Low-temperature grapho-epitaxial La-substituted BiFeO3 on metallic perovskite," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    4. Xianghan Xu & Yiqing Hao & Shiyu Peng & Qiang Zhang & Danrui Ni & Chen Yang & Xi Dai & Huibo Cao & R. J. Cava, 2023. "Large off-diagonal magnetoelectricity in a triangular Co2+-based collinear antiferromagnet," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    5. Peter Meisenheimer & Guy Moore & Shiyu Zhou & Hongrui Zhang & Xiaoxi Huang & Sajid Husain & Xianzhe Chen & Lane W. Martin & Kristin A. Persson & Sinéad Griffin & Lucas Caretta & Paul Stevenson & Ramam, 2024. "Switching the spin cycloid in BiFeO3 with an electric field," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    6. Min-Gu Kang & Jong-Guk Choi & Jimin Jeong & Jae Yeol Park & Hyeon-Jong Park & Taehwan Kim & Taekhyeon Lee & Kab-Jin Kim & Kyoung-Whan Kim & Jung Hyun Oh & Duc Duong Viet & Jong-Ryul Jeong & Jong Min Y, 2021. "Electric-field control of field-free spin-orbit torque switching via laterally modulated Rashba effect in Pt/Co/AlOx structures," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    7. Sajid Husain & Isaac Harris & Peter Meisenheimer & Sukriti Mantri & Xinyan Li & Maya Ramesh & Piush Behera & Hossein Taghinejad & Jaegyu Kim & Pravin Kavle & Shiyu Zhou & Tae Yeon Kim & Hongrui Zhang , 2024. "Non-volatile magnon transport in a single domain multiferroic," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    8. Qiwu Shi & Eric Parsonnet & Xiaoxing Cheng & Natalya Fedorova & Ren-Ci Peng & Abel Fernandez & Alexander Qualls & Xiaoxi Huang & Xue Chang & Hongrui Zhang & David Pesquera & Sujit Das & Dmitri Nikonov, 2022. "The role of lattice dynamics in ferroelectric switching," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    9. Jonghyeon Choi & Jungmin Park & Seunghyeon Noh & Jaebyeong Lee & Seunghyun Lee & Daeseong Choe & Hyeonjung Jung & Junhyeon Jo & Inseon Oh & Juwon Han & Soon-Yong Kwon & Chang Won Ahn & Byoung-Chul Min, 2024. "Non-volatile Fermi level tuning for the control of spin-charge conversion at room temperature," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    10. Ellen Fogh & Bastian Klemke & Manfred Reehuis & Philippe Bourges & Christof Niedermayer & Sonja Holm-Dahlin & Oksana Zaharko & Jürg Schefer & Andreas B. Kristensen & Michael K. Sørensen & Sebastian Pa, 2023. "Tuning magnetoelectricity in a mixed-anisotropy antiferromagnet," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    11. Jaeun Eom & In Hak Lee & Jung Yun Kee & Minhyun Cho & Jeongdae Seo & Hoyoung Suh & Hyung-Jin Choi & Yumin Sim & Shuzhang Chen & Hye Jung Chang & Seung-Hyub Baek & Cedomir Petrovic & Hyejin Ryu & Chaun, 2023. "Voltage control of magnetism in Fe3-xGeTe2/In2Se3 van der Waals ferromagnetic/ferroelectric heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-10, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34377-4. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.