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Crystal Engineering Approach for Fabrication of Inverted Perovskite Solar Cell in Ambient Conditions

Author

Listed:
  • Inga Ermanova

    (LASE—Laboratory of Advanced Solar Energy, National University of Science and Technology “MISiS”, Leninsky Prospect 4, 119049 Moscow, Russia)

  • Narges Yaghoobi Nia

    (CHOSE—Centre for Hybrid and Organic Solar Energy, University of Rome ‘‘Tor Vergata’’, via del Politecnico 1, 00133 Rome, Italy)

  • Enrico Lamanna

    (CHOSE—Centre for Hybrid and Organic Solar Energy, University of Rome ‘‘Tor Vergata’’, via del Politecnico 1, 00133 Rome, Italy)

  • Elisabetta Di Bartolomeo

    (Department of Chemical Science and Technologies, University of Rome Tor Vergata, via della Ricerca Scientifica 1, 00133 Rome, Italy)

  • Evgeny Kolesnikov

    (Department of Functional Nanosystems and High-Temperature Materials, National University of Science and Technology “MISiS”, Leninsky Prospect 4, 119049 Moscow, Russia)

  • Lev Luchnikov

    (LASE—Laboratory of Advanced Solar Energy, National University of Science and Technology “MISiS”, Leninsky Prospect 4, 119049 Moscow, Russia)

  • Aldo Di Carlo

    (LASE—Laboratory of Advanced Solar Energy, National University of Science and Technology “MISiS”, Leninsky Prospect 4, 119049 Moscow, Russia
    CHOSE—Centre for Hybrid and Organic Solar Energy, University of Rome ‘‘Tor Vergata’’, via del Politecnico 1, 00133 Rome, Italy)

Abstract

In this paper, we demonstrate the high potentialities of pristine single-cation and mixed cation/anion perovskite solar cells (PSC) fabricated by sequential method deposition in p-i-n planar architecture (ITO/NiO X /Perovskite/PCBM/BCP/Ag) in ambient conditions. We applied the crystal engineering approach for perovskite deposition to control the quality and crystallinity of the light-harvesting film. The formation of a full converted and uniform perovskite absorber layer from poriferous pre-film on a planar hole transporting layer (HTL) is one of the crucial factors for the fabrication of high-performance PSCs. We show that the in-air sequential deposited MAPbI 3 -based PSCs on planar nickel oxide (NiO X ) permitted to obtain a Power Conversion Efficiency (PCE) exceeding 14% while the (FA,MA,Cs)Pb(I,Br) 3 -based PSC achieved 15.6%. In this paper we also compared the influence of transporting layers on the cell performance by testing material depositions quantity and thickness (for hole transporting layer), and conditions of deposition processes (for electron transporting layer). Moreover, we optimized second step of perovskite deposition by varying the dipping time of substrates into the MA(I,Br) solution. We have shown that the layer by layer deposition of the NiOx is the key point to improve the efficiency for inverted perovskite solar cell out of glove-box using sequential deposition method, increasing the relative efficiency of +26% with respect to reference cells.

Suggested Citation

  • Inga Ermanova & Narges Yaghoobi Nia & Enrico Lamanna & Elisabetta Di Bartolomeo & Evgeny Kolesnikov & Lev Luchnikov & Aldo Di Carlo, 2021. "Crystal Engineering Approach for Fabrication of Inverted Perovskite Solar Cell in Ambient Conditions," Energies, MDPI, vol. 14(6), pages 1-15, March.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:6:p:1751-:d:521753
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    References listed on IDEAS

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    1. Julian Burschka & Norman Pellet & Soo-Jin Moon & Robin Humphry-Baker & Peng Gao & Mohammad K. Nazeeruddin & Michael Grätzel, 2013. "Sequential deposition as a route to high-performance perovskite-sensitized solar cells," Nature, Nature, vol. 499(7458), pages 316-319, July.
    2. Tomas Leijtens & Giles E. Eperon & Sandeep Pathak & Antonio Abate & Michael M. Lee & Henry J. Snaith, 2013. "Overcoming ultraviolet light instability of sensitized TiO2 with meso-superstructured organometal tri-halide perovskite solar cells," Nature Communications, Nature, vol. 4(1), pages 1-8, December.
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