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CO 2 Capture from Flue Gas of a Coal-Fired Power Plant Using Three-Bed PSA Process

Author

Listed:
  • Chu-Yun Cheng

    (Department of Chemical and Materials Engineering, National Central University, Zhongli District, Taoyuan City 320, Taiwan)

  • Chia-Chen Kuo

    (Department of Chemical and Materials Engineering, National Central University, Zhongli District, Taoyuan City 320, Taiwan)

  • Ming-Wei Yang

    (Chemistry and Environment Laboratory, Taiwan Power Research Institute, Shulin District, New Taipei 23847, Taiwan)

  • Zong-Yu Zhuang

    (Chemistry and Environment Laboratory, Taiwan Power Research Institute, Shulin District, New Taipei 23847, Taiwan)

  • Po-Wei Lin

    (Department of Chemical and Materials Engineering, National Central University, Zhongli District, Taoyuan City 320, Taiwan)

  • Yi-Fang Chen

    (Department of Chemical and Materials Engineering, National Central University, Zhongli District, Taoyuan City 320, Taiwan)

  • Hong-Sung Yang

    (Department of Chemical and Materials Engineering, National Central University, Zhongli District, Taoyuan City 320, Taiwan)

  • Cheng-Tung Chou

    (Department of Chemical and Materials Engineering, National Central University, Zhongli District, Taoyuan City 320, Taiwan)

Abstract

The pressure swing adsorption (PSA) process was used to capture carbon dioxide (CO 2 ) from the flue gas of a coal-fired power plant to reduce CO 2 emissions. Herein, CO 2 was captured from flue gas using the PSA process for at least 85 vol% CO 2 purity and with the other exit stream from the process of more than 90 vol% N 2 purity. The extended Langmuir–Freundlich isotherm was used for calculating the equilibrium adsorption capacity, and the linear driving force model was used to describe the gas adsorption kinetics. We compared the results of breakthrough curves obtained through experiments and simulations to verify the accuracy of the mass transfer coefficient. The flue gas obtained after desulphurization and water removal (13.5 vol% CO 2 and 86.5 vol% N 2 ) from a subcritical 1-kW coal-fired power plant served as the feed for the designed three-bed, nine-step PSA process. To determine optimal operating conditions for the process, the central composite design (CCD) was used. After CCD analysis, optimal operating conditions with a feed pressure of 3.66 atm and a vacuum pressure of 0.05 atm were obtained to produce a bottom product with a CO 2 purity of 89.20 vol% and a recovery of 88.20%, and a top product with a N 2 purity of 98.49 vol% and a recovery of 93.56%. The mechanical energy consumption was estimated to be 1.17 GJ/t-CO 2 .

Suggested Citation

  • Chu-Yun Cheng & Chia-Chen Kuo & Ming-Wei Yang & Zong-Yu Zhuang & Po-Wei Lin & Yi-Fang Chen & Hong-Sung Yang & Cheng-Tung Chou, 2021. "CO 2 Capture from Flue Gas of a Coal-Fired Power Plant Using Three-Bed PSA Process," Energies, MDPI, vol. 14(12), pages 1-15, June.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:12:p:3582-:d:575928
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    References listed on IDEAS

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    1. Subraveti, Sai Gokul & Pai, Kasturi Nagesh & Rajagopalan, Ashwin Kumar & Wilkins, Nicholas Stiles & Rajendran, Arvind & Jayaraman, Ambalavan & Alptekin, Gokhan, 2019. "Cycle design and optimization of pressure swing adsorption cycles for pre-combustion CO2 capture," Applied Energy, Elsevier, vol. 254(C).
    2. Rubin, Edward S. & Chen, Chao & Rao, Anand B., 2007. "Cost and performance of fossil fuel power plants with CO2 capture and storage," Energy Policy, Elsevier, vol. 35(9), pages 4444-4454, September.
    3. Burdyny, Thomas & Struchtrup, Henning, 2010. "Hybrid membrane/cryogenic separation of oxygen from air for use in the oxy-fuel process," Energy, Elsevier, vol. 35(5), pages 1884-1897.
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    Cited by:

    1. José Ramón Fernández, 2023. "An Overview of Advances in CO 2 Capture Technologies," Energies, MDPI, vol. 16(3), pages 1-4, February.
    2. Alejandro Lyons Cerón & Alar Konist, 2023. "Co-Pyrolysis of Woody Biomass and Oil Shale in a Batch Reactor in CO 2 , CO 2 -H 2 O, and Ar Atmospheres," Energies, MDPI, vol. 16(7), pages 1-14, March.

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