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Coupled biomass (lignin) gasification and iron ore reduction: A novel approach for biomass conversion and application

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  • Wei, Rufei
  • Feng, Shanghuan
  • Long, Hongming
  • Li, Jiaxin
  • Yuan, Zhongshun
  • Cang, Daqiang
  • Xu, Chunbao (Charles)

Abstract

Aiming at a novel application of biomass, coupled biomass gasification and iron ore reduction was investigated and demonstrated in this work through pyrolysis/gasification of iron ore–lignin pellets (ILP) at 1093–1333 K. The solid, liquid and gaseous products were analyzed by XRD, SEM, chemical analysis, GC-MS, GC and TG-FTIR. Direct reduction iron (DRI) and gaseous products (CO, H2 and CH4) were produced in the process. The metallization degree of the iron ore and CO content of the gaseous products increased with increasing the reaction temperature, as expected. The gas yield from the experiments with ILP was much higher than that from the tests with lignin pellets (LP) at 1173–1333 K, owing mainly to the iron ore reduction producing a larger amount of CO. Whereas, the yields of oil and char in the ILP reduction process were found to be much lower than those from the tests with lignin alone, due to the conversion of oil and char products into gaseous products catalyzed by the iron oxide and metallic iron. Thus, in pyrolysis/gasification of ILP the presence of lignin provided reducing agents for reduction of iron oxide, whereas the presence of iron oxide/metallic iron provided an oxidant/catalyst for biomass gasification.

Suggested Citation

  • Wei, Rufei & Feng, Shanghuan & Long, Hongming & Li, Jiaxin & Yuan, Zhongshun & Cang, Daqiang & Xu, Chunbao (Charles), 2017. "Coupled biomass (lignin) gasification and iron ore reduction: A novel approach for biomass conversion and application," Energy, Elsevier, vol. 140(P1), pages 406-414.
    • Handle: RePEc:eee:energy:v:140:y:2017:i:p1:p:406-414
    DOI: 10.1016/j.energy.2017.08.080
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    References listed on IDEAS

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    1. Kang, Shimin & Li, Xianglan & Fan, Juan & Chang, Jie, 2013. "Hydrothermal conversion of lignin: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 27(C), pages 546-558.
    2. Strezov, Vladimir, 2006. "Iron ore reduction using sawdust: Experimental analysis and kinetic modelling," Renewable Energy, Elsevier, vol. 31(12), pages 1892-1905.
    3. Wei, Rufei & Zhang, Lingling & Cang, Daqiang & Li, Jiaxin & Li, Xianwei & Xu, Chunbao Charles, 2017. "Current status and potential of biomass utilization in ferrous metallurgical industry," Renewable and Sustainable Energy Reviews, Elsevier, vol. 68(P1), pages 511-524.
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    1. Hongbo Du, & Deng, Fang & Kommalapati, Raghava R. & Amarasekara, Ananda S., 2020. "Iron based catalysts in biomass processing," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).
    2. Wei, Rufei & Xiang, Dongwen & Long, Hongming & Xu, Chunbao (Charles) & Li, Jiaxin, 2020. "Reduction of iron oxide by lignin: Characteristics, kinetics and superiority," Energy, Elsevier, vol. 197(C).
    3. Cardoso, J. & Silva, V. & Eusébio, D. & Brito, P. & Hall, M.J. & Tarelho, L., 2018. "Comparative scaling analysis of two different sized pilot-scale fluidized bed reactors operating with biomass substrates," Energy, Elsevier, vol. 151(C), pages 520-535.
    4. El Hage, Hicham & Herez, Amal & Ramadan, Mohamad & Bazzi, Hassan & Khaled, Mahmoud, 2018. "An investigation on solar drying: A review with economic and environmental assessment," Energy, Elsevier, vol. 157(C), pages 815-829.
    5. Wei, Rufei & Meng, Kangzheng & Long, Hongming & Xu, ChunbaoCharles, 2024. "Biomass metallurgy: A sustainable and green path to a carbon-neutral metallurgical industry," Renewable and Sustainable Energy Reviews, Elsevier, vol. 199(C).
    6. Guanyong Sun & Bin Li & Hanjie Guo & Wensheng Yang & Shaoying Li & Jing Guo, 2020. "Thermodynamic Study on Reduction of Iron Oxides by H 2 + CO + CH 4 + N 2 Mixture at 900 °C," Energies, MDPI, vol. 13(19), pages 1-18, September.

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