IDEAS home Printed from https://ideas.repec.org/a/gam/jeners/v15y2022i10p3702-d818511.html
   My bibliography  Save this article

Developing an Automated Tool for Quantitative Analysis of the Deconvoluted Electrochemical Impedance Response of a Solid Oxide Fuel Cell

Author

Listed:
  • Mohammad Alboghobeish

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy
    Dipartimento di Ingegneria, Università degli Studi di Napoli Parthenope, Centro Direzionale Isola C4, 80143 Napoli, Italy)

  • Andrea Monforti Ferrario

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy
    Department of Industrial Engineering and Mathematical Sciences, Università Politecnica delle Marche, Via Brecce Bianche, 60131 Ancona, Italy)

  • Davide Pumiglia

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy)

  • Massimiliano Della Pietra

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy)

  • Stephen J. McPhail

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy)

  • Sergii Pylypko

    (Elcogen AS, Valukoja 23, 11415 Tallinn, Estonia)

  • Domenico Borello

    (Dipartimento di Ingegneria Meccanica e Aerospaziale (DIMA), Sapienza University of Rome, Via Eudossiana, 18, 00184 Roma, Italy)

Abstract

Despite being commercially available, solid oxide fuel cell (SOFC) technology requires further study to understand its physicochemical processes for diagnostics, prognostics, and quality assurance purposes. Electrochemical impedance spectroscopy (EIS), a widely used characterization technique for SOFCs, is often accompanied by the distribution of relaxation times (DRT) as a method for deconvoluting the contribution of each physicochemical process from the aggregated impedance response spectra. While EIS yields valuable information for the operation of SOFCs, the quantitative analysis of the DRT and its shifts remains cumbersome. To address this issue, and to create a replicable benchmark for the assessment of DRT results, a custom tool was developed in MATLAB to numerically analyze the DRT spectra, identify the DRT peaks, and assess their deviation in terms of peak frequency and DRT amplitude from nominal operating conditions. The preliminary validation of the tool was carried out by applying the tool to an extensive experimental campaign on 23 SOFC button-sized samples from three production batches in which EIS measurements were performed in parametric operating conditions. It was concluded that the results of the automated analysis via the developed tool were in accordance with the qualitative analysis of previous studies. It is capable of providing adequate additional quantitative results in terms of DRT shifts for further analysis and provides the basis for better interoperability of DRT analyses between laboratories.

Suggested Citation

  • Mohammad Alboghobeish & Andrea Monforti Ferrario & Davide Pumiglia & Massimiliano Della Pietra & Stephen J. McPhail & Sergii Pylypko & Domenico Borello, 2022. "Developing an Automated Tool for Quantitative Analysis of the Deconvoluted Electrochemical Impedance Response of a Solid Oxide Fuel Cell," Energies, MDPI, vol. 15(10), pages 1-22, May.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:10:p:3702-:d:818511
    as

    Download full text from publisher

    File URL: https://www.mdpi.com/1996-1073/15/10/3702/pdf
    Download Restriction: no
    File URL: https://www.mdpi.com/1996-1073/15/10/3702/
    Download Restriction: no
    ---><---

