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Physical Properties of Ti 45 Zr 38 Fe 17 Alloy and Its Amorphous Hydride

Author

Listed:
  • Antoni Żywczak

    (Academic Centre for Materials and Nanotechnology, 30-059 Krakow, Poland)

  • Łukasz Gondek

    (Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, 30-059 Krakow, Poland)

  • Joanna Czub

    (Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, 30-059 Krakow, Poland)

  • Piotr Janusz

    (Faculty of Drilling, Oil, and Gas, AGH University of Science and Technology, 30-059 Krakow, Poland)

  • Nivas Babu Selvaraj

    (CICECO, Department of Materials and Ceramic Engineering, University of Aveiro, 3810-193 Aveiro, Portugal)

  • Akito Takasaki

    (Department of Engineering Science and Mechanics, Shibaura Institute of Technology, Toyosu, Kotoku, Tokyo 135-8548, Japan)

Abstract

The alloys based on Ti-Zr are considered an excellent candidate for hydrogen storage applications. In this communication, we report the results of Fe substitution for Ni in the well-known Ti 45 Zr 38 Ni 17 compound. The parent and related compounds can be obtained as amorphous powders, transforming into the quasicrystalline phase (i-phase) after annealing. The amorphous Ti 45 Zr 38 Fe 17 phase is transformed into the icosahedral quasicrystalline state, and it is a quasi-continuous process. The i-phase is well-developed close to 500 °C. At higher temperatures, the quasicrystal structure transforms into the other phase: the w-phase (an approximant to the crystalline phase) and another crystal phase with a small addition of the FeZr 3 and the Fe 2 (ZrTi) 3 . The amorphous Ti 45 Zr 38 Fe 17 phases can be hydrogenated while maintaining the amorphous nature, which constitutes another very fascinating research field for our group. The investigated alloy shows a good capacity for gaseous H 2 at level 2.54 wt.% at elevated temperatures. The ferromagnetic signal of the amorphous TiZrFe comes from magnetic nanocrystallites in the amorphous matrix. After heating, the magnetic signal significantly decreases due to the lack of long-range magnetic ordering in the i-phase of the Ti 45 Zr 38 Fe 17 alloy.

Suggested Citation

  • Antoni Żywczak & Łukasz Gondek & Joanna Czub & Piotr Janusz & Nivas Babu Selvaraj & Akito Takasaki, 2022. "Physical Properties of Ti 45 Zr 38 Fe 17 Alloy and Its Amorphous Hydride," Energies, MDPI, vol. 15(12), pages 1-8, June.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:12:p:4236-:d:834592
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    References listed on IDEAS

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    1. Yuchen Liu & Djafar Chabane & Omar Elkedim, 2021. "Intermetallic Compounds Synthesized by Mechanical Alloying for Solid-State Hydrogen Storage: A Review," Energies, MDPI, vol. 14(18), pages 1-22, September.
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    4. Erika Michela Dematteis & Jussara Barale & Marta Corno & Alessandro Sciullo & Marcello Baricco & Paola Rizzi, 2021. "Solid-State Hydrogen Storage Systems and the Relevance of a Gender Perspective," Energies, MDPI, vol. 14(19), pages 1-26, September.
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