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Three-Dimensional Fibrous Iron as Anode Current Collector for Rechargeable Zinc–Air Batteries

Author

Listed:
  • Ramin Khezri

    (Department of Chemical Engineering, Faculty of Engineering, Chulalongkorn University, Bangkok 10330, Thailand)

  • Kridsada Jirasattayaporn

    (Department of Chemical Engineering, Faculty of Engineering, Chulalongkorn University, Bangkok 10330, Thailand)

  • Ali Abbasi

    (Department of Chemical Engineering, Faculty of Engineering, Chulalongkorn University, Bangkok 10330, Thailand)

  • Thandavarayan Maiyalagan

    (Department of Chemistry, SRM Institute of Science and Technology, Kattankulathur, Chennai 603203, Tamilnadu, India)

  • Ahmad Azmin Mohamad

    (School of Materials and Mineral Resources Engineering, Universiti of Sains Malaysia, Nibong Tebal 14300, Malaysia)

  • Soorathep Kheawhom

    (Department of Chemical Engineering, Faculty of Engineering, Chulalongkorn University, Bangkok 10330, Thailand
    Research Unit of Advanced Materials for Energy Storage, Chulalongkorn University, Bangkok 10330, Thailand)

Abstract

A three-dimensional (3D) fibrous structure with a high active surface and conductive pathway proved to be an excellent anode current collector for rechargeable zinc–air batteries (ZABs). Herein, a cost-effective and highly stable zinc (Zn) electrode, based on Zn electrodeposited on iron fibers (Zn/IF), is duly examined. Electrochemical characteristics of the proposed electrode are seen to compete with a conventional zinc/nickel foam (Zn/NF) electrode, implying that it can be a suitable alternative for use in ZABs. Results show that the Zn/IF electrode exhibits an almost similar trend as Zn/NF in cyclic voltammetry (CV). Moreover, by using a Zn/IF electrode, electrochemical impedance spectroscopy (EIS) demonstrates lower charge transfer resistance. In the application of a rechargeable ZAB, the fibrous Zn/IF electrode exhibits a high coulombic efficiency (CE) of 78%, close to the conventional Zn/NF (80%), with almost similar capacity and lower charge transfer resistance, after 200 charge/discharge cycles. It is evident that all the positive features of Zn/IF, especially its low cost, shows that it can be a valuable anode for ZABs.

Suggested Citation

  • Ramin Khezri & Kridsada Jirasattayaporn & Ali Abbasi & Thandavarayan Maiyalagan & Ahmad Azmin Mohamad & Soorathep Kheawhom, 2020. "Three-Dimensional Fibrous Iron as Anode Current Collector for Rechargeable Zinc–Air Batteries," Energies, MDPI, vol. 13(6), pages 1-18, March.
    • Handle: RePEc:gam:jeners:v:13:y:2020:i:6:p:1429-:d:334224
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    References listed on IDEAS

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    1. K. David Huang & Thangavel Sangeetha & Wu-Fu Cheng & Chunyo Lin & Po-Tuan Chen, 2018. "Computational Fluid Dynamics Approach for Performance Prediction in a Zinc–Air Fuel Cell," Energies, MDPI, vol. 11(9), pages 1-13, August.
    2. Zeng, Xianlai & Li, Jinhui & Liu, Lili, 2015. "Solving spent lithium-ion battery problems in China: Opportunities and challenges," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 1759-1767.
    3. Wade, N.S. & Taylor, P.C. & Lang, P.D. & Jones, P.R., 2010. "Evaluating the benefits of an electrical energy storage system in a future smart grid," Energy Policy, Elsevier, vol. 38(11), pages 7180-7188, November.
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    Cited by:

    1. Khezri, Ramin & Motlagh, Shiva Rezaei & Etesami, Mohammad & Pakawanit, Phakkhananan & Olaru, Sorin & Somwangthanaroj, Anongnat & Kheawhom, Soorathep, 2024. "Balancing current density and electrolyte flow for improved zinc-air battery cyclability," Applied Energy, Elsevier, vol. 376(PA).
    2. Khezri, Ramin & Motlagh, Shiva Rezaei & Etesami, Mohammad & Mohamad, Ahmad Azmin & Pornprasertsuk, Rojana & Olaru, Sorin & Kheawhom, Soorathep, 2023. "High current density charging of zinc-air flow batteries: Investigating the impact of flow rate and current density on zinc electrodeposition," Applied Energy, Elsevier, vol. 348(C).

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