IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-34337-y.html
   My bibliography  Save this article

Gate-tunable quantum pathways of high harmonic generation in graphene

Author

Listed:
  • Soonyoung Cha

    (Institute for Basic Science (IBS))

  • Minjeong Kim

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Youngjae Kim

    (Daegu Gyeongbuk Institute of Science and Technology (DGIST))

  • Shinyoung Choi

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Sejong Kang

    (Pohang University of Science and Technology)

  • Hoon Kim

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Sangho Yoon

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Gunho Moon

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Taeho Kim

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Ye Won Lee

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • Gil Young Cho

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology
    Asia Pacific Center for Theoretical Physics)

  • Moon Jeong Park

    (Pohang University of Science and Technology)

  • Cheol-Joo Kim

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • B. J. Kim

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology)

  • JaeDong Lee

    (Daegu Gyeongbuk Institute of Science and Technology (DGIST))

  • Moon-Ho Jo

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology
    Pohang University of Science and Technology)

  • Jonghwan Kim

    (Institute for Basic Science (IBS)
    Pohang University of Science and Technology
    Pohang University of Science and Technology)

Abstract

Under strong laser fields, electrons in solids radiate high-harmonic fields by travelling through quantum pathways in Bloch bands in the sub-laser-cycle timescales. Understanding these pathways in the momentum space through the high-harmonic radiation can enable an all-optical ultrafast probe to observe coherent lightwave-driven processes and measure electronic structures as recently demonstrated for semiconductors. However, such demonstration has been largely limited for semimetals because the absence of the bandgap hinders an experimental characterization of the exact pathways. In this study, by combining electrostatic control of chemical potentials with HHG measurement, we resolve quantum pathways of massless Dirac fermions in graphene under strong laser fields. Electrical modulation of HHG reveals quantum interference between the multi-photon interband excitation channels. As the light-matter interaction deviates beyond the perturbative regime, elliptically polarized laser fields efficiently drive massless Dirac fermions via an intricate coupling between the interband and intraband transitions, which is corroborated by our theoretical calculations. Our findings pave the way for strong-laser-field tomography of Dirac electrons in various quantum semimetals and their ultrafast electronics with a gate control.

