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Oxygen and hydrogen productivities and repeatable reactivity of 30-mol%-Fe-, Co-, Ni-, Mn-doped CeO2−δ for thermochemical two-step water-splitting cycle

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  • Gokon, Nobuyuki
  • Suda, Toshinori
  • Kodama, Tatsuya

Abstract

The characteristics of oxygen/hydrogen productivity using 30-mol%-M (M = Fe, Co, Ni, Mn)-doped CeO2−δ (30-mol%-M-CeO2−δ) were studied for the thermochemical two-step water splitting cycle comprising TR (thermal reduction) at 1500 °C and WD (water decomposition) at 1150 °C. The reproducibility of oxygen evolution was evaluated using 30-mol%-M-CeO2−δ and the effects of different M dopants were compared in the TR temperature range of 1200–1500 °C. Two solid phases detected in the 30-mol%-M- CeO2−δ powders were involved in the redox reaction of the thermochemical two-step water splitting cycle. Among the M-CeO2−δ samples evaluated, Mn-doped CeO2−δ provided the most stable and reproducible results and the highest reactivity for oxygen evolution at all temperatures employed for the TR step of the thermochemical two-step water-splitting cycle.

Suggested Citation

  • Gokon, Nobuyuki & Suda, Toshinori & Kodama, Tatsuya, 2015. "Oxygen and hydrogen productivities and repeatable reactivity of 30-mol%-Fe-, Co-, Ni-, Mn-doped CeO2−δ for thermochemical two-step water-splitting cycle," Energy, Elsevier, vol. 90(P2), pages 1280-1289.
    • Handle: RePEc:eee:energy:v:90:y:2015:i:p2:p:1280-1289
    DOI: 10.1016/j.energy.2015.06.085
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    References listed on IDEAS

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    1. Agrafiotis, Christos & Roeb, Martin & Sattler, Christian, 2015. "A review on solar thermal syngas production via redox pair-based water/carbon dioxide splitting thermochemical cycles," Renewable and Sustainable Energy Reviews, Elsevier, vol. 42(C), pages 254-285.
    2. Kaneko, H. & Miura, T. & Ishihara, H. & Taku, S. & Yokoyama, T. & Nakajima, H. & Tamaura, Y., 2007. "Reactive ceramics of CeO2–MOx (M=Mn, Fe, Ni, Cu) for H2 generation by two-step water splitting using concentrated solar thermal energy," Energy, Elsevier, vol. 32(5), pages 656-663.
    3. Rosen, Marc A., 2010. "Advances in hydrogen production by thermochemical water decomposition: A review," Energy, Elsevier, vol. 35(2), pages 1068-1076.
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    5. Guene Lougou, Bachirou & Shuai, Yong & Zhang, Hao & Ahouannou, Clément & Zhao, Jiupeng & Kounouhewa, Basile Bruno & Tan, Heping, 2020. "Thermochemical CO2 reduction over NiFe2O4@alumina filled reactor heated by high-flux solar simulator," Energy, Elsevier, vol. 197(C).

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