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Developing an Automated Tool for Quantitative Analysis of the Deconvoluted Electrochemical Impedance Response of a Solid Oxide Fuel Cell

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  • Mohammad Alboghobeish

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy
    Dipartimento di Ingegneria, Università degli Studi di Napoli Parthenope, Centro Direzionale Isola C4, 80143 Napoli, Italy)

  • Andrea Monforti Ferrario

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy
    Department of Industrial Engineering and Mathematical Sciences, Università Politecnica delle Marche, Via Brecce Bianche, 60131 Ancona, Italy)

  • Davide Pumiglia

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy)

  • Massimiliano Della Pietra

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy)

  • Stephen J. McPhail

    (ENEA Department of Energy Technologies and Renewable Sources, Energy Storage, Batteries and Hydrogen Production & Use (TERIN-PSU-ABI), Via Anguillarese, 00123 Rome, Italy)

  • Sergii Pylypko

    (Elcogen AS, Valukoja 23, 11415 Tallinn, Estonia)

  • Domenico Borello

    (Dipartimento di Ingegneria Meccanica e Aerospaziale (DIMA), Sapienza University of Rome, Via Eudossiana, 18, 00184 Roma, Italy)

Abstract

Despite being commercially available, solid oxide fuel cell (SOFC) technology requires further study to understand its physicochemical processes for diagnostics, prognostics, and quality assurance purposes. Electrochemical impedance spectroscopy (EIS), a widely used characterization technique for SOFCs, is often accompanied by the distribution of relaxation times (DRT) as a method for deconvoluting the contribution of each physicochemical process from the aggregated impedance response spectra. While EIS yields valuable information for the operation of SOFCs, the quantitative analysis of the DRT and its shifts remains cumbersome. To address this issue, and to create a replicable benchmark for the assessment of DRT results, a custom tool was developed in MATLAB to numerically analyze the DRT spectra, identify the DRT peaks, and assess their deviation in terms of peak frequency and DRT amplitude from nominal operating conditions. The preliminary validation of the tool was carried out by applying the tool to an extensive experimental campaign on 23 SOFC button-sized samples from three production batches in which EIS measurements were performed in parametric operating conditions. It was concluded that the results of the automated analysis via the developed tool were in accordance with the qualitative analysis of previous studies. It is capable of providing adequate additional quantitative results in terms of DRT shifts for further analysis and provides the basis for better interoperability of DRT analyses between laboratories.

Suggested Citation

  • Mohammad Alboghobeish & Andrea Monforti Ferrario & Davide Pumiglia & Massimiliano Della Pietra & Stephen J. McPhail & Sergii Pylypko & Domenico Borello, 2022. "Developing an Automated Tool for Quantitative Analysis of the Deconvoluted Electrochemical Impedance Response of a Solid Oxide Fuel Cell," Energies, MDPI, vol. 15(10), pages 1-22, May.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:10:p:3702-:d:818511
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    References listed on IDEAS

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