    References listed on IDEAS

    as
    1. Silva-Mosqueda, Dulce María & Elizalde-Blancas, Francisco & Pumiglia, Davide & Santoni, Francesca & Boigues-Muñoz, Carlos & McPhail, Stephen J., 2019. "Intermediate temperature solid oxide fuel cell under internal reforming: Critical operating conditions, associated problems and their impact on the performance," Applied Energy, Elsevier, vol. 235(C), pages 625-640.
    2. Arsalis, Alexandros, 2019. "A comprehensive review of fuel cell-based micro-combined-heat-and-power systems," Renewable and Sustainable Energy Reviews, Elsevier, vol. 105(C), pages 391-414.
    3. Choudhury, Arnab & Chandra, H. & Arora, A., 2013. "Application of solid oxide fuel cell technology for power generation—A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 20(C), pages 430-442.
    4. Žnidarič, Luka & Nusev, Gjorgji & Morel, Bertrand & Mougin, Julie & Juričić, Đani & Boškoski, Pavle, 2021. "Evaluating uncertainties in electrochemical impedance spectra of solid oxide fuel cells," Applied Energy, Elsevier, vol. 298(C).
    5. Luca Del Zotto & Andrea Monforti Ferrario & Arda Hatunoglu & Alessandro Dell’Era & Stephen McPhail & Enrico Bocci, 2021. "Experimental Procedures & First Results of an Innovative Solid Oxide Fuel Cell Test Rig: Parametric Analysis and Stability Test," Energies, MDPI, vol. 14(8), pages 1-19, April.
    6. Gallo, Marco & Polverino, Pierpaolo & Mougin, Julie & Morel, Bertrand & Pianese, Cesare, 2020. "Coupling electrochemical impedance spectroscopy and model-based aging estimation for solid oxide fuel cell stacks lifetime prediction," Applied Energy, Elsevier, vol. 279(C).
    7. Mehr, A.S. & Lanzini, A. & Santarelli, M. & Rosen, Marc A., 2021. "Polygeneration systems based on high temperature fuel cell (MCFC and SOFC) technology: System design, fuel types, modeling and analysis approaches," Energy, Elsevier, vol. 228(C).
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Tanveer, Waqas Hassan & Abdelkareem, Mohammad Ali & Kolosz, Ben W. & Rezk, Hegazy & Andresen, John & Cha, Suk Won & Sayed, Enas Taha, 2021. "The role of vacuum based technologies in solid oxide fuel cell development to utilize industrial waste carbon for power production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 142(C).
    2. Dasheng Lee & Kuan-Chung Lin, 2020. "How to Transform Sustainable Energy Technology into a Unicorn Start-Up: Technology Review and Case Study," Sustainability, MDPI, vol. 12(7), pages 1-26, April.
    3. d'Amore-Domenech, Rafael & Leo, Teresa J. & Pollet, Bruno G., 2021. "Bulk power transmission at sea: Life cycle cost comparison of electricity and hydrogen as energy vectors," Applied Energy, Elsevier, vol. 288(C).
    4. Konstantina Peloriadi & Petros Iliadis & Panagiotis Boutikos & Konstantinos Atsonios & Panagiotis Grammelis & Aristeidis Nikolopoulos, 2022. "Technoeconomic Assessment of LNG-Fueled Solid Oxide Fuel Cells in Small Island Systems: The Patmos Island Case Study," Energies, MDPI, vol. 15(11), pages 1-20, May.
    5. Mingfei Li & Jingjing Wang & Zhengpeng Chen & Xiuyang Qian & Chuanqi Sun & Di Gan & Kai Xiong & Mumin Rao & Chuangting Chen & Xi Li, 2024. "A Comprehensive Review of Thermal Management in Solid Oxide Fuel Cells: Focus on Burners, Heat Exchangers, and Strategies," Energies, MDPI, vol. 17(5), pages 1-30, February.
    6. Serdar Yilmaz & Senel Cobaner & Emine Yalaz & Bahman Amini Horri, 2022. "Synthesis and Characterization of Gadolinium-Doped Zirconia as a Potential Electrolyte for Solid Oxide Fuel Cells," Energies, MDPI, vol. 15(8), pages 1-14, April.
    7. Cormos, Calin-Cristian, 2023. "Green hydrogen production from decarbonized biomass gasification: An integrated techno-economic and environmental analysis," Energy, Elsevier, vol. 270(C).
