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Comprehensive Aging Analysis of Volumetric Constrained Lithium-Ion Pouch Cells with High Concentration Silicon-Alloy Anodes

Author

Listed:
  • Lysander De Sutter

    (ETEC Department & MOBI Research Group, Vrije Universiteit Brussel (VUB), Pleinlaan 2, 1050 Brussel, Belgium—VUB-MOBI is a Core Lab Member of Flanders Make)

  • Gert Berckmans

    (ETEC Department & MOBI Research Group, Vrije Universiteit Brussel (VUB), Pleinlaan 2, 1050 Brussel, Belgium—VUB-MOBI is a Core Lab Member of Flanders Make)

  • Mario Marinaro

    (ZSW, Zentrum für Sonnenenergie- und Wasserstoff-Forschung BW, Helmholtzstraße 8, 89081 Ulm, Germany)

  • Jelle Smekens

    (ETEC Department & MOBI Research Group, Vrije Universiteit Brussel (VUB), Pleinlaan 2, 1050 Brussel, Belgium—VUB-MOBI is a Core Lab Member of Flanders Make)

  • Yousef Firouz

    (ETEC Department & MOBI Research Group, Vrije Universiteit Brussel (VUB), Pleinlaan 2, 1050 Brussel, Belgium—VUB-MOBI is a Core Lab Member of Flanders Make)

  • Margret Wohlfahrt-Mehrens

    (ZSW, Zentrum für Sonnenenergie- und Wasserstoff-Forschung BW, Helmholtzstraße 8, 89081 Ulm, Germany)

  • Joeri Van Mierlo

    (ETEC Department & MOBI Research Group, Vrije Universiteit Brussel (VUB), Pleinlaan 2, 1050 Brussel, Belgium—VUB-MOBI is a Core Lab Member of Flanders Make)

  • Noshin Omar

    (ETEC Department & MOBI Research Group, Vrije Universiteit Brussel (VUB), Pleinlaan 2, 1050 Brussel, Belgium—VUB-MOBI is a Core Lab Member of Flanders Make)

Abstract

In this research, twenty-four high capacity (1360 mAh) NMC622/Si-alloy Li-ion full pouch cells with high silicon-alloy content (55%) are cycle aged under seven different cycling conditions to study the effect of different stressors on the cycle life of Si-anode full cells, among which are the effect of ambient temperature, Depth of Discharge (DoD) and the discharge current. The cells are volumetrically constrained at an optimal initial pressure to improve their cycle life, energy and power capabilities. Furthermore, the innovative test setup allows measuring the developed pressure as a result of repeated (de-)lithiation during battery cycling. This uniquely vast testing campaign on Si-anode full cells allows us to study and quantify independently the influence of different stress factors on their cycle life for the first time, as well as to develop a new capacity fade model based on an observed linear relationship between capacity retention and total discharge capacity throughput.

Suggested Citation

  • Lysander De Sutter & Gert Berckmans & Mario Marinaro & Jelle Smekens & Yousef Firouz & Margret Wohlfahrt-Mehrens & Joeri Van Mierlo & Noshin Omar, 2018. "Comprehensive Aging Analysis of Volumetric Constrained Lithium-Ion Pouch Cells with High Concentration Silicon-Alloy Anodes," Energies, MDPI, vol. 11(11), pages 1-21, October.
    • Handle: RePEc:gam:jeners:v:11:y:2018:i:11:p:2948-:d:178979
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    References listed on IDEAS

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    1. de Hoog, Joris & Timmermans, Jean-Marc & Ioan-Stroe, Daniel & Swierczynski, Maciej & Jaguemont, Joris & Goutam, Shovon & Omar, Noshin & Van Mierlo, Joeri & Van Den Bossche, Peter, 2017. "Combined cycling and calendar capacity fade modeling of a Nickel-Manganese-Cobalt Oxide Cell with real-life profile validation," Applied Energy, Elsevier, vol. 200(C), pages 47-61.
    2. Hannan, M.A. & Lipu, M.S.H. & Hussain, A. & Mohamed, A., 2017. "A review of lithium-ion battery state of charge estimation and management system in electric vehicle applications: Challenges and recommendations," Renewable and Sustainable Energy Reviews, Elsevier, vol. 78(C), pages 834-854.
    3. Ximing Cheng & Michael Pecht, 2017. "In Situ Stress Measurement Techniques on Li-ion Battery Electrodes: A Review," Energies, MDPI, vol. 10(5), pages 1-19, April.
    4. Omar, Noshin & Monem, Mohamed Abdel & Firouz, Yousef & Salminen, Justin & Smekens, Jelle & Hegazy, Omar & Gaulous, Hamid & Mulder, Grietus & Van den Bossche, Peter & Coosemans, Thierry & Van Mierlo, J, 2014. "Lithium iron phosphate based battery – Assessment of the aging parameters and development of cycle life model," Applied Energy, Elsevier, vol. 113(C), pages 1575-1585.
    5. Jalkanen, K. & Karppinen, J. & Skogström, L. & Laurila, T. & Nisula, M. & Vuorilehto, K., 2015. "Cycle aging of commercial NMC/graphite pouch cells at different temperatures," Applied Energy, Elsevier, vol. 154(C), pages 160-172.
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    2. Xingyu Zhang & Jian Chen & Yinhua Bao, 2022. "Model-Based Investigations of Porous Si-Based Anodes for Lithium-Ion Batteries with Effects of Volume Changes," Energies, MDPI, vol. 15(23), pages 1-18, November.
    3. Imanol Landa-Medrano & Idoia Urdampilleta & Iker Castrillo & Hans-Jürgen Grande & Iratxe de Meatza & Aitor Eguia-Barrio, 2024. "Making Room for Silicon: Including SiO x in a Graphite-Based Anode Formulation and Harmonization in 1 Ah Cells," Energies, MDPI, vol. 17(7), pages 1-21, March.
    4. Hyungeun Seo & Kyungbae Kim & Jae-Hun Kim, 2020. "Spherical Sb Core/Nb 2 O 5 -C Double-Shell Structured Composite as an Anode Material for Li Secondary Batteries," Energies, MDPI, vol. 13(8), pages 1-10, April.

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