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Hybridization of solid oxide electrolysis-based power-to-methane with oxyfuel combustion and carbon dioxide utilization for energy storage

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  • Eveloy, Valerie

Abstract

The storage of excess or low-carbon electricity in the form of synthetic gas using power-to-gas technologies is a promising approach to enable high shares of renewables in power generation and reduce the fuel carbon content. However, the efficiency of standalone, low-temperature electrolysis-based power-to-methane (PtM) processes is presently limited. As a way of enhancing the potential of this technology to support the decarbonization of energy systems, this study investigates a high-temperature electrolysis-based PtM process and its integration with oxyfuel combustion to co-generate synthetic methane, heat and power. The system incorporates in-situ heat, oxygen, carbon dioxide (CO2) and water recycling. The energy and exergy-based performance of the compound system and its main structures are investigated using an overpotential-based electrochemical model. Depending on electrolysis operating temperature (800–1000 °C) and pressure (1–10 bar), overall energy and exergy efficiencies range from 75.8% to 79.3% and 64.5% to 67.4%, respectively. In quasi-continuous operation, a 6.4 MWe (AC input) hybrid PtM system would avoid approximately 1.9 GWhe of electricity consumption for oxygen-air separation, and sink 6.6 kt of CO2 from the oxyfuel co-generation plant annually. In parallel, 3.1 MWth of heat could be recovered from the pre-methanation compressor and oxyfuel conversion products for use in external applications. Based on a carbon balance evaluation from initial resource extraction to SNG conversion, the PtM-oxyfuel hybridization investigated could effectively contribute to raise the electricity greenhouse gas (GHG) emission threshold below which SNG could environmentally compete with natural gas, relative to low-temperature electrolysis-based PtM and conventional post-combustion CO2 capture.

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  • Eveloy, Valerie, 2019. "Hybridization of solid oxide electrolysis-based power-to-methane with oxyfuel combustion and carbon dioxide utilization for energy storage," Renewable and Sustainable Energy Reviews, Elsevier, vol. 108(C), pages 550-571.
    • Handle: RePEc:eee:rensus:v:108:y:2019:i:c:p:550-571
    DOI: 10.1016/j.rser.2019.02.027
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    6. Jorge Perpiñán & Manuel Bailera & Luis M. Romeo & Begoña Peña & Valerie Eveloy, 2021. "CO 2 Recycling in the Iron and Steel Industry via Power-to-Gas and Oxy-Fuel Combustion," Energies, MDPI, vol. 14(21), pages 1-15, October.
    7. Bailera, Manuel & Peña, Begoña & Lisbona, Pilar & Marín, Julián & Romeo, Luis M., 2021. "Lab-scale experimental tests of power to gas-oxycombustion hybridization: System design and preliminary results," Energy, Elsevier, vol. 226(C).
    8. Zhaojian Liang & Jingyi Wang & Keda Ren & Zhenjun Jiao & Meng Ni & Liang An & Yang Wang & Jinbin Yang & Mengying Li, 2024. "Discovering two general characteristic times of transient responses in solid oxide cells," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
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