Suggested Citation

  • Soonyoung Cha & Minjeong Kim & Youngjae Kim & Shinyoung Choi & Sejong Kang & Hoon Kim & Sangho Yoon & Gunho Moon & Taeho Kim & Ye Won Lee & Gil Young Cho & Moon Jeong Park & Cheol-Joo Kim & B. J. Kim , 2022. "Gate-tunable quantum pathways of high harmonic generation in graphene," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34337-y
    DOI: 10.1038/s41467-022-34337-y
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-34337-y
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-022-34337-y?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Nicolas Tancogne-Dejean & Oliver D. Mücke & Franz X. Kärtner & Angel Rubio, 2017. "Publisher Correction: Ellipticity dependence of high-harmonic generation in solids originating from coupled intraband and interband dynamics," Nature Communications, Nature, vol. 8(1), pages 1-1, December.
    2. C. P. Schmid & L. Weigl & P. Grössing & V. Junk & C. Gorini & S. Schlauderer & S. Ito & M. Meierhofer & N. Hofmann & D. Afanasiev & J. Crewse & K. A. Kokh & O. E. Tereshchenko & J. Güdde & F. Evers & , 2021. "Tunable non-integer high-harmonic generation in a topological insulator," Nature, Nature, vol. 593(7859), pages 385-390, May.
    3. T. T. Luu & M. Garg & S. Yu. Kruchinin & A. Moulet & M. Th. Hassan & E. Goulielmakis, 2015. "Extreme ultraviolet high-harmonic spectroscopy of solids," Nature, Nature, vol. 521(7553), pages 498-502, May.
    4. K. S. Novoselov & A. K. Geim & S. V. Morozov & D. Jiang & M. I. Katsnelson & I. V. Grigorieva & S. V. Dubonos & A. A. Firsov, 2005. "Two-dimensional gas of massless Dirac fermions in graphene," Nature, Nature, vol. 438(7065), pages 197-200, November.
    5. F. Langer & M. Hohenleutner & C. P. Schmid & C. Poellmann & P. Nagler & T. Korn & C. Schüller & M. S. Sherwin & U. Huttner & J. T. Steiner & S. W. Koch & M. Kira & R. Huber, 2016. "Lightwave-driven quasiparticle collisions on a subcycle timescale," Nature, Nature, vol. 533(7602), pages 225-229, May.
    6. J. B. Costello & S. D. O’Hara & Q. Wu & D. C. Valovcin & L. N. Pfeiffer & K. W. West & M. S. Sherwin, 2021. "Reconstruction of Bloch wavefunctions of holes in a semiconductor," Nature, Nature, vol. 599(7883), pages 57-61, November.
    7. B. Zaks & R. B. Liu & M. S. Sherwin, 2012. "Experimental observation of electron–hole recollisions," Nature, Nature, vol. 483(7391), pages 580-583, March.
    8. Tran Trung Luu & Hans Jakob Wörner, 2018. "Measurement of the Berry curvature of solids using high-harmonic spectroscopy," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
    9. Nicolas Tancogne-Dejean & Oliver D. Mücke & Franz X. Kärtner & Angel Rubio, 2017. "Ellipticity dependence of high-harmonic generation in solids originating from coupled intraband and interband dynamics," Nature Communications, Nature, vol. 8(1), pages 1-10, December.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Victor Chang Lee & Lun Yue & Mette B. Gaarde & Yang-hao Chan & Diana Y. Qiu, 2024. "Many-body enhancement of high-harmonic generation in monolayer MoS2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Álvaro Jiménez-Galán & Chandler Bossaer & Guilmot Ernotte & Andrew M. Parks & Rui E. F. Silva & David M. Villeneuve & André Staudte & Thomas Brabec & Adina Luican-Mayer & Giulio Vampa, 2023. "Orbital perspective on high-harmonic generation from solids," Nature Communications, Nature, vol. 14(1), pages 1-6, December.
    3. Sylvianne D. C. Roscam Abbing & Nataliia Kuzkova & Roy Linden & Filippo Campi & Brian Keijzer & Corentin Morice & Zhuang-Yan Zhang & Maarten L. S. Geest & Peter M. Kraus, 2024. "Enhancing the efficiency of high-order harmonics with two-color non-collinear wave mixing in silica," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    4. Yang-Yang Lv & Jinlong Xu & Shuang Han & Chi Zhang & Yadong Han & Jian Zhou & Shu-Hua Yao & Xiao-Ping Liu & Ming-Hui Lu & Hongming Weng & Zhenda Xie & Y. B. Chen & Jianbo Hu & Yan-Feng Chen & Shining , 2021. "High-harmonic generation in Weyl semimetal β-WP2 crystals," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    5. Anffany Chen & Hauke Brand & Tobias Helbig & Tobias Hofmann & Stefan Imhof & Alexander Fritzsche & Tobias Kießling & Alexander Stegmaier & Lavi K. Upreti & Titus Neupert & Tomáš Bzdušek & Martin Greit, 2023. "Hyperbolic matter in electrical circuits with tunable complex phases," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    6. Anh-Luan Phan & Dai-Nam Le, 2021. "Electronic transport in two-dimensional strained Dirac materials under multi-step Fermi velocity barrier: transfer matrix method for supersymmetric systems," The European Physical Journal B: Condensed Matter and Complex Systems, Springer;EDP Sciences, vol. 94(8), pages 1-16, August.
