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An overview on fast pyrolysis of the main constituents in lignocellulosic biomass to valued-added chemicals: Structures, pathways and interactions

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  • Shen, Dekui
  • Jin, Wei
  • Hu, Jun
  • Xiao, Rui
  • Luo, Kaihong

Abstract

Considering the huge demand of energy for social economic development and deterioration of environment due to extensive utilization of fossil fuels, green and renewable energy sources are standing in the centre for alleviating the mentioned pressure and diversifying the global energy supply. “Pyrolysis”, as one of the promising thermo-chemical conversion technologies, could convert biomass to value-added chemicals and fuels in forms of solid, liquid and gas. Fast pyrolysis of the main constituents in biomass (polysaccharides and lignin averagely accounting for 90wt%), involving the yield of liquid/solid/gas products, distribution of prominent oxygenate compounds, their formation pathways associated with the chemical structure of highly polymerized macromolecules, would be vigorously discussed in this review work, helping to improve the understanding of pyrolytic behavior of biomass, optimize the thermal conversion process and so on. Meanwhile, the interaction among the components during pyrolytic process was evidenced and briefly overviewed, in order to shorten the distance between the pyrolysis of biomass and pyrolytic behavior of its main components and design the new-concept co-pyrolysis process for promoting the production of oxygenated compounds. The challenges and wayforward in the field are addressed in estimating the formation priority of specific oxygenate compounds and developing new technology for producing the value-added compounds (chemicals) in high yields.

Suggested Citation

  • Shen, Dekui & Jin, Wei & Hu, Jun & Xiao, Rui & Luo, Kaihong, 2015. "An overview on fast pyrolysis of the main constituents in lignocellulosic biomass to valued-added chemicals: Structures, pathways and interactions," Renewable and Sustainable Energy Reviews, Elsevier, vol. 51(C), pages 761-774.
    • Handle: RePEc:eee:rensus:v:51:y:2015:i:c:p:761-774
    DOI: 10.1016/j.rser.2015.06.054
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    1. Kirubakaran, V. & Sivaramakrishnan, V. & Nalini, R. & Sekar, T. & Premalatha, M. & Subramanian, P., 2009. "A review on gasification of biomass," Renewable and Sustainable Energy Reviews, Elsevier, vol. 13(1), pages 179-186, January.
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    13. Kabir, G. & Hameed, B.H., 2017. "Recent progress on catalytic pyrolysis of lignocellulosic biomass to high-grade bio-oil and bio-chemicals," Renewable and Sustainable Energy Reviews, Elsevier, vol. 70(C), pages 945-967.
    14. Xin, Shanzhi & Huang, Fang & Qi, Wei & Mi, Tie, 2020. "Pyrolysis of torrefied herbal medicine wastes: Characterization of pyrolytic products," Energy, Elsevier, vol. 210(C).
    15. Perkins, Greg & Bhaskar, Thallada & Konarova, Muxina, 2018. "Process development status of fast pyrolysis technologies for the manufacture of renewable transport fuels from biomass," Renewable and Sustainable Energy Reviews, Elsevier, vol. 90(C), pages 292-315.
    16. Pang, Yunhui & Zhu, Xiaoli & Li, Ning & Wang, Zhenbo, 2024. "Microscopic mechanism for CO2-assisted co-gasification of polyethylene and softwood lignin: A reactive force field molecular dynamics study," Energy, Elsevier, vol. 289(C).
    17. Liu, Ruijia & Liu, Guijian & Yousaf, Balal & Niu, Zhiyuan & Abbas, Qumber, 2022. "Novel investigation of pyrolysis mechanisms and kinetics for functional groups in biomass matrix," Renewable and Sustainable Energy Reviews, Elsevier, vol. 153(C).
    18. Pang, Yunhui & Zhu, Xiaoli & Li, Ning & Wang, Zhenbo, 2023. "Investigation on reaction mechanism for CO2 gasification of softwood lignin by ReaxFF MD method," Energy, Elsevier, vol. 267(C).
    19. Tu, Ren & Sun, Yan & Wu, Yujian & Fan, Xudong & Cheng, Shuchao & Jiang, Enchen & Xu, Xiwei, 2021. "Selective production of furfural and phenols from rice husk: the influence of synergetic pretreatments with different order," Renewable Energy, Elsevier, vol. 168(C), pages 297-308.
    20. Gorugantu SriBala & Hans‐Heinrich Carstensen & Kevin M. Van Geem & Guy B. Marin, 2019. "Measuring biomass fast pyrolysis kinetics: State of the art," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 8(2), March.

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