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Ultra-compact MXene fibers by continuous and controllable synergy of interfacial interactions and thermal drawing-induced stresses

Author

Listed:
  • Tianzhu Zhou

    (Nanyang Technological University
    Beihang University)

  • Yangzhe Yu

    (Beihang University)

  • Bing He

    (Nanyang Technological University)

  • Zhe Wang

    (Nanyang Technological University)

  • Ting Xiong

    (Nanyang Technological University)

  • Zhixun Wang

    (Nanyang Technological University)

  • Yanting Liu

    (Nanyang Technological University)

  • Jiwu Xin

    (Nanyang Technological University)

  • Miao Qi

    (Nanyang Technological University)

  • Haozhe Zhang

    (Nanyang Technological University)

  • Xuhui Zhou

    (Nanyang Technological University)

  • Liheng Gao

    (Nanyang Technological University)

  • Qunfeng Cheng

    (Beihang University
    Zhengzhou University)

  • Lei Wei

    (Nanyang Technological University)

Abstract

Recent advances in MXene (Ti3C2Tx) fibers, prepared from electrically conductive and mechanically strong MXene nanosheets, address the increasing demand of emerging yet promising electrode materials for the development of textile-based devices and beyond. However, to reveal the full potential of MXene fibers, reaching a balance between electrical conductivity and mechanical property is still the fundamental challenge, mainly due to the difficulties to further compact the loose MXene nanosheets. In this work, we demonstrate a continuous and controllable route to fabricate ultra-compact MXene fibers with an in-situ generated protective layer via the synergy of interfacial interactions and thermal drawing-induced stresses. The resulting ultra-compact MXene fibers with high orientation and low porosity exhibit not only excellent tensile strength and ultra-high toughness, but also high electrical conductivity. Then, we construct meter-scale MXene textiles using these ultra-compact fibers to achieve high-performance electromagnetic interference shielding and personal thermal management, accompanied by the high mechanical durability and stability even after multiple washing cycles. The demonstrated generic strategy can be applied to a broad range of nanostructured materials to construct functional fibers for large-scale applications in both space and daily lives.

Suggested Citation

  • Tianzhu Zhou & Yangzhe Yu & Bing He & Zhe Wang & Ting Xiong & Zhixun Wang & Yanting Liu & Jiwu Xin & Miao Qi & Haozhe Zhang & Xuhui Zhou & Liheng Gao & Qunfeng Cheng & Lei Wei, 2022. "Ultra-compact MXene fibers by continuous and controllable synergy of interfacial interactions and thermal drawing-induced stresses," Nature Communications, Nature, vol. 13(1), pages 1-13, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32361-6
    DOI: 10.1038/s41467-022-32361-6
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    References listed on IDEAS

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    1. Wang, Dongfang & Li, Jialong & Zheng, Lun & Sun, Xiang & Sun, Mengfan & Wang, Chen & Bi, Zhaojie & Zhou, Baokai & Wang, Lixia & Li, Qian, 2024. "Lightweight thermoplastic polyurethane/multi-wall carbon nanotube foams with a continuous gradient cell structure for electromagnetic interference shielding," Energy, Elsevier, vol. 304(C).
    2. Snehi Shrestha & Kieran James Barvenik & Tianle Chen & Haochen Yang & Yang Li & Meera Muthachi Kesavan & Joshua M. Little & Hayden C. Whitley & Zi Teng & Yaguang Luo & Eleonora Tubaldi & Po-Yen Chen, 2024. "Machine intelligence accelerated design of conductive MXene aerogels with programmable properties," Nature Communications, Nature, vol. 15(1), pages 1-14, December.

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