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Ionic liquid coupled with nickel salt for enhancing the hydro-liquefaction efficiency of the major biomass components

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  • Li, Qingyin
  • Zhang, Shu
  • Wang, Yi
  • Xiang, Jun
  • Hu, Song
  • Yuan, Xiangzhou
  • Gholizadeh, Mortaza
  • Hu, Xun

Abstract

Ionic liquid combined with metal species is considered as a promising catalytic system for biomass liquefaction, which complies with the requirement of green chemistry and promotes utilization of biomass resources. The catalytic systems containing imidazolium-based ionic liquids and nickel chloride were applied to the hydro-liquefaction of major biomass constituents (cellulose, xylan and lignin) in this work. The anion type in ionic liquid played a vital role in the liquefaction of feedstock. The results indicated that the maximum conversion and bio-oil yield were achieved in 1-butyl-3-methylimidazolium bromide ([BMIM]Br)/NiCl2 system, which was attributed to the strong nucleophile and coordinating capacity of bromide ion. The ionic liquid-based catalyst was more effective in the conversion of cellulose and xylan, due to their high reactivity. Additionally, the ionic liquid-based catalyst facilitated the thermal degradation of feedstocks and intermediates, resulting in the increased content of organics with the smaller molecular sizes. The deoxy-hydrogenation reaction was enhanced over ionic liquid-based catalyst, improving the quality of the resulting bio-oils.

Suggested Citation

  • Li, Qingyin & Zhang, Shu & Wang, Yi & Xiang, Jun & Hu, Song & Yuan, Xiangzhou & Gholizadeh, Mortaza & Hu, Xun, 2021. "Ionic liquid coupled with nickel salt for enhancing the hydro-liquefaction efficiency of the major biomass components," Renewable Energy, Elsevier, vol. 175(C), pages 296-306.
    • Handle: RePEc:eee:renene:v:175:y:2021:i:c:p:296-306
    DOI: 10.1016/j.renene.2021.04.143
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    References listed on IDEAS

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