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High-efficiency dye-sensitized solar cells based on electrospun TiO2 multi-layered composite film photoanodes

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  • Wang, Guanxi
  • Xiao, Wei
  • Yu, Jiaguo

Abstract

High-efficiency DSSCs (dye-sensitized solar cells) based on multi-layered composite film photoanodes consisting of the TiO2 blocking layer, the commercial Degussa P25 nanoparticles layer and 1D (one-dimensional) TiO2 nanorods layer were fabricated. The 1D TiO2 nanorods were prepared by a simple electrospinning technology and grinding process. The photovoltaic properties of different DSSCs based on nanoparticles/nanoparticles (DNP), nanorods/nanorods (DNR) and nanoparticles/nanorods (NPR) photoanodes were investigated and their photoelectric conversion efficiencies were 6.37, 4.92 and 8.03%. The dye-sensitized solar cells based on NPR photoanodes exhibited the best photovoltaic performance with a short-circuit current of 15.7 mA cm−2. The enhanced photo-electricity performance of NPR solar cells could be attributed to the synergistic effect of following factors. (1) The P25 underlayer ensured intimate contact in DSSCs films structure and superior dye adsorption. (2) The nanorods overlayer with 1D structure showed strong light scattering ability, which significantly enhanced light harvesting efficiency. In addition, the 1D geometry of TiO2 nanorods provided a fast and long charge carrier transfer pathway, thus improving the transfer of photo-induced electrons in the DSSCs.

Suggested Citation

  • Wang, Guanxi & Xiao, Wei & Yu, Jiaguo, 2015. "High-efficiency dye-sensitized solar cells based on electrospun TiO2 multi-layered composite film photoanodes," Energy, Elsevier, vol. 86(C), pages 196-203.
    • Handle: RePEc:eee:energy:v:86:y:2015:i:c:p:196-203
    DOI: 10.1016/j.energy.2015.03.127
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    References listed on IDEAS

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    1. Cauda, Valentina & Pugliese, Diego & Garino, Nadia & Sacco, Adriano & Bianco, Stefano & Bella, Federico & Lamberti, Andrea & Gerbaldi, Claudio, 2014. "Multi-functional energy conversion and storage electrodes using flower-like Zinc oxide nanostructures," Energy, Elsevier, vol. 65(C), pages 639-646.
    2. Yue, Gentian & Wang, Lei & Zhang, Xin'an & Wu, Jihuai & Jiang, Qiwei & Zhang, Weifeng & Huang, Miaoliang & Lin, Jianming, 2014. "Fabrication of high performance multi-walled carbon nanotubes/polypyrrole counter electrode for dye-sensitized solar cells," Energy, Elsevier, vol. 67(C), pages 460-467.
    3. Yue, Gentian & Wu, Jihuai & Xiao, Yaoming & Lin, Jianming & Huang, Miaoliang & Lan, Zhang & Fan, Leqing, 2013. "Functionalized graphene/poly(3,4-ethylenedioxythiophene):polystyrenesulfonate as counter electrode catalyst for dye-sensitized solar cells," Energy, Elsevier, vol. 54(C), pages 315-321.
    4. Francis, L. & Sreekumaran Nair, A. & Jose, R. & Ramakrishna, S. & Thavasi, V. & Marsano, E., 2011. "Fabrication and characterization of dye-sensitized solar cells from rutile nanofibers and nanorods," Energy, Elsevier, vol. 36(1), pages 627-632.
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    1. Alami, Abdul Hai & Rajab, Bilal & Aokal, Kamilia, 2017. "Assessment of silver nanowires infused with zinc oxide as a transparent electrode for dye-sensitized solar cell applications," Energy, Elsevier, vol. 139(C), pages 1231-1236.
    2. Hosseinnezhad, Mozhgan & Gharanjig, Kamaladin & Moradian, Siamak & Saeb, Mohammad Reza, 2017. "In quest of power conversion efficiency in nature-inspired dye-sensitized solar cells: Individual, co-sensitized or tandem configuration?," Energy, Elsevier, vol. 134(C), pages 864-870.
    3. Liu, Qin & Zhu, Jinghui & Zhang, Liwen & Qiu, Yejun, 2018. "Recent advances in energy materials by electrospinning," Renewable and Sustainable Energy Reviews, Elsevier, vol. 81(P2), pages 1825-1858.
    4. Alami, Abdul Hai & Rajab, Bilal & Abed, Jehad & Faraj, Mohammed & Hawili, Abdullah Abu & Alawadhi, Hussain, 2019. "Investigating various copper oxides-based counter electrodes for dye sensitized solar cell applications," Energy, Elsevier, vol. 174(C), pages 526-533.
    5. Ghorbani, Masoomeh & Solaimany Nazar, Ali Reza & Farhadian, Mehrdad & Tangestaninejad, Shahram, 2023. "Efficient tetracycline degradation and electricity production in photocatalytic fuel cell based on ZnO nanorod/BiOBr/UiO-66-NH2 photoanode and Cu2O/CuO photocathode," Energy, Elsevier, vol. 272(C).
    6. Zainal Arifin & Suyitno Suyitno & Syamsul Hadi & Bayu Sutanto, 2018. "Improved Performance of Dye-Sensitized Solar Cells with TiO 2 Nanoparticles/Zn-Doped TiO 2 Hollow Fiber Photoanodes," Energies, MDPI, vol. 11(11), pages 1-11, October.

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