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The effects of sub-critical and super-critical carbon dioxide adsorption-induced coal matrix swelling on the permeability of naturally fractured black coal

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  • Perera, M.S.A.
  • Ranjith, P.G.
  • Choi, S.K.
  • Airey, D.

Abstract

Swelling of the coal matrix with the adsorption of CO2 is one of the leading problems for CO2 sequestration in deep coal seams as it causes coal seam permeability to be significantly reduced. The main objective of this study was to investigate the effect of coal mass swelling on the permeability of naturally fractured black coal. A series of permeability tests were conducted using a newly developed tri-axial apparatus on 38mm by 76mm naturally fractured black coal specimens. These tests were carried out for CO2 and N2 injections at 2–20MPa injection pressures under 10 to 24MPa confining pressures at 33°C. Each coal specimen was then allowed to swell under sub-critical and super-critical CO2 adsorption and the corresponding effects on CO2 and N2 permeabilities were examined. Results indicate that the permeability of naturally fractured black coal is significantly reduced due to matrix swelling, which starts as quickly as within 1h of CO2 injection. A further reduction is then observed, and the maximum swelling rate occurs within the first 3–4h of CO2 adsorption. The amount of coal matrix swelling due to CO2 adsorption clearly depends on the phase condition of the CO2, and super-critical CO2 adsorption-induced swelling is about two times higher than that induced by sub-critical CO2 adsorption. Interestingly, although a fractured coal specimen which has already fully swelled under sub-critical CO2 adsorption can swell significantly more under super-critical CO2 adsorption, after swelling under super-critical CO2 adsorption, no further swelling effect occurs under any CO2 pressure or phase condition. Moreover, the swelling process continues longer under super-critical CO2 adsorption. It is concluded that super-critical CO2 adsorption can induce more matrix swelling than sub-critical CO2 adsorption under the same adsorption pressure.

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  • Perera, M.S.A. & Ranjith, P.G. & Choi, S.K. & Airey, D., 2011. "The effects of sub-critical and super-critical carbon dioxide adsorption-induced coal matrix swelling on the permeability of naturally fractured black coal," Energy, Elsevier, vol. 36(11), pages 6442-6450.
    • Handle: RePEc:eee:energy:v:36:y:2011:i:11:p:6442-6450
    DOI: 10.1016/j.energy.2011.09.023
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    15. Psaltis, Steven & Farrell, Troy & Burrage, Kevin & Burrage, Pamela & McCabe, Peter & Moroney, Timothy & Turner, Ian & Mazumder, Saikat, 2015. "Mathematical modelling of gas production and compositional shift of a CSG (coal seam gas) field: Local model development," Energy, Elsevier, vol. 88(C), pages 621-635.
    16. Qiao Lyu & Xinping Long & Pathegama Gamage Ranjith & Yong Kang, 2016. "Unconventional Gas: Experimental Study of the Influence of Subcritical Carbon Dioxide on the Mechanical Properties of Black Shale," Energies, MDPI, vol. 9(7), pages 1-15, July.
    17. Vishal, V. & Singh, Lokendra & Pradhan, S.P. & Singh, T.N. & Ranjith, P.G., 2013. "Numerical modeling of Gondwana coal seams in India as coalbed methane reservoirs substituted for carbon dioxide sequestration," Energy, Elsevier, vol. 49(C), pages 384-394.
    18. Perera, M.S.A. & Ranjith, P.G. & Viete, D.R., 2013. "Effects of gaseous and super-critical carbon dioxide saturation on the mechanical properties of bituminous coal from the Southern Sydney Basin," Applied Energy, Elsevier, vol. 110(C), pages 73-81.
    19. Enbin Liu & Xudong Lu & Daocheng Wang, 2023. "A Systematic Review of Carbon Capture, Utilization and Storage: Status, Progress and Challenges," Energies, MDPI, vol. 16(6), pages 1-48, March.
    20. Zhou, Yan & Guan, Wei & Cong, Peichao & Sun, Qiji, 2022. "Effects of heterogeneous pore closure on the permeability of coal involving adsorption-induced swelling: A micro pore-scale simulation," Energy, Elsevier, vol. 258(C).
    21. Zhou, Yinbo & Zhang, Ruilin & Huang, Jilei & Li, Zenghua & Chen, Zhao & Zhao, Zhou & Hong, Yidu, 2020. "Influence of alkaline solution injection for wettability and permeability of coal with CO2 injection," Energy, Elsevier, vol. 202(C).

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