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Ion transport membrane reactors for oxy-combustion–Part II: Analysis and comparison of alternatives

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  • Mancini, N.D.
  • Mitsos, A.

Abstract

In order to design ITM-based oxy-combustion power cycles, various reactor engineering analyses must be conducted with detailed modeling and simulation. An intermediate-fidelity ITM model is used to explore the dependence of ITM performance on reactor geometric structure, flow configuration, operating conditions, membrane material properties, and uncertainty in key modeling assumptions, such as the dominant fuel conversion mechanism. Many operational constraints are presented that are usually overlooked by black-box modeling strategies, and the implications of these constraints are explored. Further, a comparison is made between reactive and separation-only ITMs to assess the relative merits and disadvantages of each. The results show that although a reactive ITM significantly improves the partial pressure driving force, practical reactor engineering considerations indicate that this concept is not superior to counter-current separation-only ITMs, mainly because of the stringent temperature limitations of the membrane material. A Second Law assessment of certain ITM configurations is performed to evaluate the potential of ITM technology to reduce the air separation penalty, and to provide insight for effective systems-level integration. Overall, the results of our analyses capture the essential characteristics of ITM air separation systems for power cycles, and enable detailed systems-level studies to be performed.

Suggested Citation

  • Mancini, N.D. & Mitsos, A., 2011. "Ion transport membrane reactors for oxy-combustion–Part II: Analysis and comparison of alternatives," Energy, Elsevier, vol. 36(8), pages 4721-4739.
    • Handle: RePEc:eee:energy:v:36:y:2011:i:8:p:4721-4739
    DOI: 10.1016/j.energy.2011.05.024
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    1. Mancini, N.D. & Mitsos, A., 2011. "Ion transport membrane reactors for oxy-combustion – Part I: intermediate-fidelity modeling," Energy, Elsevier, vol. 36(8), pages 4701-4720.
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    1. Mansir, Ibrahim B. & Ben-Mansour, Rached & Habib, Mohamed A., 2018. "Oxy-fuel combustion in a two-pass oxygen transport reactor for fire tube boiler application," Applied Energy, Elsevier, vol. 229(C), pages 828-840.
    2. Mancini, N.D. & Mitsos, A., 2011. "Ion transport membrane reactors for oxy-combustion – Part I: intermediate-fidelity modeling," Energy, Elsevier, vol. 36(8), pages 4701-4720.
    3. Nemitallah, Medhat A. & Habib, Mohamed A. & Mezghani, K., 2015. "Experimental and numerical study of oxygen separation and oxy-combustion characteristics inside a button-cell LNO-ITM reactor," Energy, Elsevier, vol. 84(C), pages 600-611.
    4. Ben Mansour, R. & Nemitallah, M.A. & Habib, M.A., 2013. "Numerical investigation of oxygen permeation and methane oxy-combustion in a stagnation flow ion transport membrane reactor," Energy, Elsevier, vol. 54(C), pages 322-332.
    5. Habib, Mohamed A. & Nemitallah, Medhat A., 2015. "Design of an ion transport membrane reactor for application in fire tube boilers," Energy, Elsevier, vol. 81(C), pages 787-801.
    6. Habib, Mohamed A. & Imteyaz, Binash & Nemitallah, Medhat A., 2020. "Second law analysis of premixed and non-premixed oxy-fuel combustion cycles utilizing oxygen separation membranes," Applied Energy, Elsevier, vol. 259(C).
    7. Shin, Donghwan & Kang, Sanggyu, 2018. "Numerical analysis of an ion transport membrane system for oxy–fuel combustion," Applied Energy, Elsevier, vol. 230(C), pages 875-888.
    8. Gunasekaran, S. & Mancini, N.D. & El-Khaja, R. & Sheu, E.J. & Mitsos, A., 2014. "Solar–thermal hybridization of advanced zero emissions power cycle," Energy, Elsevier, vol. 65(C), pages 152-165.
    9. Siefert, Nicholas S. & Litster, Shawn, 2013. "Exergy and economic analyses of advanced IGCC–CCS and IGFC–CCS power plants," Applied Energy, Elsevier, vol. 107(C), pages 315-328.
    10. Kotowicz, Janusz & Job, Marcin & Brzęczek, Mateusz, 2020. "Thermodynamic analysis and optimization of an oxy-combustion combined cycle power plant based on a membrane reactor equipped with a high-temperature ion transport membrane ITM," Energy, Elsevier, vol. 205(C).
    11. Te Zhao & Chusheng Chen & Hong Ye, 2021. "CFD Simulation of Hydrogen Generation and Methane Combustion Inside a Water Splitting Membrane Reactor," Energies, MDPI, vol. 14(21), pages 1-17, November.
    12. Turi, Davide Maria & Chiesa, Paolo & Macchi, Ennio & Ghoniem, Ahmed F., 2016. "High fidelity model of the oxygen flux across ion transport membrane reactor: Mechanism characterization using experimental data," Energy, Elsevier, vol. 96(C), pages 127-141.
    13. Habib, Mohamed A. & Nemitallah, Medhat A. & Ahmed, Pervez & Sharqawy, Mostafa H. & Badr, Hassan M. & Muhammad, Inam & Yaqub, Mohamed, 2015. "Experimental analysis of oxygen-methane combustion inside a gas turbine reactor under various operating conditions," Energy, Elsevier, vol. 86(C), pages 105-114.
    14. Gunasekaran, S. & Mancini, N.D. & Mitsos, A., 2014. "Optimal design and operation of membrane-based oxy-combustion power plants," Energy, Elsevier, vol. 70(C), pages 338-354.
    15. Fu, Chao & Gundersen, Truls, 2012. "Using exergy analysis to reduce power consumption in air separation units for oxy-combustion processes," Energy, Elsevier, vol. 44(1), pages 60-68.
    16. Habib, Mohamed A. & Salaudeen, Shakirudeen A. & Nemitallah, Medhat A. & Ben-Mansour, R. & Mokheimer, Esmail M.A., 2016. "Numerical investigation of syngas oxy-combustion inside a LSCF-6428 oxygen transport membrane reactor," Energy, Elsevier, vol. 96(C), pages 654-665.
    17. Ahmed, Pervez & Habib, Mohamed A. & Ben-Mansour, Rached & Kirchen, Patrick & Ghoniem, Ahmed F., 2014. "CFD (computational fluid dynamics) analysis of a novel reactor design using ion transport membranes for oxy-fuel combustion," Energy, Elsevier, vol. 77(C), pages 932-944.

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    2. Turi, Davide Maria & Chiesa, Paolo & Macchi, Ennio & Ghoniem, Ahmed F., 2016. "High fidelity model of the oxygen flux across ion transport membrane reactor: Mechanism characterization using experimental data," Energy, Elsevier, vol. 96(C), pages 127-141.
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    11. Gunasekaran, S. & Mancini, N.D. & El-Khaja, R. & Sheu, E.J. & Mitsos, A., 2014. "Solar–thermal hybridization of advanced zero emissions power cycle," Energy, Elsevier, vol. 65(C), pages 152-165.
    12. Habib, Mohamed A. & Imteyaz, Binash & Nemitallah, Medhat A., 2020. "Second law analysis of premixed and non-premixed oxy-fuel combustion cycles utilizing oxygen separation membranes," Applied Energy, Elsevier, vol. 259(C).
    13. Fu, Chao & Gundersen, Truls, 2012. "Using exergy analysis to reduce power consumption in air separation units for oxy-combustion processes," Energy, Elsevier, vol. 44(1), pages 60-68.
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