    7. Wang, Qing & Han, Ning & Bokhari, Awais & Li, Xue & Cao, Yue & Asif, Saira & Shen, Zhengfeng & Si, Weimeng & Wang, Fagang & Klemeš, Jiří Jaromír & Zhao, Xiaolin, 2022. "Insights into MXenes-based electrocatalysts for oxygen reduction," Energy, Elsevier, vol. 255(C).
    8. Di Molfetta, Giuseppe & Brachet, Marc & Debbasch, Fabrice, 2014. "Quantum walks in artificial electric and gravitational fields," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 397(C), pages 157-168.
    9. Shidong Yang & Xiwang Liu & Jinyan Lin & Ruixin Zuo & Xiaohong Song & Marcelo Ciappina & Weifeng Yang, 2022. "Reconstructing the Semiconductor Band Structure by Deep Learning," Mathematics, MDPI, vol. 10(22), pages 1-11, November.
    10. Juntao Zhang & Xiaozhi Liu & Yujin Ji & Xuerui Liu & Dong Su & Zhongbin Zhuang & Yu-Chung Chang & Chih-Wen Pao & Qi Shao & Zhiwei Hu & Xiaoqing Huang, 2023. "Atomic-thick metastable phase RhMo nanosheets for hydrogen oxidation catalysis," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    11. Cao, Rui-rui & Li, Xuan & Chen, Sai & Yuan, Hao-ran & Zhang, Xing-xiang, 2017. "Fabrication and characterization of novel shape-stabilized synergistic phase change materials based on PHDA/GO composites," Energy, Elsevier, vol. 138(C), pages 157-166.
    12. González, Ander & Goikolea, Eider & Barrena, Jon Andoni & Mysyk, Roman, 2016. "Review on supercapacitors: Technologies and materials," Renewable and Sustainable Energy Reviews, Elsevier, vol. 58(C), pages 1189-1206.
    13. Dasari, Bhagya Lakshmi & Nouri, Jamshid M. & Brabazon, Dermot & Naher, Sumsun, 2017. "Graphene and derivatives – Synthesis techniques, properties and their energy applications," Energy, Elsevier, vol. 140(P1), pages 766-778.
    14. Chen, Yuanhan, 2024. "Cleaning Russian oil industry for energy resource exploration and industrial transformation towards zero carbon green recovery: Role of inclusive digital finance," Resources Policy, Elsevier, vol. 88(C).
    15. M. T. Greenaway & P. Kumaravadivel & J. Wengraf & L. A. Ponomarenko & A. I. Berdyugin & J. Li & J. H. Edgar & R. Krishna Kumar & A. K. Geim & L. Eaves, 2021. "Graphene’s non-equilibrium fermions reveal Doppler-shifted magnetophonon resonances accompanied by Mach supersonic and Landau velocity effects," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
    16. Maria Karaulova & Abdullah Gök & Oliver Shackleton & Philip Shapira, 2016. "Science system path-dependencies and their influences: nanotechnology research in Russia," Scientometrics, Springer;Akadémiai Kiadó, vol. 107(2), pages 645-670, May.
    17. Zheyu Cheng & Yi-Jun Guan & Haoran Xue & Yong Ge & Ding Jia & Yang Long & Shou-Qi Yuan & Hong-Xiang Sun & Yidong Chong & Baile Zhang, 2024. "Three-dimensional flat Landau levels in an inhomogeneous acoustic crystal," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    18. Ying Zhou & Hongqian Mu & Tongbiao Wang & Tianbao Yu & Qinghua Liao, 2022. "Tunable broadband superradiance near a graphene/hyperbolic metamaterial/graphene sandwich structure," The European Physical Journal B: Condensed Matter and Complex Systems, Springer;EDP Sciences, vol. 95(11), pages 1-10, November.
    19. Benyahia, Ahmed & Bouamrane, Rachid, 2023. "Modelling the minimum conductivity of graphene using random resistor networks," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 626(C).
    20. Xuefei Liu & Zhaocai Zhang & Bing Lv & Zhao Ding & Zijiang Luo, 2021. "Impact of the vertical strain on the Schottky barrier height for graphene/AlN heterojunction: a study by the first-principles method," The European Physical Journal B: Condensed Matter and Complex Systems, Springer;EDP Sciences, vol. 94(1), pages 1-7, January.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34337-y. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.