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Polysilane-Inserted Methylammonium Lead Iodide Perovskite Solar Cells Doped with Formamidinium and Potassium

Author

Listed:
  • Takeo Oku

    (Department of Materials Science, The University of Shiga Prefecture, 2500 Hassaka, Hikone, Shiga 522-8533, Japan)

  • Satsuki Kandori

    (Department of Materials Science, The University of Shiga Prefecture, 2500 Hassaka, Hikone, Shiga 522-8533, Japan)

  • Masaya Taguchi

    (Department of Materials Science, The University of Shiga Prefecture, 2500 Hassaka, Hikone, Shiga 522-8533, Japan)

  • Atsushi Suzuki

    (Department of Materials Science, The University of Shiga Prefecture, 2500 Hassaka, Hikone, Shiga 522-8533, Japan)

  • Masanobu Okita

    (Osaka Gas Chemicals Co., Ltd., 5-11-61 Torishima, Konohana-ku, Osaka 554-0051, Japan)

  • Satoshi Minami

    (Osaka Gas Chemicals Co., Ltd., 5-11-61 Torishima, Konohana-ku, Osaka 554-0051, Japan)

  • Sakiko Fukunishi

    (Osaka Gas Chemicals Co., Ltd., 5-11-61 Torishima, Konohana-ku, Osaka 554-0051, Japan)

  • Tomoharu Tachikawa

    (Osaka Gas Chemicals Co., Ltd., 5-11-61 Torishima, Konohana-ku, Osaka 554-0051, Japan)

Abstract

Polysilane-inserted CH 3 NH 3 PbI 3 perovskite photovoltaic devices combined with potassium and formamidinium iodides were fabricated and characterized. Decaphenylcyclopentasilane layers were inserted at the perovskite/hole transport interface and annealed across a temperature range of 180–220 °C. These polysilane-coated cells prevented PbI 2 formation, and the conversion efficiencies were improved over extended periods of time.

Suggested Citation

  • Takeo Oku & Satsuki Kandori & Masaya Taguchi & Atsushi Suzuki & Masanobu Okita & Satoshi Minami & Sakiko Fukunishi & Tomoharu Tachikawa, 2020. "Polysilane-Inserted Methylammonium Lead Iodide Perovskite Solar Cells Doped with Formamidinium and Potassium," Energies, MDPI, vol. 13(18), pages 1-11, September.
    • Handle: RePEc:gam:jeners:v:13:y:2020:i:18:p:4776-:d:412949
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    References listed on IDEAS

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    1. Zhaolai Chen & Qingfeng Dong & Ye Liu & Chunxiong Bao & Yanjun Fang & Yun Lin & Shi Tang & Qi Wang & Xun Xiao & Yang Bai & Yehao Deng & Jinsong Huang, 2017. "Thin single crystal perovskite solar cells to harvest below-bandgap light absorption," Nature Communications, Nature, vol. 8(1), pages 1-7, December.
    2. Alexander D. Jodlowski & Cristina Roldán-Carmona & Giulia Grancini & Manuel Salado & Maryline Ralaiarisoa & Shahzada Ahmad & Norbert Koch & Luis Camacho & Gustavo de Miguel & Mohammad Khaja Nazeeruddi, 2017. "Large guanidinium cation mixed with methylammonium in lead iodide perovskites for 19% efficient solar cells," Nature Energy, Nature, vol. 2(12), pages 972-979, December.
    3. Tae-Hee Han & Jin-Wook Lee & Chungseok Choi & Shaun Tan & Changsoo Lee & Yepin Zhao & Zhenghong Dai & Nicholas Marco & Sung-Joon Lee & Sang-Hoon Bae & Yonghai Yuan & Hyuck Mo Lee & Yu Huang & Yang Yan, 2019. "Perovskite-polymer composite cross-linker approach for highly-stable and efficient perovskite solar cells," Nature Communications, Nature, vol. 10(1), pages 1-10, December.
    4. Dongqin Bi & Chenyi Yi & Jingshan Luo & Jean-David Décoppet & Fei Zhang & Shaik Mohammed Zakeeruddin & Xiong Li & Anders Hagfeldt & Michael Grätzel, 2016. "Polymer-templated nucleation and crystal growth of perovskite films for solar cells with efficiency greater than 21%," Nature Energy, Nature, vol. 1(10), pages 1-5, October.
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