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Thermodynamic equilibrium analysis of H2-rich syngas production via sorption-enhanced chemical looping biomass gasification

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  • Chein, Rei-Yu
  • Hsu, Wen-Huai

Abstract

In this study, thermodynamic equilibrium analysis of the sorption-enhanced chemical looping biomass gasification (SE-CL-BG) using Fe2O3 as the oxygen carrier, CaO as the CO2 sorbent, and CO2 or H2O as the gasifying agent for producing H2 rich syngas was conducted. Based on the amount of OC introduced, highly selective syngas can only result when a small amount of oxygen carrier is introduced. Due to carbon and hydrogen oxidations, the yields of CO and H2, cold gas efficiency, and the second-law efficiency of SE-CL-BG case were found to be lower than the conventional biomass gasification case in which no oxygen carrier and CO2 sorbent were introduced. Compared with conventional biomass gasification, the advantage of SE-CL-BG is that biomass gasification can be operated at lower temperatures (500–750 °C) with higher H2 yield due to the enhanced water-gas shift reaction and lower heat duty due to heat release from the CO2 absorption reaction. The computed results indicated that CaO loses the ability to absorb CO2 as the temperature becomes higher than 800 °C.

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  • Chein, Rei-Yu & Hsu, Wen-Huai, 2020. "Thermodynamic equilibrium analysis of H2-rich syngas production via sorption-enhanced chemical looping biomass gasification," Renewable Energy, Elsevier, vol. 153(C), pages 117-129.
    • Handle: RePEc:eee:renene:v:153:y:2020:i:c:p:117-129
    DOI: 10.1016/j.renene.2019.10.097
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    2. Osat, Mohammad & Shojaati, Faryar & Osat, Mojtaba, 2023. "A solar-biomass system associated with CO2 capture, power generation and waste heat recovery for syngas production from rice straw and microalgae: Technological, energy, exergy, exergoeconomic and env," Applied Energy, Elsevier, vol. 340(C).
    3. Osat, Mohammad & Shojaati, Faryar & Osat, Mojtaba, 2023. "Techno-economic assessment of butanol and pentanol productions from sorption enhanced chemical looping gasification of a lignocellulosic biomass," Renewable Energy, Elsevier, vol. 217(C).
    4. Gao, Ningbo & Śliz, Maciej & Quan, Cui & Bieniek, Artur & Magdziarz, Aneta, 2021. "Biomass CO2 gasification with CaO looping for syngas production in a fixed-bed reactor," Renewable Energy, Elsevier, vol. 167(C), pages 652-661.
    5. Wan, Zhanghao & Hu, Jianhang & Qi, Xianjin, 2021. "Numerical analysis of hydrodynamics and thermochemical property of biomass gasification in a pilot-scale circulating fluidized bed," Energy, Elsevier, vol. 225(C).
    6. Laixing Luo & Xing Zheng & Jianye Wang & Wu Qin & Xianbin Xiao & Zongming Zheng, 2021. "Catalyzed Ethanol Chemical Looping Gasification Mechanism on the Perfect and Reduced Fe 2 O 3 Surfaces," Energies, MDPI, vol. 14(6), pages 1-15, March.
    7. Adnan, Muflih A. & Hossain, Mohammad M. & Kibria, Md Golam, 2020. "Biomass upgrading to high-value chemicals via gasification and electrolysis: A thermodynamic analysis," Renewable Energy, Elsevier, vol. 162(C), pages 1367-1379.

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