    8. Li, Feng & Yuan, Yupeng & Yan, Xinping & Malekian, Reza & Li, Zhixiong, 2018. "A study on a numerical simulation of the leakage and diffusion of hydrogen in a fuel cell ship," Renewable and Sustainable Energy Reviews, Elsevier, vol. 97(C), pages 177-185.
    9. de Avila Ferreira, Tafarel & Wuillemin, Zacharie & Faulwasser, Timm & Salzmann, Christophe & Van herle, Jan & Bonvin, Dominique, 2019. "Enforcing optimal operation in solid-oxide fuel-cell systems," Energy, Elsevier, vol. 181(C), pages 281-293.
    10. Nhuchhen, Daya R. & Sit, Song P. & Layzell, David B., 2022. "Towards net-zero emission cement and power production using Molten Carbonate Fuel Cells," Applied Energy, Elsevier, vol. 306(PB).
    11. Hou, Rui & Zhang, Nachuan & Gao, Wei & Chen, Kang & Liu, Yongqiu, 2023. "Thermodynamic, environmental, and exergoeconomic feasibility analyses and optimization of biomass gasifier-solid oxide fuel cell boosting a doable-flash binary geothermal cycle; a novel trigeneration ," Energy, Elsevier, vol. 265(C).
    12. Elmer, Theo & Worall, Mark & Wu, Shenyi & Riffat, Saffa B., 2015. "Fuel cell technology for domestic built environment applications: State of-the-art review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 42(C), pages 913-931.
    13. Pang, Kang Ying & Liew, Peng Yen & Woon, Kok Sin & Ho, Wai Shin & Wan Alwi, Sharifah Rafidah & Klemeš, Jiří Jaromír, 2023. "Multi-period multi-objective optimisation model for multi-energy urban-industrial symbiosis with heat, cooling, power and hydrogen demands," Energy, Elsevier, vol. 262(PA).
    14. Ahmad Baroutaji & Arun Arjunan & John Robinson & Tabbi Wilberforce & Mohammad Ali Abdelkareem & Abdul Ghani Olabi, 2021. "PEMFC Poly-Generation Systems: Developments, Merits, and Challenges," Sustainability, MDPI, vol. 13(21), pages 1-31, October.
    15. Pan, Zehua & Shen, Jian & Wang, Jingyi & Xu, Xinhai & Chan, Wei Ping & Liu, Siyu & Zhou, Yexin & Yan, Zilin & Jiao, Zhenjun & Lim, Teik-Thye & Zhong, Zheng, 2022. "Thermodynamic analyses of a standalone diesel-fueled distributed power generation system based on solid oxide fuel cells," Applied Energy, Elsevier, vol. 308(C).
    16. Fabrizio, Enrico & Seguro, Federico & Filippi, Marco, 2014. "Integrated HVAC and DHW production systems for Zero Energy Buildings," Renewable and Sustainable Energy Reviews, Elsevier, vol. 40(C), pages 515-541.
    17. Ramadhani, F. & Hussain, M.A. & Mokhlis, H. & Hajimolana, S., 2017. "Optimization strategies for Solid Oxide Fuel Cell (SOFC) application: A literature survey," Renewable and Sustainable Energy Reviews, Elsevier, vol. 76(C), pages 460-484.
    18. Ou, Kai & Yuan, Wei-Wei & Kim, Young-Bae, 2021. "Development of optimal energy management for a residential fuel cell hybrid power system with heat recovery," Energy, Elsevier, vol. 219(C).
    19. Sven Gruber & Klemen Rola & Danijela Urbancl & Darko Goričanec, 2023. "Carbon-Free Heat Production for High-Temperature Heating Systems," Sustainability, MDPI, vol. 15(20), pages 1-18, October.
    20. Yuanwu Xu & Hao Shu & Hongchuan Qin & Xiaolong Wu & Jingxuan Peng & Chang Jiang & Zhiping Xia & Yongan Wang & Xi Li, 2022. "Real-Time State of Health Estimation for Solid Oxide Fuel Cells Based on Unscented Kalman Filter," Energies, MDPI, vol. 15(7), pages 1-17, March.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:gam:jeners:v:15:y:2022:i:10:p:3702-:d:818511. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: MDPI Indexing Manager (email available below). General contact details of provider: https://www.mdpi.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.