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Adiabatic effects in nucleation near the gas-liquid critical point

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  • Onuki, Akira

Abstract

Nucleation near the gas-liquid critical point sensitively depends on whether the pressure or the volume is fixed. Upon decompression to a constant pressure, bulk nucleation can well be induced from a gas state, whereas phase separation from a liquid state is more easily triggered in the thermal diffusion layer near the boundary. In this case bulk nucleation in a metastable gas is described by the classical Lifshitz-Slyozov theory. On the other hand, upon cooling of the boundary temperature under the fixed-volume condition, bulk nucleation can be realized in a liquid and a modified Lifshitz-Slyozov theory follows. However, if a gas is cooled from the boundary at a fixed volume, phase separation readily occurs in the thermal diffusion layer, apparently suggesting no metastability in a gas in agreement with previous experiments.

Suggested Citation

  • Onuki, Akira, 1996. "Adiabatic effects in nucleation near the gas-liquid critical point," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 234(1), pages 189-205.
    • Handle: RePEc:eee:phsmap:v:234:y:1996:i:1:p:189-205
    DOI: 10.1016/S0378-4371(96)00262-2
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